Multiple Wurtzite Twinning in CdTe Nanocrystals Induced by Methylphosphonic Acid
Branching in semiconductor nanocrystals, which leads to tetrapods and to more complex architectures, is the subject of intensive investigation. Here we support the model according to which branching in CdTe nanocrystals is driven by the formation of multiple wurtzite twins. This is in contrast to pr...
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| Published in | Journal of the American Chemical Society Vol. 128; no. 3; pp. 748 - 755 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Washington, DC
American Chemical Society
25.01.2006
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Branching in semiconductor nanocrystals, which leads to tetrapods and to more complex architectures, is the subject of intensive investigation. Here we support the model according to which branching in CdTe nanocrystals is driven by the formation of multiple wurtzite twins. This is in contrast to previous models for this material. We found that twinning, as well as anisotropic growth, can be triggered by the presence of suitable molecules, such as for instance methylphosphonic acid. In the case of CdTe nanocrystals, we designed a robust growth scheme in which the variation of a single parameter (the concentration of methylphosphonic acid in solution) leads to the controlled formation of nanocrystals with shapes ranging from spheres to anisotropic structures with varying level of branching, as both twinning and anisotropic growth are progressively favored. We believe that these concepts can be extended to other nanocrystal systems. |
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| AbstractList | Branching in semiconductor nanocrystals, which leads to tetrapods and to more complex architectures, is the subject of intensive investigation. Here we support the model according to which branching in CdTe nanocrystals is driven by the formation of multiple wurtzite twins. This is in contrast to previous models for this material. We found that twinning, as well as anisotropic growth, can be triggered by the presence of suitable molecules, such as for instance methylphosphonic acid. In the case of CdTe nanocrystals, we designed a robust growth scheme in which the variation of a single parameter (the concentration of methylphosphonic acid in solution) leads to the controlled formation of nanocrystals with shapes ranging from spheres to anisotropic structures with varying level of branching, as both twinning and anisotropic growth are progressively favored. We believe that these concepts can be extended to other nanocrystal systems. Branching in semiconductor nanocrystals, which leads to tetrapods and to more complex architectures, is the subject of intensive investigation. Here we support the model according to which branching in CdTe nanocrystals is driven by the formation of multiple wurtzite twins. This is in contrast to previous models for this material. We found that twinning, as well as anisotropic growth, can be triggered by the presence of suitable molecules, such as for instance methylphosphonic acid. In the case of CdTe nanocrystals, we designed a robust growth scheme in which the variation of a single parameter (the concentration of methylphosphonic acid in solution) leads to the controlled formation of nanocrystals with shapes ranging from spheres to anisotropic structures with varying level of branching, as both twinning and anisotropic growth are progressively favored. We believe that these concepts can be extended to other nanocrystal systems.Branching in semiconductor nanocrystals, which leads to tetrapods and to more complex architectures, is the subject of intensive investigation. Here we support the model according to which branching in CdTe nanocrystals is driven by the formation of multiple wurtzite twins. This is in contrast to previous models for this material. We found that twinning, as well as anisotropic growth, can be triggered by the presence of suitable molecules, such as for instance methylphosphonic acid. In the case of CdTe nanocrystals, we designed a robust growth scheme in which the variation of a single parameter (the concentration of methylphosphonic acid in solution) leads to the controlled formation of nanocrystals with shapes ranging from spheres to anisotropic structures with varying level of branching, as both twinning and anisotropic growth are progressively favored. We believe that these concepts can be extended to other nanocrystal systems. |
| Author | Kudera, Stefan Carlino, Elvio Cingolani, Roberto Carbone, Luigi Giannini, Cinzia Parak, Wolfgang J Manna, Liberato |
| Author_xml | – sequence: 1 givenname: Luigi surname: Carbone fullname: Carbone, Luigi – sequence: 2 givenname: Stefan surname: Kudera fullname: Kudera, Stefan – sequence: 3 givenname: Elvio surname: Carlino fullname: Carlino, Elvio – sequence: 4 givenname: Wolfgang J surname: Parak fullname: Parak, Wolfgang J – sequence: 5 givenname: Cinzia surname: Giannini fullname: Giannini, Cinzia – sequence: 6 givenname: Roberto surname: Cingolani fullname: Cingolani, Roberto – sequence: 7 givenname: Liberato surname: Manna fullname: Manna, Liberato |
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| Keywords | Crystal growth Pseudopotential methods Theoretical study Transition elements Compounds Nanostructures Experimental study Transmission electron microscopy II-VI semiconductors Cadmium tellurides Density functional method Wurtzite structure Colloidal crystals Crystal nucleation Ab initio calculations Local density approximation Growth twin |
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| Snippet | Branching in semiconductor nanocrystals, which leads to tetrapods and to more complex architectures, is the subject of intensive investigation. Here we support... |
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| SubjectTerms | Cross-disciplinary physics: materials science; rheology Exact sciences and technology Growth from solutions Materials science Methods of crystal growth; physics of crystal growth Physics Theory and models of crystal growth; physics of crystal growth, crystal morphology and orientation |
| Title | Multiple Wurtzite Twinning in CdTe Nanocrystals Induced by Methylphosphonic Acid |
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