Characterizing the availability of metals in contaminated soils. I. The solid phase: sequential extraction and isotopic dilution
. The two approaches most commonly applied to characterizing the chemical form and ‘reactivity’ of metals in the soil solid phase are sequential extraction procedures (SEPs) and isotopic dilution (ID). The development and limitations of both approaches are described and their application to contamin...
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| Published in | Soil use and management Vol. 21; no. s2; pp. 450 - 458 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford, UK
Blackwell Publishing Ltd
01.12.2005
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0266-0032 1475-2743 |
| DOI | 10.1079/SUM2005348 |
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| Abstract | . The two approaches most commonly applied to characterizing the chemical form and ‘reactivity’ of metals in the soil solid phase are sequential extraction procedures (SEPs) and isotopic dilution (ID). The development and limitations of both approaches are described and their application to contaminated soils discussed. It may be argued that ID offers a better means of discriminating between ‘reactive’ and ‘inert’ forms of metal. However, the literature on SEPs is considerably larger, providing greater scope for comparative analysis of new data. Although ID methods are subject to operational constraints, the procedural dependency of SEPs is probably much greater. Thus greater effort has been expended to standardize and verify methodologies for SEPs. However, despite achieving a level of ‘political ratification’ at the procedural level, the use of SEPs within risk assessments for planning or development purposes is currently almost absent. The future for ID methods in this context may lie in site‐specific risk assessments that include improved methods for the prediction of metal solubility and bioavailability. |
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| AbstractList | The two approaches most commonly applied to characterizing the chemical form and ‘reactivity’ of metals in the soil solid phase are sequential extraction procedures (SEPs) and isotopic dilution (ID). The development and limitations of both approaches are described and their application to contaminated soils discussed. It may be argued that ID offers a better means of discriminating between ‘reactive’ and ‘inert’ forms of metal. However, the literature on SEPs is considerably larger, providing greater scope for comparative analysis of new data. Although ID methods are subject to operational constraints, the procedural dependency of SEPs is probably much greater. Thus greater effort has been expended to standardize and verify methodologies for SEPs. However, despite achieving a level of ‘political ratification’ at the procedural level, the use of SEPs within risk assessments for planning or development purposes is currently almost absent. The future for ID methods in this context may lie in site‐specific risk assessments that include improved methods for the prediction of metal solubility and bioavailability. . The two approaches most commonly applied to characterizing the chemical form and ‘reactivity’ of metals in the soil solid phase are sequential extraction procedures (SEPs) and isotopic dilution (ID). The development and limitations of both approaches are described and their application to contaminated soils discussed. It may be argued that ID offers a better means of discriminating between ‘reactive’ and ‘inert’ forms of metal. However, the literature on SEPs is considerably larger, providing greater scope for comparative analysis of new data. Although ID methods are subject to operational constraints, the procedural dependency of SEPs is probably much greater. Thus greater effort has been expended to standardize and verify methodologies for SEPs. However, despite achieving a level of ‘political ratification’ at the procedural level, the use of SEPs within risk assessments for planning or development purposes is currently almost absent. The future for ID methods in this context may lie in site‐specific risk assessments that include improved methods for the prediction of metal solubility and bioavailability. |
| Author | Thornton, I. Young, S.D. Maxted, A. Zhang, H. Tye, A.M. Thums, C. |
| Author_xml | – sequence: 1 givenname: S.D. surname: Young fullname: Young, S.D. email: scott.young@nottingham.ac.uk organization: School of Biosciences, University of Nottingham, Biology Building, University Park, Nottingham NG7 2RD, UK – sequence: 2 givenname: H. surname: Zhang fullname: Zhang, H. organization: Department of Environmental Science, IENS, Lancaster University, Lancaster LA1 4YQ, UK – sequence: 3 givenname: A.M. surname: Tye fullname: Tye, A.M. organization: British Geological Survey, Kinsley Durham Center, Keyworth, Nottingham NG12 5GG, UK – sequence: 4 givenname: A. surname: Maxted fullname: Maxted, A. organization: School of Biosciences, University of Nottingham, Biology Building, University Park, Nottingham NG7 2RD, UK – sequence: 5 givenname: C. surname: Thums fullname: Thums, C. organization: Environmental Geochemistry Research Group, Department of Environmental Science and Technology, Royal School of Mines, Prince Consort Road, London SW7 2BP, UK – sequence: 6 givenname: I. surname: Thornton fullname: Thornton, I. organization: Environmental Geochemistry Research Group, Department of Environmental Science and Technology, Royal School of Mines, Prince Consort Road, London SW7 2BP, UK |
