Retention Effects of Soil Humic Substances on the Diffusive Transportation of Metal Ions During Sediment Porewater Membrane Dialysis Sampling
In situ sampling techniques such as membrane dialysis are widely applied to the monitoring of heavy metal contamination in water-saturated environments. In this study, batch experiments were conducted to investigate the influence of humic substances (HS) on the diffusive transportation of metal ions...
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Published in | Water, air, and soil pollution Vol. 224; no. 6; p. 1 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
Published |
Dordrecht
Springer Netherlands
01.06.2013
Springer Springer Nature B.V |
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Abstract | In situ sampling techniques such as membrane dialysis are widely applied to the monitoring of heavy metal contamination in water-saturated environments. In this study, batch experiments were conducted to investigate the influence of humic substances (HS) on the diffusive transportation of metal ions across sampling membranes. The presence of HS substantially slowed the transportation of metal ions by 22.2, 20.3, 17.4, 16.6, and 14.9 % for Zn
2+
, Cu
2+
, Ni
2+
, Co
2+
, and Mn
2+
, respectively, in the 100-mg/L HS-amended treatments relative to the treatments without HS under acidic conditions (pH = 5.0). The retention effect of HS on the metal ions appeared to be relieved at a higher pH of 8.5. However, HS also slowed the transportation of metal ions (Cu
2+
, Zn
2+
, Ni
2+
and Co
2+
) into the sampling cells when membranes soaked previously in porewater solution. The retention effects of HS can be attributed to the enhanced adsorption of metal ions on the surfaces of the membranes. Further study in saturated sediments verified that the membrane dialysis technique could underestimate the concentrations of metal ions by 13.3–40.2 % at the presences of HS. These findings suggest that collected porewater data using the membrane dialysis technique should be interpreted with caution with the consideration of in situ geochemical conditions such as HS or pH in water-saturated environments. |
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AbstractList | In situ sampling techniques such as membrane dialysis are widely applied to the monitoring of heavy metal contamination in water-saturated environments. In this study, batch experiments were conducted to investigate the influence of humic substances (HS) on the diffusive transportation of metal ions across sampling membranes. The presence of HS substantially slowed the transportation of metal ions by 22.2, 20.3, 17.4, 16.6, and 14.9 % for [Zn.sup.2+],[Cu.sup.2+], [Ni.sup.2+], [Co.sup.2+], and [Mn.sup.2+], respectively, in the 100-mg/L HS-amended treatments relative to the treatments without HS under acidic conditions (pH = 5.0). The retention effect of HS on the metal ions appeared to be relieved at a higher pH of 8.5. However, HS also slowed the transportation of metal ions ([Cu.sup.2+],[Zn.sup.2+], [Ni.sup.2+] and [Co.sup.2+]) into the sampling cells when membranes soaked previously in porewater solution. The retention effects of HS can be attributed to the enhanced adsorption of metal ions on the surfaces of the membranes. Further study in saturated sediments verified that the membrane dialysis technique could underestimate the concentrations of metal ions by 13.340.2 % at the presences of HS. These findings suggest that collected porewater data using the membrane dialysis technique should be interpreted with caution with the consideration of in situ geochemical conditions such as HS or pH in water-saturated environments. Keywords Membrane dialysis * Diffusive transportation * Heavy metals * Humic substances In situ sampling techniques such as membrane dialysis are widely applied to the monitoring of heavy metal contamination in water-saturated environments. In this study, batch experiments were conducted to investigate the influence of humic substances (HS) on the diffusive transportation of metal ions across sampling membranes. The presence of HS substantially slowed the transportation of metal ions by 22.2, 20.3, 17.4, 16.6, and 14.9 % for Zn^sup 2+^, Cu^sup 2+^, Ni^sup 2+^, Co^sup 2+^, and Mn^sup 2+^, respectively, in the 100-mg/L HS-amended treatments relative to the treatments without HS under acidic conditions (pH=5.0). The retention effect of HS on the metal ions appeared to be relieved at a higher pH of 8.5. However, HS also slowed the transportation of metal ions (Cu^sup 2+^, Zn^sup 2+^, Ni^sup 2+^ and Co^sup 2+^) into the sampling cells when membranes soaked previously in porewater solution. The retention effects of HS can be attributed to the enhanced adsorption of metal ions on the surfaces of the membranes. Further study in saturated sediments verified that the membrane dialysis technique could underestimate the concentrations of metal ions by 13.3-40.2 % at the presences of HS. These findings suggest that collected porewater data using the membrane dialysis technique should be interpreted with caution with the consideration of in situ geochemical conditions such as HS or pH in water-saturated environments.[PUBLICATION ABSTRACT] In situ sampling techniques such as membrane dialysis are widely applied to the monitoring of heavy metal contamination in water-saturated environments. In this study, batch experiments were conducted to investigate the influence of humic substances (HS) on the diffusive transportation of metal ions across sampling membranes. The presence of HS substantially slowed the transportation of metal ions by 22.2, 20.3, 17.4, 16.6, and 14.9 % for Zn 2+ , Cu 2+ , Ni 2+ , Co 2+ , and Mn 2+ , respectively, in the 100-mg/L HS-amended treatments relative to the treatments without HS under acidic conditions (pH = 5.0). The retention effect of HS on the metal ions appeared to be relieved at a higher pH of 8.5. However, HS also slowed the transportation of metal ions (Cu 2+ , Zn 2+ , Ni 2+ and Co 2+ ) into the sampling cells when membranes soaked previously in porewater solution. The retention effects of HS can be attributed to the enhanced adsorption of metal ions on the surfaces of the membranes. Further study in saturated sediments verified that the membrane dialysis technique could underestimate the concentrations of metal ions by 13.3–40.2 % at the presences of HS. These findings suggest that collected porewater data using the membrane dialysis technique should be interpreted with caution with the consideration of in situ geochemical conditions such as HS or pH in water-saturated environments. |
ArticleNumber | 1577 |
Audience | Academic |
Author | Hu, Chaohua Luo, Wensui Zhang, Youchi |
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Keywords | Membrane dialysis Diffusive transportation Humic substances Heavy metals Transportation Metal ion Sediments Organic acids Diffusivity Interstitial water Heavy metal Trace element Soils Pollution Membrane Dialysis Humic substance Diffusion coefficient Sampling |
Language | English |
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SubjectTerms | Adsorption Analysis Applied sciences Atmospheric Protection/Air Quality Control/Air Pollution Climate Change/Climate Change Impacts Contact angle Copper Dialysis Diffusion Earth and Environmental Science Environment Environmental monitoring Exact sciences and technology Experiments Fourier transforms Heavy metals Hemodialysis Humic acid Humic acids Hydrogeology Membrane filters Membranes Metal concentrations Metal ions Metals pH effects Pollution Pore water Retention Sampling Sampling techniques Sediments Sediments (Geology) Soil pollution Soil Science & Conservation Studies Thin films Water pollution Water Quality/Water Pollution Zinc compounds |
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Title | Retention Effects of Soil Humic Substances on the Diffusive Transportation of Metal Ions During Sediment Porewater Membrane Dialysis Sampling |
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