Nonionic Surfactant-Assisted In Situ Generation of Stable Passivation Protective Layer for Highly Stable Aqueous Zn Metal Anodes

A highly stable interface for aqueous rechargeable Zn batteries is of importance to inhibit the growth of Zn dendrites and suppress the side reactions. In this work, we have developed a stable honeycomb-like ZnO passivation protective layer on the Zn surface, which is in situ generated with the assi...

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Published inNano letters Vol. 22; no. 21; pp. 8574 - 8583
Main Authors Zhang, Yuanjun, Zheng, Xiaoyang, Wu, Kuan, Zhang, Ying, Xu, Gang, Wu, Minghong, Liu, Hua-Kun, Dou, Shi-Xue, Wu, Chao
Format Journal Article
LanguageEnglish
Published American Chemical Society 09.11.2022
Subjects
Aqueous Zn-ion battery
Protection layer
High areal capacity
Nonionic surfactant
Zn metal anodes
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Abstract A highly stable interface for aqueous rechargeable Zn batteries is of importance to inhibit the growth of Zn dendrites and suppress the side reactions. In this work, we have developed a stable honeycomb-like ZnO passivation protective layer on the Zn surface, which is in situ generated with the assistance of a nonionic surfactant additive (polyethylene glycol tert-octylphenyl ether, denoted as PEGTE). The ZnO passivation layer can facilitate the uniform distribution of the electric field, guiding the uniform deposition of Zn2+ and inhibit the generation of dendrites. As a result, the symmetric cell using the electrolyte with PEGTE shows an excellent performance at high areal capacity, reflected by stable cycling for over 2400 h at 5 mAh/cm2 and 1300 h at 10 mAh/cm2. The full cell paired with V2O5 demonstrates a long lifespan for more than 600 cycles at a low negative/positive capacity ratio.
AbstractList A highly stable interface for aqueous rechargeable Zn batteries is of importance to inhibit the growth of Zn dendrites and suppress the side reactions. In this work, we have developed a stable honeycomb-like ZnO passivation protective layer on the Zn surface, which is in situ generated with the assistance of a nonionic surfactant additive (polyethylene glycol tert-octylphenyl ether, denoted as PEGTE). The ZnO passivation layer can facilitate the uniform distribution of the electric field, guiding the uniform deposition of Zn2+ and inhibit the generation of dendrites. As a result, the symmetric cell using the electrolyte with PEGTE shows an excellent performance at high areal capacity, reflected by stable cycling for over 2400 h at 5 mAh/cm2 and 1300 h at 10 mAh/cm2. The full cell paired with V2O5 demonstrates a long lifespan for more than 600 cycles at a low negative/positive capacity ratio.A highly stable interface for aqueous rechargeable Zn batteries is of importance to inhibit the growth of Zn dendrites and suppress the side reactions. In this work, we have developed a stable honeycomb-like ZnO passivation protective layer on the Zn surface, which is in situ generated with the assistance of a nonionic surfactant additive (polyethylene glycol tert-octylphenyl ether, denoted as PEGTE). The ZnO passivation layer can facilitate the uniform distribution of the electric field, guiding the uniform deposition of Zn2+ and inhibit the generation of dendrites. As a result, the symmetric cell using the electrolyte with PEGTE shows an excellent performance at high areal capacity, reflected by stable cycling for over 2400 h at 5 mAh/cm2 and 1300 h at 10 mAh/cm2. The full cell paired with V2O5 demonstrates a long lifespan for more than 600 cycles at a low negative/positive capacity ratio.
A highly stable interface for aqueous rechargeable Zn batteries is of importance to inhibit the growth of Zn dendrites and suppress the side reactions. In this work, we have developed a stable honeycomb-like ZnO passivation protective layer on the Zn surface, which is in situ generated with the assistance of a nonionic surfactant additive (polyethylene glycol tert-octylphenyl ether, denoted as PEGTE). The ZnO passivation layer can facilitate the uniform distribution of the electric field, guiding the uniform deposition of Zn2+ and inhibit the generation of dendrites. As a result, the symmetric cell using the electrolyte with PEGTE shows an excellent performance at high areal capacity, reflected by stable cycling for over 2400 h at 5 mAh/cm2 and 1300 h at 10 mAh/cm2. The full cell paired with V2O5 demonstrates a long lifespan for more than 600 cycles at a low negative/positive capacity ratio.
Author Zheng, Xiaoyang
Wu, Kuan
Wu, Chao
Zhang, Yuanjun
Liu, Hua-Kun
Zhang, Ying
Wu, Minghong
Dou, Shi-Xue
Xu, Gang
AuthorAffiliation School of Intelligent Manufacturing
Huzhou College
Graduate School of Pure and Applied Sciences
School of Materials Science and Engineering
Institute of Energy Materials Science (IEMS)
Southwest University of Science and Technology
Institute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials
School of Environmental and Chemical Engineering
Key Laboratory of Organic Compound Pollution Control Engineering (MOE)
University of Shanghai for Science and Technology
AuthorAffiliation_xml – name: Key Laboratory of Organic Compound Pollution Control Engineering (MOE)
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  organization: Institute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials
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Keywords Aqueous Zn-ion battery
Protection layer
High areal capacity
Nonionic surfactant
Zn metal anodes
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Snippet A highly stable interface for aqueous rechargeable Zn batteries is of importance to inhibit the growth of Zn dendrites and suppress the side reactions. In this...
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Title Nonionic Surfactant-Assisted In Situ Generation of Stable Passivation Protective Layer for Highly Stable Aqueous Zn Metal Anodes
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