Ultrastable FeCo Bifunctional Electrocatalyst on Se-Doped CNTs for Liquid and Flexible All-Solid-State Rechargeable Zn–Air Batteries

The rechargeable Zn–air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge to develop non-noble metal bifunctional catalysts with high oxygen reduction as well as oxygen evolution reaction (ORR and OER) activity and...

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Published inNano letters Vol. 21; no. 5; pp. 2255 - 2264
Main Authors Zhang, Hongwei, Zhao, Meiqi, Liu, Haoran, Shi, Shuangrui, Wang, Zhenhua, Zhang, Biao, Song, Lin, Shang, Jingzhi, Yang, Yong, Ma, Chao, Zheng, Lirong, Han, Yunhu, Huang, Wei
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 10.03.2021
Subjects
Se-doped CNTs
liquid and flexible solid rechargeable Zn−air batteries
bifunctional oxygen electrocatalyst
outstanding durability
gravity guided CVD strategy
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Abstract The rechargeable Zn–air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge to develop non-noble metal bifunctional catalysts with high oxygen reduction as well as oxygen evolution reaction (ORR and OER) activity and superior durability, which limit the large-scale application of rechargeable Zn–air batteries. Herein, we synthesized an ultrastable FeCo bifunctional oxygen electrocatalyst on Se-doped CNTs (FeCo/Se-CNT) via a gravity guided chemical vapor deposition (CVD) strategy. The catalyst exhibits excellent ORR (E 1/2 = 0.9 V) and OER (overpotential at 10 mA cm–2 = 340 mV) properties simultaneously, surpassing commercial Pt/C and RuO2/C catalysts. More importantly, the catalyst shows an unordinary stability, that is, is no obvious decrease after 30K cycles accelerated durability test for ORR and OER processes. The small potential gap (0.75 V) represents superior bifunctional ORR and OER activities of the FeCo/Se-CNT catalyst. The FeCo/Se-CNT catalyst possesses outstanding electrochemical performance for the rechargeable liquid and flexible all-solid-state Zn–air batteries, for example, a high open circuit voltage (OCV) and peak power density of 1.543 and 1.405 V and 173.4 and 37.5 mW cm–2, respectively.
AbstractList The rechargeable Zn-air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge to develop non-noble metal bifunctional catalysts with high oxygen reduction as well as oxygen evolution reaction (ORR and OER) activity and superior durability, which limit the large-scale application of rechargeable Zn-air batteries. Herein, we synthesized an ultrastable FeCo bifunctional oxygen electrocatalyst on Se-doped CNTs (FeCo/Se-CNT) via a gravity guided chemical vapor deposition (CVD) strategy. The catalyst exhibits excellent ORR ( = 0.9 V) and OER (overpotential at 10 mA cm = 340 mV) properties simultaneously, surpassing commercial Pt/C and RuO /C catalysts. More importantly, the catalyst shows an unordinary stability, that is, is no obvious decrease after 30K cycles accelerated durability test for ORR and OER processes. The small potential gap (0.75 V) represents superior bifunctional ORR and OER activities of the FeCo/Se-CNT catalyst. The FeCo/Se-CNT catalyst possesses outstanding electrochemical performance for the rechargeable liquid and flexible all-solid-state Zn-air batteries, for example, a high open circuit voltage (OCV) and peak power density of 1.543 and 1.405 V and 173.4 and 37.5 mW cm , respectively.
The rechargeable Zn-air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge to develop non-noble metal bifunctional catalysts with high oxygen reduction as well as oxygen evolution reaction (ORR and OER) activity and superior durability, which limit the large-scale application of rechargeable Zn-air batteries. Herein, we synthesized an ultrastable FeCo bifunctional oxygen electrocatalyst on Se-doped CNTs (FeCo/Se-CNT) via a gravity guided chemical vapor deposition (CVD) strategy. The catalyst exhibits excellent ORR (E1/2 = 0.9 V) and OER (overpotential at 10 mA cm-2 = 340 mV) properties simultaneously, surpassing commercial Pt/C and RuO2/C catalysts. More importantly, the catalyst shows an unordinary stability, that is, is no obvious decrease after 30K cycles accelerated durability test for ORR and OER processes. The small potential gap (0.75 V) represents superior bifunctional ORR and OER activities of the FeCo/Se-CNT catalyst. The FeCo/Se-CNT catalyst possesses outstanding electrochemical performance for the rechargeable liquid and flexible all-solid-state Zn-air batteries, for example, a high open circuit voltage (OCV) and peak power density of 1.543 and 1.405 V and 173.4 and 37.5 mW cm-2, respectively.The rechargeable Zn-air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge to develop non-noble metal bifunctional catalysts with high oxygen reduction as well as oxygen evolution reaction (ORR and OER) activity and superior durability, which limit the large-scale application of rechargeable Zn-air batteries. Herein, we synthesized an ultrastable FeCo bifunctional oxygen electrocatalyst on Se-doped CNTs (FeCo/Se-CNT) via a gravity guided chemical vapor deposition (CVD) strategy. The catalyst exhibits excellent ORR (E1/2 = 0.9 V) and OER (overpotential at 10 mA cm-2 = 340 mV) properties simultaneously, surpassing commercial Pt/C and RuO2/C catalysts. More importantly, the catalyst shows an unordinary stability, that is, is no obvious decrease after 30K cycles accelerated durability test for ORR and OER processes. The small potential gap (0.75 V) represents superior bifunctional ORR and OER activities of the FeCo/Se-CNT catalyst. The FeCo/Se-CNT catalyst possesses outstanding electrochemical performance for the rechargeable liquid and flexible all-solid-state Zn-air batteries, for example, a high open circuit voltage (OCV) and peak power density of 1.543 and 1.405 V and 173.4 and 37.5 mW cm-2, respectively.
