Carbon-Supported Pt-Based Alloy Electrocatalysts for the Oxygen Reduction Reaction in Polymer Electrolyte Membrane Fuel Cells: Particle Size, Shape, and Composition Manipulation and Their Impact to Activity

A scientific review addresses the current development of size-dependent, shape-selected, and composition-controlled carbon-supported Pt-alloy electrocatalysts for enhancing electrochemical catalytic performance in polymer electrolyte membrane fuel cells (PEMFCs). It starts with an overview of carbon...

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Bibliographic Details
Published in	Chemical reviews Vol. 115; no. 9; pp. 3433 - 3467
Main Authors	Wang, Yan-Jie, Zhao, Nana, Fang, Baizeng, Li, Hui, Bi, Xiaotao T, Wang, Haijiang
Format	Journal Article
Language	English
Published	United States American Chemical Society 13.05.2015
Subjects	Alloys Carbon Carbon support Carbon-supported Pt Catalyst activity Catalysts Catalytic performance Chemical reactions Electrocatalysts Electrolysis Electrolytes Electrolytic reduction Fuel cells Fuel technology Molecular biology Oxygen Oxygen reduction reaction Particle shape Particle size Platinum Platinum alloys Polyelectrolytes Polymer electrolyte membrane fuel cell (PEMFCs) Polymers Proton exchange membrane fuel cells (PEMFC) Solid electrolytes Theoretical study
Online Access	Get full text
ISSN	0009-2665 1520-6890 1520-6890
DOI	10.1021/cr500519c

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Abstract	A scientific review addresses the current development of size-dependent, shape-selected, and composition-controlled carbon-supported Pt-alloy electrocatalysts for enhancing electrochemical catalytic performance in polymer electrolyte membrane fuel cells (PEMFCs). It starts with an overview of carbon support in carbon-supported Pt-alloy electrocatalysts and proceeds to the theoretical studies on the impact of Pt-alloy particle size, shape, and composition, and the experimental research on the particle size, shape, and composition of Pt-alloy catalysts. It particularly emphasizes on strategies to control particle size, shape, composition, and their impacts on catalyst activity toward the oxygen reduction reaction. NRC publication: Yes
AbstractList	Wang et al examine carbon-supported Pt-based alloy electrocatalysts for the oxygen reduction reaction in polymer electrolyte membrane fuel cells. They focus on particle size, shape, and composition manipulation, as well as their impact to activity. They provide information on theoretical studies, experimental studies on the control of carbon-supported Pt-alloy particle size, experimental studies on the control of carbon-supported Pt-alloy particle shape, and experimental studies on the control of carbon-supported Pt-alloy composition. A scientific review addresses the current development of size-dependent, shape-selected, and composition-controlled carbon-supported Pt-alloy electrocatalysts for enhancing electrochemical catalytic performance in polymer electrolyte membrane fuel cells (PEMFCs). It starts with an overview of carbon support in carbon-supported Pt-alloy electrocatalysts and proceeds to the theoretical studies on the impact of Pt-alloy particle size, shape, and composition, and the experimental research on the particle size, shape, and composition of Pt-alloy catalysts. It particularly emphasizes on strategies to control particle size, shape, composition, and their impacts on catalyst activity toward the oxygen reduction reaction.
Author	Fang, Baizeng Li, Hui Wang, Haijiang Bi, Xiaotao T Wang, Yan-Jie Zhao, Nana
AuthorAffiliation	University of British Columbia National Research Council Canada Vancouver International Clean-Tech Research Institute Inc Department of Chemical and Biological Engineering Electrochemical Materials, Energy, Mining and Environment
AuthorAffiliation_xml	– name: Electrochemical Materials, Energy, Mining and Environment – name: University of British Columbia – name: National Research Council Canada – name: Vancouver International Clean-Tech Research Institute Inc – name: Department of Chemical and Biological Engineering
Author_xml	– sequence: 1 givenname: Yan-Jie surname: Wang fullname: Wang, Yan-Jie – sequence: 2 givenname: Nana surname: Zhao fullname: Zhao, Nana – sequence: 3 givenname: Baizeng surname: Fang fullname: Fang, Baizeng – sequence: 4 givenname: Hui surname: Li fullname: Li, Hui email: Hui.Li@nrc-cnrc.gc.ca – sequence: 5 givenname: Xiaotao T surname: Bi fullname: Bi, Xiaotao T email: xbi@chbe.ubc.ca – sequence: 6 givenname: Haijiang surname: Wang fullname: Wang, Haijiang email: Haijiang.Wang@nrc-cnrc.gc.ca
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/25871490$$D View this record in MEDLINE/PubMed
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Snippet	A scientific review addresses the current development of size-dependent, shape-selected, and composition-controlled carbon-supported Pt-alloy electrocatalysts... Wang et al examine carbon-supported Pt-based alloy electrocatalysts for the oxygen reduction reaction in polymer electrolyte membrane fuel cells. They focus on...
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SubjectTerms	Alloys Carbon Carbon support Carbon-supported Pt Catalyst activity Catalysts Catalytic performance Chemical reactions Electrocatalysts Electrolysis Electrolytes Electrolytic reduction Fuel cells Fuel technology Molecular biology Oxygen Oxygen reduction reaction Particle shape Particle size Platinum Platinum alloys Polyelectrolytes Polymer electrolyte membrane fuel cell (PEMFCs) Polymers Proton exchange membrane fuel cells (PEMFC) Solid electrolytes Theoretical study
Title	Carbon-Supported Pt-Based Alloy Electrocatalysts for the Oxygen Reduction Reaction in Polymer Electrolyte Membrane Fuel Cells: Particle Size, Shape, and Composition Manipulation and Their Impact to Activity
URI	http://dx.doi.org/10.1021/cr500519c https://nrc-publications.canada.ca/eng/view/object/?id=ae2f91b3-90e5-4e97-a317-644dd7668e12 https://www.ncbi.nlm.nih.gov/pubmed/25871490 https://www.proquest.com/docview/1706226132 https://www.proquest.com/docview/1680958042
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