Simple Solvent Treatment Enabled Improved PEDOT:PSS Performance toward Highly Efficient Binary Organic Solar Cells

PEDOT:PSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great importance for realizing high power conversion efficiency (PCE). However, its performance in OSC devices has been continuously challenged by vari...

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Published inACS omega Vol. 7; no. 45; pp. 41789 - 41795
Main Authors Shi, Shasha, Hou, Yiwen, Yang, Tao, Huang, Ciyuan, Yao, Shangfei, Zhao, Chenfu, Liu, Yudie, Zhang, Ziyang, Liu, Tao, Zou, Bingsuo
Format Journal Article
LanguageEnglish
Published American Chemical Society 15.11.2022
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Abstract PEDOT:PSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great importance for realizing high power conversion efficiency (PCE). However, its performance in OSC devices has been continuously challenged by various replacing materials and different doping strategies, for better conductivity, work function, and surface property. Here, we report a simple dopant-free method to tune the phase separation of the PEDOT:PSS layer, which results in better charge transport and extraction in devices. Specifically, high PCEs for binary polymer-small-molecule (>18%) and polymer–polymer (>17%) systems are simultaneously achieved. This work engineeringly provides encouraging improvement for OSC device performance with easy modification and scientifically offers insights into tuning the property of the PEDOT:PSS layer.
AbstractList PEDOTPSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great importance for realizing high power conversion efficiency (PCE). However, its performance in OSC devices has been continuously challenged by various replacing materials and different doping strategies, for better conductivity, work function, and surface property. Here, we report a simple dopant-free method to tune the phase separation of the PEDOT:PSS layer, which results in better charge transport and extraction in devices. Specifically, high PCEs for binary polymer-small-molecule (>18%) and polymer-polymer (>17%) systems are simultaneously achieved. This work engineeringly provides encouraging improvement for OSC device performance with easy modification and scientifically offers insights into tuning the property of the PEDOT:PSS layer.
PEDOT:PSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great importance for realizing high power conversion efficiency (PCE). However, its performance in OSC devices has been continuously challenged by various replacing materials and different doping strategies, for better conductivity, work function, and surface property. Here, we report a simple dopant-free method to tune the phase separation of the PEDOT:PSS layer, which results in better charge transport and extraction in devices. Specifically, high PCEs for binary polymer-small-molecule (>18%) and polymer–polymer (>17%) systems are simultaneously achieved. This work engineeringly provides encouraging improvement for OSC device performance with easy modification and scientifically offers insights into tuning the property of the PEDOT:PSS layer.
PEDOT:PSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great importance for realizing high power conversion efficiency (PCE). However, its performance in OSC devices has been continuously challenged by various replacing materials and different doping strategies, for better conductivity, work function, and surface property. Here, we report a simple dopant-free method to tune the phase separation of the PEDOT:PSS layer, which results in better charge transport and extraction in devices. Specifically, high PCEs for binary polymer-small-molecule (>18%) and polymer–polymer (>17%) systems are simultaneously achieved. This work engineeringly provides encouraging improvement for OSC device performance with easy modification and scientifically offers insights into tuning the property of the PEDOT:PSS layer.
Author Yao, Shangfei
Yang, Tao
Zou, Bingsuo
Zhao, Chenfu
Huang, Ciyuan
Zhang, Ziyang
Shi, Shasha
Liu, Yudie
Hou, Yiwen
Liu, Tao
AuthorAffiliation Julong College
Guangxi Key Lab of Processing for Nonferrous Metals and Featured Materials and Key Lab of New Processing Technology for Nonferrous Metals and Materials, Ministry of Education; School of Resources, Environments and Materials
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Snippet PEDOT:PSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great...
PEDOTPSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great...
PEDOT:PSS is the most popular hole-transporting material (HTM) for conventional structural organic solar cell (OSC) devices, whose performance is of great...
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Title Simple Solvent Treatment Enabled Improved PEDOT:PSS Performance toward Highly Efficient Binary Organic Solar Cells
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