Imaging the Nonlinear Plasmoemission Dynamics of Electrons from Strong Plasmonic Fields

We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused purely by the plasmonic field (termed “plasmoemission”). We find from time-resolved imaging that nonlinear plasmoemission is dominated by the...

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Published inNano letters Vol. 17; no. 11; pp. 6569 - 6574
Main Authors Podbiel, Daniel, Kahl, Philip, Makris, Andreas, Frank, Bettina, Sindermann, Simon, Davis, Timothy J, Giessen, Harald, Hoegen, Michael Horn-von, Meyer zu Heringdorf, Frank-J
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 08.11.2017
Subjects
photoemission
Time-resolved photoemission microscopy
plasmoemission
above-threshold photoemission
surface plasmon polariton
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Abstract We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused purely by the plasmonic field (termed “plasmoemission”). We find from time-resolved imaging that nonlinear plasmoemission is dominated by the transverse plasmon field component by utilizing a transient standing wave from two counter-propagating plasmon pulses of opposite transverse spin. From plasmonic foci on flat metal surfaces, we observe highly nonlinear plasmoemission up to the fifth power of intensity and quantized energy transfer, which reflects the quantum-mechanical nature of surface plasmons. Our work constitutes the basis for novel plasmonic devices such as nanometer-confined ultrafast electron sources as well as applications in time-resolved electron microscopy.
AbstractList We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused purely by the plasmonic field (termed "plasmoemission"). We find from time-resolved imaging that nonlinear plasmoemission is dominated by the transverse plasmon field component by utilizing a transient standing wave from two counter-propagating plasmon pulses of opposite transverse spin. From plasmonic foci on flat metal surfaces, we observe highly nonlinear plasmoemission up to the fifth power of intensity and quantized energy transfer, which reflects the quantum-mechanical nature of surface plasmons. Our work constitutes the basis for novel plasmonic devices such as nanometer-confined ultrafast electron sources as well as applications in time-resolved electron microscopy.We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused purely by the plasmonic field (termed "plasmoemission"). We find from time-resolved imaging that nonlinear plasmoemission is dominated by the transverse plasmon field component by utilizing a transient standing wave from two counter-propagating plasmon pulses of opposite transverse spin. From plasmonic foci on flat metal surfaces, we observe highly nonlinear plasmoemission up to the fifth power of intensity and quantized energy transfer, which reflects the quantum-mechanical nature of surface plasmons. Our work constitutes the basis for novel plasmonic devices such as nanometer-confined ultrafast electron sources as well as applications in time-resolved electron microscopy.
We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused purely by the plasmonic field (termed "plasmoemission"). We find from time-resolved imaging that nonlinear plasmoemission is dominated by the transverse plasmon field component by utilizing a transient standing wave from two counter-propagating plasmon pulses of opposite transverse spin. From plasmonic foci on flat metal surfaces, we observe highly nonlinear plasmoemission up to the fifth power of intensity and quantized energy transfer, which reflects the quantum-mechanical nature of surface plasmons. Our work constitutes the basis for novel plasmonic devices such as nanometer-confined ultrafast electron sources as well as applications in time-resolved electron microscopy.
Author Kahl, Philip
Giessen, Harald
Podbiel, Daniel
Meyer zu Heringdorf, Frank-J
Frank, Bettina
Davis, Timothy J
Sindermann, Simon
Hoegen, Michael Horn-von
Makris, Andreas
AuthorAffiliation University of Stuttgart
University of Duisburg-Essen
Fourth Physics Institute and Research Center SCoPE
Faculty of Physics and CENIDE
School of Physics
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/28945435$$D View this record in MEDLINE/PubMed
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Time-resolved photoemission microscopy
plasmoemission
above-threshold photoemission
surface plasmon polariton
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Snippet We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused...
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Title Imaging the Nonlinear Plasmoemission Dynamics of Electrons from Strong Plasmonic Fields
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