The rechargeable Zn–air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge to develop non-noble metal bifunctional catalysts with high oxygen reduction as well as oxygen evolution reaction (ORR and OER) activity and superior durability, which limit the large-scale application of rechargeable Zn–air batteries. Herein, we synthesized an ultrastable FeCo bifunctional oxygen electrocatalyst on Se-doped CNTs (FeCo/Se-CNT) via a gravity guided chemical vapor deposition (CVD) strategy. The catalyst exhibits excellent ORR (E 1/2 = 0.9 V) and OER (overpotential at 10 mA cm–2 = 340 mV) properties simultaneously, surpassing commercial Pt/C and RuO2/C catalysts. More importantly, the catalyst shows an unordinary stability, that is, is no obvious decrease after 30K cycles accelerated durability test for ORR and OER processes. The small potential gap (0.75 V) represents superior bifunctional ORR and OER activities of the FeCo/Se-CNT catalyst. The FeCo/Se-CNT catalyst possesses outstanding electrochemical performance for the rechargeable liquid and flexible all-solid-state Zn–air batteries, for example, a high open circuit voltage (OCV) and peak power density of 1.543 and 1.405 V and 173.4 and 37.5 mW cm–2, respectively.
Author Shi, Shuangrui
Zheng, Lirong
Shang, Jingzhi
Zhang, Biao
Ma, Chao
Song, Lin
Han, Yunhu
Huang, Wei
Wang, Zhenhua
Liu, Haoran
Zhang, Hongwei
Zhao, Meiqi
Yang, Yong
AuthorAffiliation State Key Laboratory of Structural Chemistry
Department of Chemistry
School of Materials Science and Engineering
Key Laboratory for Organic Electronics and Information Displays and Institute of Advanced Materials (IAM)
Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences
Beijing Synchrotron Radiation Facility, Institute of High Energy Physics
Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering
Nanjing University of Posts and Telecommunications
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– name: Department of Chemistry
– name: Nanjing University of Posts and Telecommunications
– name: Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences
– name: Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering
– name: School of Materials Science and Engineering
– name: State Key Laboratory of Structural Chemistry
– name: Beijing Synchrotron Radiation Facility, Institute of High Energy Physics
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  orcidid: 0000-0002-9028-6799
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– sequence: 6
  givenname: Biao
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– sequence: 7
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  orcidid: 0000-0003-4971-6301
  surname: Song
  fullname: Song, Lin
  organization: Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering
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  givenname: Jingzhi
  surname: Shang
  fullname: Shang, Jingzhi
  organization: Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering
– sequence: 9
  givenname: Yong
  orcidid: 0000-0002-1238-2945
  surname: Yang
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  orcidid: 0000-0003-0354-4479
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  orcidid: 0000-0001-7004-6408
  surname: Huang
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  email: iamwhuang@nwpu.edu.cn
  organization: Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering
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Issue 5
Keywords Se-doped CNTs
liquid and flexible solid rechargeable Zn−air batteries
bifunctional oxygen electrocatalyst
outstanding durability
gravity guided CVD strategy
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Snippet The rechargeable Zn–air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge...
The rechargeable Zn-air batteries as an environmentally friendly sustainable energy technology have been extensively studied. However, it is still a challenge...
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Title Ultrastable FeCo Bifunctional Electrocatalyst on Se-Doped CNTs for Liquid and Flexible All-Solid-State Rechargeable Zn–Air Batteries
URI http://dx.doi.org/10.1021/acs.nanolett.1c00077
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