Bright Fluorescence from Individual Single-Walled Carbon Nanotubes
Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the fluorescence efficiency of individual DNA-wrapped SWNTs upon addition of reducing agents, including dithiothreitol, Trolox, and β-mercaptoethanol. B...
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Published in | Nano letters Vol. 11; no. 4; pp. 1636 - 1640 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
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Washington, DC
American Chemical Society
13.04.2011
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Abstract | Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the fluorescence efficiency of individual DNA-wrapped SWNTs upon addition of reducing agents, including dithiothreitol, Trolox, and β-mercaptoethanol. Brightening was reversible upon removal of the reducing molecules, suggesting that a transient reduction of defect sites on the SWNT sidewall causes the effect. These results imply that SWNTs are intrinsically bright emitters and that their poor emission arises from defective nanotubes. |
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AbstractList | Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the fluorescence efficiency of individual DNA-wrapped SWNTs upon addition of reducing agents, including dithiothreitol, Trolox, and β-mercaptoethanol. Brightening was reversible upon removal of the reducing molecules, suggesting that a transient reduction of defect sites on the SWNT sidewall causes the effect. These results imply that SWNTs are intrinsically bright emitters and that their poor emission arises from defective nanotubes. |
Author | Zheng, Ming Carlson, Lisa J Lee, Andrea J Loesch, Bradford Smyder, Julie A Wang, Xiaoyong Tu, Xiaomin Krauss, Todd D |
AuthorAffiliation | University of Rochester DuPont Central Research and Development |
AuthorAffiliation_xml | – name: University of Rochester – name: DuPont Central Research and Development |
Author_xml | – sequence: 1 givenname: Andrea J surname: Lee fullname: Lee, Andrea J – sequence: 2 givenname: Xiaoyong surname: Wang fullname: Wang, Xiaoyong – sequence: 3 givenname: Lisa J surname: Carlson fullname: Carlson, Lisa J – sequence: 4 givenname: Julie A surname: Smyder fullname: Smyder, Julie A – sequence: 5 givenname: Bradford surname: Loesch fullname: Loesch, Bradford – sequence: 6 givenname: Xiaomin surname: Tu fullname: Tu, Xiaomin – sequence: 7 givenname: Ming surname: Zheng fullname: Zheng, Ming – sequence: 8 givenname: Todd D surname: Krauss fullname: Krauss, Todd D email: krauss@chem.rochester.edu |
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Keywords | near-infrared fluorescence fluorescence Single-walled carbon nanotubes epifluorescence microscopy Fluorescence Singlewalled nanotube Photoelectronic properties Nanocomposites Carbon Transients |
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Snippet | Single-walled carbon nanotubes (SWNTs) have unique photophysical properties but low fluorescence efficiency. We have found significant increases in the... |
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SubjectTerms | Cross-disciplinary physics: materials science; rheology Equipment Design Equipment Failure Analysis Exact sciences and technology Fluorescence Lighting - instrumentation Luminescent Measurements - instrumentation Materials science Nanoscale materials and structures: fabrication and characterization Nanotubes Nanotubes, Carbon - chemistry Nanotubes, Carbon - ultrastructure Particle Size Physics |
Title | Bright Fluorescence from Individual Single-Walled Carbon Nanotubes |
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