Common Origin of Green Luminescence in Carbon Nanodots and Graphene Quantum Dots
Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origi...
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| Published in | ACS nano Vol. 8; no. 3; pp. 2541 - 2547 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
25.03.2014
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origin in these fluorescent carbon nanomaterials is one of the important matters of current debates. Here, a common origin of green luminescence in these C-dots and GQDs is unraveled by ultrafast spectroscopy. According to the change of surface functional groups during surface chemical reduction experiments, which are also accompanied by obvious emission-type transform, these common green luminescence emission centers that emerge in these C-dots and GQDs synthesized by bottom-up and top-down methods are unambiguously assigned to special edge states consisting of several carbon atoms on the edge of carbon backbone and functional groups with CO (carbonyl and carboxyl groups). Our findings further suggest that the competition among various emission centers (bright edge states) and traps dominates the optical properties of these fluorescent carbon nanomaterials. |
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| AbstractList | Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origin in these fluorescent carbon nanomaterials is one of the important matters of current debates. Here, a common origin of green luminescence in these C-dots and GQDs is unraveled by ultrafast spectroscopy. According to the change of surface functional groups during surface chemical reduction experiments, which are also accompanied by obvious emission-type transform, these common green luminescence emission centers that emerge in these C-dots and GQDs synthesized by bottom-up and top-down methods are unambiguously assigned to special edge states consisting of several carbon atoms on the edge of carbon backbone and functional groups with C═O (carbonyl and carboxyl groups). Our findings further suggest that the competition among various emission centers (bright edge states) and traps dominates the optical properties of these fluorescent carbon nanomaterials.Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origin in these fluorescent carbon nanomaterials is one of the important matters of current debates. Here, a common origin of green luminescence in these C-dots and GQDs is unraveled by ultrafast spectroscopy. According to the change of surface functional groups during surface chemical reduction experiments, which are also accompanied by obvious emission-type transform, these common green luminescence emission centers that emerge in these C-dots and GQDs synthesized by bottom-up and top-down methods are unambiguously assigned to special edge states consisting of several carbon atoms on the edge of carbon backbone and functional groups with C═O (carbonyl and carboxyl groups). Our findings further suggest that the competition among various emission centers (bright edge states) and traps dominates the optical properties of these fluorescent carbon nanomaterials. Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origin in these fluorescent carbon nanomaterials is one of the important matters of current debates. Here, a common origin of green luminescence in these C-dots and GQDs is unraveled by ultrafast spectroscopy. According to the change of surface functional groups during surface chemical reduction experiments, which are also accompanied by obvious emission-type transform, these common green luminescence emission centers that emerge in these C-dots and GQDs synthesized by bottom-up and top-down methods are unambiguously assigned to special edge states consisting of several carbon atoms on the edge of carbon backbone and functional groups with C=O (carbonyl and carboxyl groups). Our findings further suggest that the competition among various emission centers (bright edge states) and traps dominates the optical properties of these fluorescent carbon nanomaterials. Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origin in these fluorescent carbon nanomaterials is one of the important matters of current debates. Here, a common origin of green luminescence in these C-dots and GQDs is unraveled by ultrafast spectroscopy. According to the change of surface functional groups during surface chemical reduction experiments, which are also accompanied by obvious emission-type transform, these common green luminescence emission centers that emerge in these C-dots and GQDs synthesized by bottom-up and top-down methods are unambiguously assigned to special edge states consisting of several carbon atoms on the edge of carbon backbone and functional groups with CO (carbonyl and carboxyl groups). Our findings further suggest that the competition among various emission centers (bright edge states) and traps dominates the optical properties of these fluorescent carbon nanomaterials. Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by solvothermally cutting graphene oxide, are three kinds of typical green fluorescence carbon nanomaterials. Insight into the photoluminescence origin in these fluorescent carbon nanomaterials is one of the important matters of current debates. Here, a common origin of green luminescence in these C-dots and GQDs is unraveled by ultrafast spectroscopy. According to the change of surface functional groups during surface chemical reduction experiments, which are also accompanied by obvious emission-type transform, these common green luminescence emission centers that emerge in these C-dots and GQDs synthesized by bottom-up and top-down methods are unambiguously assigned to special edge states consisting of several carbon atoms on the edge of carbon backbone and functional groups with C═O (carbonyl and carboxyl groups). Our findings further suggest that the competition among various emission centers (bright edge states) and traps dominates the optical properties of these fluorescent carbon nanomaterials. |
| Author | Chen, Qi-Dai Han, Wei Xu, Huai-Liang Zhu, Shou-Jun Sun, Hong-Bo Qu, Song-Nan Zhang, Jun-Hu Wang, Lei Wang, Hai-Yu Zhang, Yong-Lai Yang, Bai |
| AuthorAffiliation | College of Physics Jilin University Chinese Academy of Sciences State Key Laboratory on Integrated Optoelectronics, College of Electronic Science and Engineering State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry |
| AuthorAffiliation_xml | – name: State Key Laboratory on Integrated Optoelectronics, College of Electronic Science and Engineering – name: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry – name: Jilin University – name: College of Physics – name: Chinese Academy of Sciences |
| Author_xml | – sequence: 1 givenname: Lei surname: Wang fullname: Wang, Lei – sequence: 2 givenname: Shou-Jun surname: Zhu fullname: Zhu, Shou-Jun – sequence: 3 givenname: Hai-Yu surname: Wang fullname: Wang, Hai-Yu email: hbsun@jlu.edu.cn, haiyu_wang@jlu.edu.cn, byangchem@jlu.edu.cn – sequence: 4 givenname: Song-Nan surname: Qu fullname: Qu, Song-Nan – sequence: 5 givenname: Yong-Lai surname: Zhang fullname: Zhang, Yong-Lai – sequence: 6 givenname: Jun-Hu surname: Zhang fullname: Zhang, Jun-Hu – sequence: 7 givenname: Qi-Dai surname: Chen fullname: Chen, Qi-Dai – sequence: 8 givenname: Huai-Liang surname: Xu fullname: Xu, Huai-Liang – sequence: 9 givenname: Wei surname: Han fullname: Han, Wei – sequence: 10 givenname: Bai surname: Yang fullname: Yang, Bai email: hbsun@jlu.edu.cn, haiyu_wang@jlu.edu.cn, byangchem@jlu.edu.cn – sequence: 11 givenname: Hong-Bo surname: Sun fullname: Sun, Hong-Bo email: hbsun@jlu.edu.cn, haiyu_wang@jlu.edu.cn, byangchem@jlu.edu.cn |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24517361$$D View this record in MEDLINE/PubMed |
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| Copyright | Copyright © 2014 American Chemical Society |
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| Snippet | Carbon nanodots (C-dots) synthesized by electrochemical ablation and small molecule carbonization, as well as graphene quantum dots (GQDs) fabricated by... |
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| SubjectTerms | Carbon Fluorescence Functional groups Graphene Luminescence Nanomaterials Nanostructure Origins Quantum dots |
| Title | Common Origin of Green Luminescence in Carbon Nanodots and Graphene Quantum Dots |
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