Highly Luminescent and Photostable Quantum Dot–Silica Monolith and Its Application to Light-Emitting Diodes
A highly luminescent and photostable quantum dot–silica monolith (QD–SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed sol–gel condensation of silica. The SM was heavily doped with 6-mercaptohexanol exchanged QDs up to 12 vol % (26 wt %) without particle aggreg...
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| Published in | ACS nano Vol. 7; no. 2; pp. 1472 - 1477 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
26.02.2013
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A highly luminescent and photostable quantum dot–silica monolith (QD–SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed sol–gel condensation of silica. The SM was heavily doped with 6-mercaptohexanol exchanged QDs up to 12 vol % (26 wt %) without particle aggregation. Propylamine catalyst was important in maintaining the original luminescence of the QDs in the SM during sol–gel condensation. The silica layer was a good barrier against oxygen and moisture, so that the QD–SM maintained its initial luminescence after high-power UV radiation (∼1 W) for 200 h and through the 150 °C LED encapsulant curing process. Green and red light-emitting QD–SMs were applied as color-converting layers on blue LEDs, and the external quantum efficiency reached up to 89% for the green QD–SM and 63% for the red one. A white LED made with a mixture of green and red QDs in the SM, in which the color coordinate was adjusted at (0.23, 0.21) in CIE1931 color space for a backlight application, showed an efficacy of 47 lm/W, the highest value yet reported. |
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| AbstractList | A highly luminescent and photostable quantum dot-silica monolith (QD-SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed sol-gel condensation of silica. The SM was heavily doped with 6-mercaptohexanol exchanged QDs up to 12 vol % (26 wt %) without particle aggregation. Propylamine catalyst was important in maintaining the original luminescence of the QDs in the SM during sol-gel condensation. The silica layer was a good barrier against oxygen and moisture, so that the QD-SM maintained its initial luminescence after high-power UV radiation (1 W) for 200 h and through the 150 degree C LED encapsulant curing process. Green and red light-emitting QD-SMs were applied as color-converting layers on blue LEDs, and the external quantum efficiency reached up to 89% for the green QD-SM and 63% for the red one. A white LED made with a mixture of green and red QDs in the SM, in which the color coordinate was adjusted at (0.23, 0.21) in CIE1931 color space for a backlight application, showed an efficacy of 47 lm/W, the highest value yet reported. A highly luminescent and photostable quantum dot–silica monolith (QD–SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed sol–gel condensation of silica. The SM was heavily doped with 6-mercaptohexanol exchanged QDs up to 12 vol % (26 wt %) without particle aggregation. Propylamine catalyst was important in maintaining the original luminescence of the QDs in the SM during sol–gel condensation. The silica layer was a good barrier against oxygen and moisture, so that the QD–SM maintained its initial luminescence after high-power UV radiation (∼1 W) for 200 h and through the 150 °C LED encapsulant curing process. Green and red light-emitting QD–SMs were applied as color-converting layers on blue LEDs, and the external quantum efficiency reached up to 89% for the green QD–SM and 63% for the red one. A white LED made with a mixture of green and red QDs in the SM, in which the color coordinate was adjusted at (0.23, 0.21) in CIE1931 color space for a backlight application, showed an efficacy of 47 lm/W, the highest value yet reported. A highly luminescent and photostable quantum dot-silica monolith (QD-SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed sol-gel condensation of silica. The SM was heavily doped with 6-mercaptohexanol exchanged QDs up to 12 vol % (26 wt %) without particle aggregation. Propylamine catalyst was important in maintaining the original luminescence of the QDs in the SM during sol-gel condensation. The silica layer was a good barrier against oxygen and moisture, so that the QD-SM maintained its initial luminescence after high-power UV radiation (∼1 W) for 200 h and through the 150 °C LED encapsulant curing process. Green and red light-emitting QD-SMs were applied as color-converting layers on blue LEDs, and the external quantum efficiency reached up to 89% for the green QD-SM and 63% for the red one. A white LED made with a mixture of green and red QDs in the SM, in which the color coordinate was adjusted at (0.23, 0.21) in CIE1931 color space for a backlight application, showed an efficacy of 47 lm/W, the highest value yet reported.A highly luminescent and photostable quantum dot-silica monolith (QD-SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed sol-gel condensation of silica. The SM was heavily doped with 6-mercaptohexanol exchanged QDs up to 12 vol % (26 wt %) without particle aggregation. Propylamine catalyst was important in maintaining the original luminescence of the QDs in the SM during sol-gel condensation. The silica layer was a good barrier against oxygen and moisture, so that the QD-SM maintained its initial luminescence after high-power UV radiation (∼1 W) for 200 h and through the 150 °C LED encapsulant curing process. Green and red light-emitting QD-SMs were applied as color-converting layers on blue LEDs, and the external quantum efficiency reached up to 89% for the green QD-SM and 63% for the red one. A white LED made with a mixture of green and red QDs in the SM, in which the color coordinate was adjusted at (0.23, 0.21) in CIE1931 color space for a backlight application, showed an efficacy of 47 lm/W, the highest value yet reported. |
| Author | Lee, Junho Jun, Shinae Jang, Eunjoo |
| AuthorAffiliation | Samsung Electronics Co |
| AuthorAffiliation_xml | – name: Samsung Electronics Co |
| Author_xml | – sequence: 1 givenname: Shinae surname: Jun fullname: Jun, Shinae – sequence: 2 givenname: Junho surname: Lee fullname: Lee, Junho – sequence: 3 givenname: Eunjoo surname: Jang fullname: Jang, Eunjoo email: ejjang12@samsung.com |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23363407$$D View this record in MEDLINE/PubMed |
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| Snippet | A highly luminescent and photostable quantum dot–silica monolith (QD–SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed... A highly luminescent and photostable quantum dot-silica monolith (QD-SM) substance was prepared by preliminary surface exchange of the QDs and base-catalyzed... |
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| SubjectTerms | Agglomeration Color Condensing Curing Exchange Luminescence Nanostructure Quantum dots Silicon dioxide Sol gel process |
| Title | Highly Luminescent and Photostable Quantum Dot–Silica Monolith and Its Application to Light-Emitting Diodes |
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