Selected element concentrations in alluvial sediments under garbage disposal site (Zagreb, Croatia)
Ag, Ba, Cd, Ce, Cs, Co, Cr, Cu, Eu, Fe, Ga, Mn, Ni, Pb, Rb, Sb, Sc, Sr, Th, Ti, V, Zn and Zr concentrations in alluvial sediments were determined by INAA and OES in the area used as a garbage disposal site in the vicinity of a water-well field. Results show that total concentrations of analysed elem...
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Published in | Water research (Oxford) Vol. 31; no. 6; pp. 1421 - 1429 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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Oxford
Elsevier Ltd
01.06.1997
Elsevier Science |
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Abstract | Ag, Ba, Cd, Ce, Cs, Co, Cr, Cu, Eu, Fe, Ga, Mn, Ni, Pb, Rb, Sb, Sc, Sr, Th, Ti, V, Zn and Zr concentrations in alluvial sediments were determined by INAA and OES in the area used as a garbage disposal site in the vicinity of a water-well field. Results show that total concentrations of analysed elements depend on sediment characteristics: mineral composition, specific surface area, cation exchange capacity, organic matter and clay-grain size fraction content. On the other hand, concentrations in sediment depend on physico-chemical forms and geochemical characteristics of the elements in question. Most of the elements reveal excellent/very good correlations with iron, while strontium shows negative correlation with iron. Strontium has a very good, positive correlation with carbonate content, while all other analysed elements, except silver, have excellent negative correlations with carbonates. Correlations with clay-grain size fraction are good or very good for all elements, except strontium and silver. The only element which is not correlated, either with iron, carbonate, or with clay-grain size fraction is silver. One can conclude, therefore, that silver is introduced as discrete particles. Extremely high silver concentration was found 6.5–6.8 m below the garbage in the aerated layer, occasionally under the water table. The enrichment factor for silver is found to be 127, which is a clear indication of sediment pollution with silver. Long-lasting clandestine deposition of industrial wastes on a disposal site meant for domestic wastes might be the reason. The elevated concentrations found on the 11.2–11.4 m depth are concordant with mineralogical composition (MnO-hydroxides, iron minerals, illite, chlorite) and enrichment factors for the majority of analysed elements are below 2. For the time being, this sediment layer acts as a chemical filter preventing infiltration in the vertical direction. Concentrations and enrichment factors of all determined elements from the uppermost and deeper water bearing layers are of natural values. Taking into account these, and additional, piezometer results, it can be concluded that the quality of water taken from the water-well field downstream of the garbage disposal site is not endangered so far. |
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AbstractList | Ag, Ba, Cd, Ce, Cs, Co, Cr, Cu, Eu, Fe, Ga, Mn, Ni, Pb, Rb, Sb, Sc, Sr, Th, Ti, V, Zn and Zr concentrations in alluvial sediments were determined by INAA and OES in the area used as a garbage disposal site in the vicinity of a water-well field. Results show that total concentrations of analysed elements depend on sediment characteristics: mineral composition, specific surface area, cation exchange capacity, organic matter and clay-grain size fraction content. On the other hand, concentrations in sediment depend on physico-chemical forms and geochemical characteristics of the elements in question. Most of the elements reveal excellent/very good correlations with iron, while strontium shows negative correlation with iron. Strontium has a very good, positive correlation with carbonate content, while all other analysed elements, except silver, have excellent negative correlations with carbonates. Correlations with clay-grain size fraction are good or very good for all elements, except strontium and silver. The only element which is not correlated, either with iron, carbonate, or with clay-grain size fraction is silver. One can conclude, therefore, that silver is introduced as discrete particles. Extremely high silver concentration was found 6.5-6.8 m below the garbage in the aerated layer, occasionally under the water table. The enrichment factor for silver is found to be 127, which is a clear indication of sediment pollution with silver. Long-lasting clandestine deposition of industrial wastes on a disposal site meant for domestic wastes might be the reason. The elevated concentrations found on the 11.2-11.4 m depth are concordant with mineralogical composition (MnO-hydroxides, iron minerals, illite, chlorite) and enrichment factors for the majority of analysed elements are below 2. For the time being, this sediment layer acts as a chemical filter preventing infiltration in the vertical direction. Concentrations and enrichment factors of all determined elements from the uppermost and deeper water bearing layers are of natural values. Taking into account these, and additional, piezometer results, it can be concluded that the quality of water taken from the water-well field downstream of the garbage disposal site is not endangered so far. |
Author | Juračić, M. Vertačnik, A. Prohić, E. Barišić, D. Lulić, S. |
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Cites_doi | 10.1007/BF02060365 10.1007/BF01664699 10.1016/0043-1354(90)90130-X 10.1007/BF02040385 10.1017/S0263593300005319 10.1016/0043-1354(94)E0114-L |
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Keywords | alluvial sediment garbage disposal site trace elements Ag enrichment factor INAA OES correlations illite trace metals oxides waste disposal cation exchange capacity heavy metals ground water pollution specific surface mineral assemblages enrichment aquifers human waste sheet silicates silicates alluvium Europe strontium chlorite carbonates chemical analysis industrial waste contamination oxihydroxides granulometry correlation organic materials clay minerals iron silver sediments |
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References | Vertačnik (BIB11) 1994 Čakarun, Mraz, Babić, Mutić, Sokač, Franić (BIB2) 1987; 40 Musani, Juračić, Konrad, Prohić, Vertačnik (BIB8) 1989 Foerstner (BIB3) 1985 Berrow, Mitchell (BIB1) 1991; 82 Vertačnik, Prohić, Kozar, Juračić (BIB12) 1995; 29 Musani, Kvastek (BIB7) 1986 Fuller, Davis, Cain, Lamothe, Fries, Fernandez, Vargas, Murillo (BIB4) 1990; 24 Golchert, Landsberger, Hopke (BIB5) 1991; 148 Li, Tong (BIB6) 1991; 147 Salomons, Foerstner (BIB10) 1984 Prohić, Juračić (BIB9) 1989; 13 Čakarun (10.1016/S0043-1354(96)00346-6_BIB2) 1987; 40 Foerstner (10.1016/S0043-1354(96)00346-6_BIB3) 1985 Salomons (10.1016/S0043-1354(96)00346-6_BIB10) 1984 Musani (10.1016/S0043-1354(96)00346-6_BIB8) 1989 Berrow (10.1016/S0043-1354(96)00346-6_BIB1) 1991; 82 Prohić (10.1016/S0043-1354(96)00346-6_BIB9) 1989; 13 Golchert (10.1016/S0043-1354(96)00346-6_BIB5) 1991; 148 Li (10.1016/S0043-1354(96)00346-6_BIB6) 1991; 147 Vertačnik (10.1016/S0043-1354(96)00346-6_BIB12) 1995; 29 Fuller (10.1016/S0043-1354(96)00346-6_BIB4) 1990; 24 Musani (10.1016/S0043-1354(96)00346-6_BIB7) 1986 Vertačnik (10.1016/S0043-1354(96)00346-6_BIB11) 1994 |
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Snippet | Ag, Ba, Cd, Ce, Cs, Co, Cr, Cu, Eu, Fe, Ga, Mn, Ni, Pb, Rb, Sb, Sc, Sr, Th, Ti, V, Zn and Zr concentrations in alluvial sediments were determined by INAA and... |
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SubjectTerms | alluvial sediment correlations Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics enrichment factor Exact sciences and technology garbage disposal site Geochemistry INAA OES Pollution, environment geology Soil and rock geochemistry trace elements |
Title | Selected element concentrations in alluvial sediments under garbage disposal site (Zagreb, Croatia) |
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