Re, Os and Ir in Antarctic unequilibrated ordinary chondrites and implications for the solar system abundance of Re
The concentrations of Re, Os and Ir in Antarctic unequilibrated ordinary chondrites (UOC) were determined by radiochemical neutron activation analysis. Large fractionations among these elements were found in Antarctic UOC. This is quite different from non‐Antarctic UOC and equilibrated ordinary chon...
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Published in | Geophysical research letters Vol. 22; no. 16; pp. 2167 - 2170 |
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Main Authors | , |
Format | Journal Article |
Language | English |
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Washington, DC
Blackwell Publishing Ltd
15.08.1995
American Geophysical Union |
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Abstract | The concentrations of Re, Os and Ir in Antarctic unequilibrated ordinary chondrites (UOC) were determined by radiochemical neutron activation analysis. Large fractionations among these elements were found in Antarctic UOC. This is quite different from non‐Antarctic UOC and equilibrated ordinary chondrites (EOC). Average Re/Os and Re/Ir ratios in ordinary chondrites are 25–30% higher than those in C1 chondrites and 10–15% higher than those in C2 and C3 chondrites. In contrast, the Os/Ir ratio is not variable among these chondrite groups. It is therefore suggested that Re is fractionated among ordinary and carbonaceous chondrites. Atom abundances of Os and Ir relative to 106 Si atoms of H chondrites are nearly equal to those of C1 chondrites, but their Re value is 30% higher than the C1 value. Considering that the currently accepted value for solar system abundance of Re (0.517 atom relative to 106 Si atoms) [Anders and Grevesse, 1989] is the lowest value among (Sinormalized) Re abundances in C1, C2, C3 and H chondrites, its value should be changed to a larger value. If C2 chondrites are adopted as the solar system standard, the solar system abundance of Re is changed to 0.0589, with those of Os and Ir being 0.740 and 0.685, respectively, at the same time. |
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AbstractList | The concentrations of Re, Os and Ir in Antarctic unequilibrated ordinary chondrites (UOC) were determined by radiochemical neutron activation analysis. Large fractionations among these elements were found in Antarctic UOC. This is quite different from non-Antarctic UOC and equilibrated ordinary chondrites (EOC). Average Re/Os and Re/Ir ratios in ordinary chondrites are 25-30% higher than those in C1 chondrites and 10-15% higher than those in C2 and C3 chondrites. In contrast, the Os/Ir ratio is not variable among these chondrite groups. It is therefore suggested that Re is fractionated among ordinary and carbonaceous chondrites. Atom abundances of Os and Ir relative to 10 super(6) Si atoms of H chondrites are nearly equal to those of C1 chondrites, but their Re value is 30% higher than the C1 value. Considering that the currently accepted value for solar system abundance of Re (0.517 atom relative to 10 super(6) Si atoms) [Anders and Grevesse, 1989] is the lowest value among (Sinormalized) Re abundances in C1, C2, C3 and H chondrites, its value should be changed to a larger value. If C2 chondrites are adopted as the solar system standard, the solar system abundance of Re is changed to 0.0589, with those of Os and Ir being 0.740 and 0.685, respectively, at the same time. The concentrations of Re, Os and Ir in Antarctic unequilibrated ordinary chondrites (UOC) were determined by radiochemical neutron activation analysis. Large fractionations among these elements were found in Antarctic UOC. This is quite different from non‐Antarctic UOC and equilibrated ordinary chondrites (EOC). Average Re/Os and Re/Ir ratios in ordinary chondrites are 25–30% higher than those in C1 chondrites and 10–15% higher than those in C2 and C3 chondrites. In contrast, the Os/Ir ratio is not variable among these chondrite groups. It is therefore suggested that Re is fractionated among ordinary and carbonaceous chondrites. Atom abundances of Os and Ir relative to 10 6 Si atoms of H chondrites are nearly equal to those of C1 chondrites, but their Re value is 30% higher than the C1 value. Considering that the currently accepted value for solar system abundance of Re (0.517 atom relative to 10 6 Si atoms) [ Anders and Grevesse, 1989] is the lowest value among (Sinormalized) Re abundances in C1, C2, C3 and H chondrites, its value should be changed to a larger value. If C2 chondrites are adopted as the solar system standard, the solar system abundance of Re is changed to 0.0589, with those of Os and Ir being 0.740 and 0.685, respectively, at the same time. The concentrations of Re, Os and Ir in Antarctic unequilibrated ordinary chondrites (UOC) were determined by radiochemical neutron activation analysis. Large fractionations among these elements were found in Antarctic UOC. This is quite different from non‐Antarctic UOC and equilibrated ordinary chondrites (EOC). Average Re/Os and Re/Ir ratios in ordinary chondrites are 25–30% higher than those in C1 chondrites and 10–15% higher than those in C2 and C3 chondrites. In contrast, the Os/Ir ratio is not variable among these chondrite groups. It is therefore suggested that Re is fractionated among ordinary and carbonaceous chondrites. Atom abundances of Os and Ir relative to 106 Si atoms of H chondrites are nearly equal to those of C1 chondrites, but their Re value is 30% higher than the C1 value. Considering that the currently accepted value for solar system abundance of Re (0.517 atom relative to 106 Si atoms) [Anders and Grevesse, 1989] is the lowest value among (Sinormalized) Re abundances in C1, C2, C3 and H chondrites, its value should be changed to a larger value. If C2 chondrites are adopted as the solar system standard, the solar system abundance of Re is changed to 0.0589, with those of Os and Ir being 0.740 and 0.685, respectively, at the same time. |
