Fabrication of Freestanding Nanoparticle Membranes over Wells
Freestanding nanoparticle membranes over circular wells are prepared by utilizing surface engineering. The crucial step of this method is the hydrophobic treatment of the substrate surface, which causes the water droplet to be suspended over wells during drying. Consequently, the nanoparticle monola...
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Published in | Langmuir Vol. 31; no. 12; pp. 3738 - 3744 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
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United States
American Chemical Society
31.03.2015
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Abstract | Freestanding nanoparticle membranes over circular wells are prepared by utilizing surface engineering. The crucial step of this method is the hydrophobic treatment of the substrate surface, which causes the water droplet to be suspended over wells during drying. Consequently, the nanoparticle monolayer self-assembled at the surface of the water droplet would drape itself over wells instead of being dragged into wells and ruptured into patches after the evaporation of water. This scenario was confirmed by the results of control experiments with changes in the hydrophobicity of the surface and the depth of wells. Moreover, the NaCl crystallization experiment provides additional evidence for the dynamic process of drying. Freestanding nanoparticle membranes with different nanoparticle core sizes and different lengths of ligands have been successfully prepared using the same route. The Young’s modulus of one typical kind of prepared freestanding nanoparticle membrane was measured with force microscopy. |
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AbstractList | Freestanding nanoparticle membranes over circular wells are prepared by utilizing surface engineering. The crucial step of this method is the hydrophobic treatment of the substrate surface, which causes the water droplet to be suspended over wells during drying. Consequently, the nanoparticle monolayer self-assembled at the surface of the water droplet would drape itself over wells instead of being dragged into wells and ruptured into patches after the evaporation of water. This scenario was confirmed by the results of control experiments with changes in the hydrophobicity of the surface and the depth of wells. Moreover, the NaCl crystallization experiment provides additional evidence for the dynamic process of drying. Freestanding nanoparticle membranes with different nanoparticle core sizes and different lengths of ligands have been successfully prepared using the same route. The Young's modulus of one typical kind of prepared freestanding nanoparticle membrane was measured with force microscopy. |
Author | Liu, Shuhai Zhang, Chaoying Zhang, Li Guan, Changrong Wang, Ying Huang, Wenhong Liao, Jianhui |
AuthorAffiliation | Key Laboratory for the Physics and Chemistry of Nanodevices, Department of Electronics Peking University Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of Science |
AuthorAffiliation_xml | – name: Peking University – name: Key Laboratory for the Physics and Chemistry of Nanodevices, Department of Electronics – name: Beijing Institute of Nanoenergy and Nanosystems – name: Chinese Academy of Science |
Author_xml | – sequence: 1 givenname: Changrong surname: Guan fullname: Guan, Changrong – sequence: 2 givenname: Li surname: Zhang fullname: Zhang, Li – sequence: 3 givenname: Shuhai surname: Liu fullname: Liu, Shuhai – sequence: 4 givenname: Ying surname: Wang fullname: Wang, Ying – sequence: 5 givenname: Wenhong surname: Huang fullname: Huang, Wenhong – sequence: 6 givenname: Chaoying surname: Zhang fullname: Zhang, Chaoying – sequence: 7 givenname: Jianhui surname: Liao fullname: Liao, Jianhui email: Jianhui.Liao@pku.edu.cn |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25741888$$D View this record in MEDLINE/PubMed |
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