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Inhibition of Pb redistribution by two complexing agents (crypt and NTA) during a sequential extraction of soil models. Analytica Chimica Acta 347, 313-323 Hamel SC Ellickson KM Lioy PJ 1999. The estimation of the bioaccessibility of heavy metals in soils using artificial biofluids by two novel methods: mass balance and soil recapture. The Science of the Total Environment 243/244, 273-283 Pandeya SB Singh AK Jha P 1998. Labile pool of cadmium in sludge-treated soils. Plant and Soil 203, 1-13 Onken BM Hossner LR 1996. Determination of arsenic species in soil solution under flooded conditions. Soil Sc 1987; 33 2000; 258 2000; 254 1998; 84 2001; 45 2001; 43 1957; 84 1995; 28 1998b; 17 2000; 96 1967; 18 1996; 60 1998; 209 1995; 124 1998; 203 1995; 120 1991; 105 2001; 442 1973; 37 1999; 243/244 2002; 76 1999; 25 1998 1997 1986; 18 1995 1999; 20 2000; 110 1996; 91 2001; B84 2001; 445 1987; 59 2004; 55 1997; 206 1997; 31 1978; 42 1997; 35 2000; 109 1999; 33 2001; 35 1999; 236 2001; 30 2001; 436 1996; 89 2002; 472 1990; 19 2000; 41 2004; 68 1999; 363 2002; 118 2000; 51 1996; 30 1999; 87 1972a; 10 1998; 40 1999; 401 2004; 76 2002; 49 1997; 347 1998a; 17 2001 2000 2002; 42 2002; 184 1997; 18 2001; 16 1998; 369 1999; 91 1996; 178 1996; 332 1998; 27 2002; 36 2000; 29 1986; 50 1978; 12 1993; 82 2002; 295 2000; 22 2000; 20 1998; 218 2002; 459 1999; 382 2005 1999; 63 2002 1979; 51 1972; 114 2001; 113 1972b; 10 2000; 146 2000; 34 2002; 21 2000; 31 1952; 4 2000; 263 1994b; 20 1998; 32 1998; 102 2001; 76 2003; 67 e_1_2_1_111_1 e_1_2_1_81_1 e_1_2_1_20_1 e_1_2_1_66_1 e_1_2_1_89_1 e_1_2_1_24_1 e_1_2_1_62_1 e_1_2_1_43_1 e_1_2_1_85_1 e_1_2_1_28_1 e_1_2_1_47_1 e_1_2_1_92_1 e_1_2_1_103_1 Åsgeir A (e_1_2_1_4_1) 2001 Young SD (e_1_2_1_114_1) 2005 e_1_2_1_107_1 e_1_2_1_31_1 e_1_2_1_54_1 e_1_2_1_77_1 e_1_2_1_8_1 e_1_2_1_12_1 e_1_2_1_35_1 e_1_2_1_50_1 e_1_2_1_73_1 e_1_2_1_96_1 e_1_2_1_110_1 e_1_2_1_16_1 e_1_2_1_39_1 e_1_2_1_58_1 e_1_2_1_82_1 e_1_2_1_40_1 e_1_2_1_67_1 MAFF (Ministry of Agriculture, Fisheries and Food) (e_1_2_1_61_1) 1998 e_1_2_1_21_1 e_1_2_1_44_1 e_1_2_1_63_1 e_1_2_1_86_1 e_1_2_1_25_1 e_1_2_1_48_1 e_1_2_1_29_1 e_1_2_1_93_1 e_1_2_1_70_1 e_1_2_1_102_1 e_1_2_1_106_1 e_1_2_1_7_1 e_1_2_1_55_1 e_1_2_1_78_1 e_1_2_1_3_1 Tipping E (e_1_2_1_105_1) 2000 e_1_2_1_13_1 e_1_2_1_51_1 e_1_2_1_32_1 e_1_2_1_74_1 e_1_2_1_17_1 e_1_2_1_36_1 Young SD (e_1_2_1_113_1) 2001 e_1_2_1_59_1 e_1_2_1_60_1 e_1_2_1_41_1 e_1_2_1_87_1 e_1_2_1_68_1 e_1_2_1_45_1 e_1_2_1_83_1 e_1_2_1_22_1 e_1_2_1_64_1 e_1_2_1_26_1 e_1_2_1_109_1 e_1_2_1_101_1 e_1_2_1_71_1 e_1_2_1_90_1 e_1_2_1_56_1 e_1_2_1_79_1 e_1_2_1_98_1 e_1_2_1_6_1 e_1_2_1_10_1 e_1_2_1_33_1 e_1_2_1_52_1 e_1_2_1_75_1 e_1_2_1_94_1 e_1_2_1_2_1 Kersten M (e_1_2_1_49_1) 1995 e_1_2_1_14_1 e_1_2_1_37_1 e_1_2_1_18_1 Collins RMJ (e_1_2_1_15_1) 2001 e_1_2_1_80_1 e_1_2_1_112_1 e_1_2_1_42_1 e_1_2_1_65_1 Prohaska T (e_1_2_1_76_1) 1997 e_1_2_1_88_1 e_1_2_1_23_1 e_1_2_1_46_1 e_1_2_1_84_1 e_1_2_1_27_1 e_1_2_1_69_1 e_1_2_1_108_1 e_1_2_1_100_1 e_1_2_1_91_1 e_1_2_1_104_1 e_1_2_1_30_1 Sun B (e_1_2_1_97_1) 2000 e_1_2_1_5_1 e_1_2_1_57_1 e_1_2_1_99_1 e_1_2_1_72_1 e_1_2_1_11_1 Gérard E (e_1_2_1_34_1) 2001 e_1_2_1_53_1 e_1_2_1_95_1 e_1_2_1_38_1 e_1_2_1_9_1 e_1_2_1_19_1 |
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| Snippet | . The two approaches most commonly applied to characterizing the chemical form and ‘reactivity’ of metals in the soil solid phase are sequential extraction... The two approaches most commonly applied to characterizing the chemical form and ‘reactivity’ of metals in the soil solid phase are sequential extraction... The two approaches most commonly applied to characterizing the chemical form and `reactivity' of metals in the soil solid phase are sequential extraction... The two approaches most commonly applied to characterizing the chemical form and 'reactivity' of metals in the soil solid phase are sequential extraction... |
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| SubjectTerms | Contaminated soils isotopic dilution metal fractionation sequential extraction |
| Title | Characterizing the availability of metals in contaminated soils. I. The solid phase: sequential extraction and isotopic dilution |
| URI | https://api.istex.fr/ark:/67375/WNG-C1Q3BMFW-J/fulltext.pdf https://onlinelibrary.wiley.com/doi/abs/10.1079%2FSUM2005348 https://www.proquest.com/docview/20092071 https://www.proquest.com/docview/28913784 |
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