Author | Ozaki, Hiromasa Ebihara, Mitsuru |
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Cites_doi | 10.1029/RG012i001p00071 10.1016/0016-7037(82)90123-5 10.1016/0016-7037(89)90286-X 10.1016/0016-7037(78)90220-X 10.1016/0016-7037(67)90130-5 10.1111/j.1945-5100.1994.tb00661.x 10.1016/0016-7037(82)90208-3 10.1007/BF02042947 10.1016/0016-7037(83)90048-0 |
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Keywords | meteorites rhenium neutron activation analysis solar system abundance osmium chemical fractionation H chondrites iridium Yamato Meteorites carbonaceous chondrites Allan Hills Meteorites Allende Meteorite |
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References_xml | – volume: 42 start-page: 97 year: 1978 end-page: 106 article-title: Further studies of trace elements in C3 chondrites publication-title: Geochim. Cosmochim. Acta – volume: 185 start-page: 3 year: 1994 end-page: 13 article-title: Simultaneous determination of rhenium, osmium and iridium in meteoritic samples by neutron activation analysis using simple and effective radiochemical procedures publication-title: J. Radioanal. Nucl. Chem. – volume: 10 start-page: 997 year: 1979 end-page: 1010 article-title: Interelement refractory siderophile fractionation in ordinary chondrites publication-title: Proc. Lunar Sci. Conf. – year: 1988 – volume: 47 start-page: 2257 year: 1983 end-page: 2270 article-title: Aubrites and diogenites: Trace element clues to their origin publication-title: Geochim. Cosmochim. Acta – year: 1987 – volume: 29 start-page: 100 year: 1994 end-page: 143 article-title: The meteoritical bulletin, No. 76, 1994 January: The U. S. Antarctic meteorite collection publication-title: Meteoritics – volume: 31 start-page: 1893 year: 1967 end-page: 1909 article-title: Rhenium and osmium abundances in chondritic meteorites publication-title: Geochim. Cosmochim. Acta – volume: 46 start-page: 2363 year: 1982 end-page: 2380 article-title: Solar system abundances of the elements publication-title: Geochim. Cosmochim. Acta – volume: 12 start-page: 71 year: 1974 end-page: 101 article-title: Early chemical history of the solar system publication-title: Rev. Geophys. Space Phys. – volume: 53 start-page: 197 year: 1989 end-page: 214 article-title: Abundances of the elements: Meteoritic and solar publication-title: Geochim. Cosmochim. Acta – start-page: 196 year: 1993 end-page: 221 – volume: 46 start-page: 1849 year: 1982 end-page: 1861 article-title: Are Cl chondrites chemically fractionated? A trace element study publication-title: Geochim. Cosmochim. Acta – start-page: 161 year: 1992 end-page: 169 – volume: 27 start-page: 30 year: 1987 article-title: Neutron activation analysis of some trace elements in the Allende meteorite reference sample publication-title: Smithson. Contrib. Earth Sci. – volume-title: Radiochemical neutron activation analysis for 36 elements in geological materials: Au, Ag, Bi, Br, Cd, Cs, Ge, In, Ir, Ni, Os, Pd, Rb, Re, Sb, Se, Te, Tl, U, and Zn as well as Sc, Y, and REE year: 1988 ident: e_1_2_1_4_1 contributor: fullname: Anders E. – ident: e_1_2_1_8_1 doi: 10.1029/RG012i001p00071 – start-page: 161 volume-title: Unstable Nuclei in Astrophysics year: 1992 ident: e_1_2_1_5_1 contributor: fullname: Ebihara M. – start-page: 196 volume-title: Landolt‐Börnstein Group VI: Astronomy and Astrophysics year: 1993 ident: e_1_2_1_12_1 contributor: fullname: Palme H. – ident: e_1_2_1_6_1 doi: 10.1016/0016-7037(82)90123-5 – ident: e_1_2_1_3_1 doi: 10.1016/0016-7037(89)90286-X – volume-title: Photographic catalog of the Antarctic meteorites year: 1987 ident: e_1_2_1_16_1 contributor: fullname: Yanai K. – volume: 27 start-page: 30 year: 1987 ident: e_1_2_1_9_1 article-title: Neutron activation analysis of some trace elements in the Allende meteorite reference sample publication-title: Smithson. Contrib. Earth Sci. contributor: fullname: Lovering J. F. – ident: e_1_2_1_14_1 doi: 10.1016/0016-7037(78)90220-X – ident: e_1_2_1_10_1 doi: 10.1016/0016-7037(67)90130-5 – volume: 10 start-page: 997 year: 1979 ident: e_1_2_1_13_1 article-title: Interelement refractory siderophile fractionation in ordinary chondrites publication-title: Proc. Lunar Sci. Conf. contributor: fullname: Rambaldi E. R. – ident: e_1_2_1_7_1 doi: 10.1111/j.1945-5100.1994.tb00661.x – ident: e_1_2_1_2_1 doi: 10.1016/0016-7037(82)90208-3 – ident: e_1_2_1_11_1 doi: 10.1007/BF02042947 – ident: e_1_2_1_15_1 doi: 10.1016/0016-7037(83)90048-0 |
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SubjectTerms | Abundance Antarctica Carbonaceous chondrites Chondrites Cosmochemistry. Extraterrestrial geology Distillation Earth sciences Earth, ocean, space Exact sciences and technology Iridium Meteorites. Tectites. Impactites Silicon Solar system |
Title | Re, Os and Ir in Antarctic unequilibrated ordinary chondrites and implications for the solar system abundance of Re |
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