The geochemical behavior and isotopic composition of Hg in a mid-Pleistocene western Mediterranean sapropel

The concentrations of mercury (Hg) and other trace metals (Ni, Cu, Zn, Mo, Ba, Re, U) and the Hg isotopic composition were examined across a dramatic redox and productivity transition in a mid-Pleistocene Mediterranean Sea sapropel sequence. Characteristic trace metal enrichment in organic-rich laye...

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Published inGeochimica et cosmochimica acta Vol. 73; no. 6; pp. 1651 - 1665
Main Authors Gehrke, Gretchen E., Blum, Joel D., Meyers, Philip A.
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 15.03.2009
Subjects
Concentration (composition)
Enrichment
Marine
Mediterranean Sea
Mercury
Scavenging
Sea water
Sediments
Trace metals
Uranium
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Abstract The concentrations of mercury (Hg) and other trace metals (Ni, Cu, Zn, Mo, Ba, Re, U) and the Hg isotopic composition were examined across a dramatic redox and productivity transition in a mid-Pleistocene Mediterranean Sea sapropel sequence. Characteristic trace metal enrichment in organic-rich layers was observed, with organic-rich sapropel layers ranging in Hg concentration from 314 to 488 ng/g (avg = 385), with an average enrichment in Hg by a factor of 5.9 compared to organic-poor background sediments, which range from 39 to 94 ng/g Hg (avg = 66). Comparison of seawater concentrations and sapropel accumulations of trace metals suggests that organic matter quantitatively delivers Hg to the seafloor. Near complete scavenging of Hg from the water column renders the sapropel Hg isotopic composition representative of mid-Pleistocene Mediterranean seawater. Sapropels have an average δ 202Hg value of −0.91‰ ± 0.15‰ ( n = 5, 1 SD) and Δ 199Hg value of 0.11‰ ± 0.03‰ ( n = 5, 1 SD). Background sediments have an average δ 202Hg of −0.76‰ ± 0.16‰ ( n = 5, 1 SD) and Δ 199Hg of 0.05‰ ± 0.01‰ ( n = 5, 1 SD), which is indistinguishable from the sapropel values. We suggest that the sapropel isotopic composition is most representative of the mid-Pleistocene Tyrrhenian Sea.
AbstractList The concentrations of mercury (Hg) and other trace metals (Ni, Cu, Zn, Mo, Ba, Re, U) and the Hg isotopic composition were examined across a dramatic redox and productivity transition in a mid-Pleistocene Mediterranean Sea sapropel sequence. Characteristic trace metal enrichment in organic-rich layers was observed, with organic-rich sapropel layers ranging in Hg concentration from 314 to 488 ng/g (avg = 385), with an average enrichment in Hg by a factor of 5.9 compared to organic-poor background sediments, which range from 39 to 94 ng/g Hg (avg = 66). Comparison of seawater concentrations and sapropel accumulations of trace metals suggests that organic matter quantitatively delivers Hg to the seafloor. Near complete scavenging of Hg from the water column renders the sapropel Hg isotopic composition representative of mid-Pleistocene Mediterranean seawater. Sapropels have an average δ 202Hg value of −0.91‰ ± 0.15‰ ( n = 5, 1 SD) and Δ 199Hg value of 0.11‰ ± 0.03‰ ( n = 5, 1 SD). Background sediments have an average δ 202Hg of −0.76‰ ± 0.16‰ ( n = 5, 1 SD) and Δ 199Hg of 0.05‰ ± 0.01‰ ( n = 5, 1 SD), which is indistinguishable from the sapropel values. We suggest that the sapropel isotopic composition is most representative of the mid-Pleistocene Tyrrhenian Sea.
The concentrations of mercury (Hg) and other trace metals (Ni, Cu, Zn, Mo, Ba, Re, U) and the Hg isotopic composition were examined across a dramatic redox and productivity transition in a mid-Pleistocene Mediterranean Sea sapropel sequence. Characteristic trace metal enrichment in organic-rich layers was observed, with organic-rich sapropel layers ranging in Hg concentration from 314 to 488 ng/g (avg = 385), with an average enrichment in Hg by a factor of 5.9 compared to organic-poor background sediments, which range from 39 to 94 ng/g Hg (avg = 66). Comparison of seawater concentrations and sapropel accumulations of trace metals suggests that organic matter quantitatively delivers Hg to the seafloor. Near complete scavenging of Hg from the water column renders the sapropel Hg isotopic composition representative of mid-Pleistocene Mediterranean seawater. Sapropels have an average d super(202)Hg value of -0.91ppt +/- 0.15ppt (n = 5, 1 SD) and super(199)Hg value of 0.11ppt +/- 0.03ppt (n = 5, 1 SD). Background sediments have an average d super(202)Hg of -0.76ppt +/- 0.16ppt (n = 5, 1 SD) and super(199)Hg of 0.05ppt +/- 0.01ppt (n = 5, 1 SD), which is indistinguishable from the sapropel values. We suggest that the sapropel isotopic composition is most representative of the mid-Pleistocene Tyrrhenian Sea.
Author Blum, Joel D.
Meyers, Philip A.
Gehrke, Gretchen E.
Author_xml – sequence: 1
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  surname: Gehrke
  fullname: Gehrke, Gretchen E.
  email: gegehrke@umich.edu
  organization: Department of Geological Sciences, University of Michigan, 1100 North University Avenue, Ann Arbor, MI 48109, USA
– sequence: 2
  givenname: Joel D.
  surname: Blum
  fullname: Blum, Joel D.
  organization: Department of Geological Sciences, University of Michigan, 1100 North University Avenue, Ann Arbor, MI 48109, USA
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  givenname: Philip A.
  surname: Meyers
  fullname: Meyers, Philip A.
  organization: Department of Geological Sciences, University of Michigan, 1100 North University Avenue, Ann Arbor, MI 48109, USA
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Snippet The concentrations of mercury (Hg) and other trace metals (Ni, Cu, Zn, Mo, Ba, Re, U) and the Hg isotopic composition were examined across a dramatic redox and...
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SubjectTerms Concentration (composition)
Enrichment
Marine
Mediterranean Sea
Mercury
Scavenging
Sea water
Sediments
Trace metals
Uranium
Title The geochemical behavior and isotopic composition of Hg in a mid-Pleistocene western Mediterranean sapropel
URI https://dx.doi.org/10.1016/j.gca.2008.12.012
https://search.proquest.com/docview/1671572341
https://search.proquest.com/docview/759317048
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