High Charge Mobility in a Tetrathiafulvalene-Based Microporous Metal–Organic Framework
The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal–organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge m...
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| Published in | Journal of the American Chemical Society Vol. 134; no. 31; pp. 12932 - 12935 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
WASHINGTON
American Chemical Society
08.08.2012
Amer Chemical Soc |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal–organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge mobility commensurate with some of the best organic semiconductors, confirmed by flash-photolysis-time-resolved microwave conductivity measurements. Zn2(TTFTB) represents the first example of a permanently porous MOF with high charge mobility and may inspire further exploration of the electronic properties of these materials. |
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| AbstractList | The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal–organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge mobility commensurate with some of the best organic semiconductors, confirmed by flash-photolysis-time-resolved microwave conductivity measurements. Zn2(TTFTB) represents the first example of a permanently porous MOF with high charge mobility and may inspire further exploration of the electronic properties of these materials. The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal-organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge mobility commensurate with some of the best organic semiconductors, confirmed by flash-photolysis-time-resolved microwave conductivity measurements. Zn2(TTFTB) represents the first example of a permanently porous MOF with high charge mobility and may inspire further exploration of the electronic properties of these materials.The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal-organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge mobility commensurate with some of the best organic semiconductors, confirmed by flash-photolysis-time-resolved microwave conductivity measurements. Zn2(TTFTB) represents the first example of a permanently porous MOF with high charge mobility and may inspire further exploration of the electronic properties of these materials. The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H₄TTFTB) is used to synthesize Zn₂(TTFTB), a new metal–organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge mobility commensurate with some of the best organic semiconductors, confirmed by flash-photolysis-time-resolved microwave conductivity measurements. Zn₂(TTFTB) represents the first example of a permanently porous MOF with high charge mobility and may inspire further exploration of the electronic properties of these materials. The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn-2(TTFTB), a new metal-organic framework that contains columnar stacks of tetrathiafulvalene and benzoate-lined infinite one-dimensional channels. The new MOF remains porous upon desolvation and exhibits charge mobility commensurate with some of the best organic semiconductors, confirmed by flash-photolysis-time-resolved microwave conductivity measurements. Zn-2(TTFTB) represents the first example of a permanently porous MOF with high charge mobility and may inspire further exploration of the electronic properties of these materials. |
| Author | Narayan, Tarun C Dincă, Mircea Miyakai, Tomoyo Seki, Shu |
| AuthorAffiliation | Massachusetts Institute of Technology Osaka University |
| AuthorAffiliation_xml | – name: Osaka University – name: Massachusetts Institute of Technology |
| Author_xml | – sequence: 1 givenname: Tarun C surname: Narayan fullname: Narayan, Tarun C – sequence: 2 givenname: Tomoyo surname: Miyakai fullname: Miyakai, Tomoyo – sequence: 3 givenname: Shu surname: Seki fullname: Seki, Shu – sequence: 4 givenname: Mircea surname: Dincă fullname: Dincă, Mircea email: mdinca@mit.edu |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22827709$$D View this record in MEDLINE/PubMed |
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| Snippet | The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal–organic framework that contains columnar stacks... The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn-2(TTFTB), a new metal-organic framework that contains columnar stacks... The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H4TTFTB) is used to synthesize Zn2(TTFTB), a new metal-organic framework that contains columnar stacks... The tetratopic ligand tetrathiafulvalene-tetrabenzoate (H₄TTFTB) is used to synthesize Zn₂(TTFTB), a new metal–organic framework that contains columnar stacks... |
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| SubjectTerms | Chemistry Chemistry, Multidisciplinary ligands Physical Sciences porous media Science & Technology semiconductors |
| Title | High Charge Mobility in a Tetrathiafulvalene-Based Microporous Metal–Organic Framework |
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