Stibonium Ions for the Fluorescence Turn-On Sensing of F– in Drinking Water at Parts per Million Concentrations

The 9-anthryltriphenylstibonium cation, [1]+, has been synthesized and used as a sensor for the toxic fluoride anion in water. This stibonium cation complexes fluoride ions to afford the corresponding fluorostiborane 1-F. This reaction, which occurs at fluoride concentrations in the parts per millio...

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Published inJournal of the American Chemical Society Vol. 134; no. 37; pp. 15309 - 15311
Main Authors Ke, Iou-Sheng, Myahkostupov, Mykhaylo, Castellano, Felix N, Gabbaï, François P
Format Journal Article
LanguageEnglish
Published WASHINGTON American Chemical Society 19.09.2012
Amer Chemical Soc
Subjects
Anions
Chemistry
Chemistry, Multidisciplinary
Drinking Water - analysis
Fluorescence
Fluorides - analysis
Physical Sciences
Science & Technology
Spectrometry, Fluorescence
ANIONS
GOLD
COMPLEXATION
ENHANCEMENT
FLUORIDE
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Abstract The 9-anthryltriphenylstibonium cation, [1]+, has been synthesized and used as a sensor for the toxic fluoride anion in water. This stibonium cation complexes fluoride ions to afford the corresponding fluorostiborane 1-F. This reaction, which occurs at fluoride concentrations in the parts per million range, is accompanied by a drastic fluorescence turn-on response. It is also highly selective and can be used in plain tap water or bottled water to test fluoridation levels.
AbstractList The 9-anthryltriphenylstibonium cation, [1](+), has been synthesized and used as a sensor for the toxic fluoride anion in water. This stibonium cation complexes fluoride ions to afford the corresponding fluorostiborane 1-F. This reaction, which occurs at fluoride concentrations in the parts per million range, is accompanied by a drastic fluorescence turn-on response. It is also highly selective and can be used in plain tap water or bottled water to test fluoridation levels.
Author Gabbaï, François P
Myahkostupov, Mykhaylo
Ke, Iou-Sheng
Castellano, Felix N
AuthorAffiliation Texas A&M University
Bowling Green State University
AuthorAffiliation_xml – name: Bowling Green State University
– name: Texas A&M University
Author_xml – sequence: 1
  givenname: Iou-Sheng
  surname: Ke
  fullname: Ke, Iou-Sheng
– sequence: 2
  givenname: Mykhaylo
  surname: Myahkostupov
  fullname: Myahkostupov, Mykhaylo
– sequence: 3
  givenname: Felix N
  surname: Castellano
  fullname: Castellano, Felix N
  email: francois@tamu.edu, castell@bgsu.edu
– sequence: 4
  givenname: François P
  surname: Gabbaï
  fullname: Gabbaï, François P
  email: francois@tamu.edu, castell@bgsu.edu
BackLink https://www.ncbi.nlm.nih.gov/pubmed/22954306$$D View this record in MEDLINE/PubMed
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GOLD
COMPLEXATION
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FLUORIDE
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Snippet The 9-anthryltriphenylstibonium cation, [1]+, has been synthesized and used as a sensor for the toxic fluoride anion in water. This stibonium cation complexes...
The 9-anthryltriphenylstibonium cation, [1](+), has been synthesized and used as a sensor for the toxic fluoride anion in water. This stibonium cation...
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StartPage 15309
SubjectTerms Anions
Chemistry
Chemistry, Multidisciplinary
Drinking Water - analysis
Fluorescence
Fluorides - analysis
Physical Sciences
Science & Technology
Spectrometry, Fluorescence
Title Stibonium Ions for the Fluorescence Turn-On Sensing of F– in Drinking Water at Parts per Million Concentrations
URI http://dx.doi.org/10.1021/ja308194w
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https://www.ncbi.nlm.nih.gov/pubmed/22954306
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