Bright Fluorescence from Individual Single-Walled Carbon Nanotubes

Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the fluorescence efficiency of individual DNA-wrapped SWNTs upon addition of reducing agents, including dithiothreitol, Trolox, and β-mercaptoethanol. B...

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Published inNano letters Vol. 11; no. 4; pp. 1636 - 1640
Main Authors Lee, Andrea J, Wang, Xiaoyong, Carlson, Lisa J, Smyder, Julie A, Loesch, Bradford, Tu, Xiaomin, Zheng, Ming, Krauss, Todd D
Format Journal Article
LanguageEnglish
Published Washington, DC American Chemical Society 13.04.2011
Subjects
Cross-disciplinary physics: materials science; rheology
Equipment Design
Equipment Failure Analysis
Exact sciences and technology
Fluorescence
Lighting - instrumentation
Luminescent Measurements - instrumentation
Materials science
Nanoscale materials and structures: fabrication and characterization
Nanotubes
Nanotubes, Carbon - chemistry
Nanotubes, Carbon - ultrastructure
Particle Size
Physics
near-infrared fluorescence
fluorescence
Single-walled carbon nanotubes
epifluorescence microscopy
Fluorescence
Singlewalled nanotube
Photoelectronic properties
Nanocomposites
Carbon
Transients
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Abstract Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the fluorescence efficiency of individual DNA-wrapped SWNTs upon addition of reducing agents, including dithiothreitol, Trolox, and β-mercaptoethanol. Brightening was reversible upon removal of the reducing molecules, suggesting that a transient reduction of defect sites on the SWNT sidewall causes the effect. These results imply that SWNTs are intrinsically bright emitters and that their poor emission arises from defective nanotubes.
AbstractList Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the fluorescence efficiency of individual DNA-wrapped SWNTs upon addition of reducing agents, including dithiothreitol, Trolox, and β-mercaptoethanol. Brightening was reversible upon removal of the reducing molecules, suggesting that a transient reduction of defect sites on the SWNT sidewall causes the effect. These results imply that SWNTs are intrinsically bright emitters and that their poor emission arises from defective nanotubes.
Author Zheng, Ming
Carlson, Lisa J
Lee, Andrea J
Loesch, Bradford
Smyder, Julie A
Wang, Xiaoyong
Tu, Xiaomin
Krauss, Todd D
AuthorAffiliation University of Rochester
DuPont Central Research and Development
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  surname: Lee
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Keywords near-infrared fluorescence
fluorescence
Single-walled carbon nanotubes
epifluorescence microscopy
Fluorescence
Singlewalled nanotube
Photoelectronic properties
Nanocomposites
Carbon
Transients
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Snippet Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the...
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StartPage 1636
SubjectTerms Cross-disciplinary physics: materials science; rheology
Equipment Design
Equipment Failure Analysis
Exact sciences and technology
Fluorescence
Lighting - instrumentation
Luminescent Measurements - instrumentation
Materials science
Nanoscale materials and structures: fabrication and characterization
Nanotubes
Nanotubes, Carbon - chemistry
Nanotubes, Carbon - ultrastructure
Particle Size
Physics
Title Bright Fluorescence from Individual Single-Walled Carbon Nanotubes
URI http://dx.doi.org/10.1021/nl200077t
https://www.ncbi.nlm.nih.gov/pubmed/21417364
https://search.proquest.com/docview/862008012
Volume 11
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