Rapid Interchangeable Hydrogen, Hydride, and Proton Species at the Interface of Transition Metal Atom on Oxide Surface

• Published in: Journal of the American Chemical Society Vol. 143; no. 24; pp. 9105 - 9112
• Main Authors: Wu, Simson, Tseng, Kai-Yu, Kato, Ryuichi, Wu, Tai-Sing, Large, Alexander, Peng, Yung-Kang, Xiang, Weikai, Fang, Huihuang, Mo, Jiaying, Wilkinson, Ian, Soo, Yun-Liang, Held, Georg, Suenaga, Kazu, Li, Tong, Chen, Hsin-Yi Tiffany, Tsang, Shik Chi Edman
• Format: Journal Article
• Language: English
• Published: American Chemical Society 23.06.2021
• Subjects: hydrides; hydrogen; spectroscopy

Hydrogen spillover is the phenomenon where a hydrogen atom, generated from the dissociative chemisorption of dihydrogen on the surface of a metal species, migrates from the metal to the catalytic support. This phenomenon is regarded as a promising avenue for hydrogen storage, yet the atomic mechanis...