Spontaneous Periodic Diameter Oscillations in InP Nanowires: The Role of Interface Instabilities
We have observed that thin InP nanowires generated by vapor–liquid–solid growth display spontaneous periodic diameter oscillations when large group III supersaturations are used. Diameter variations are associated with a large number of stacking faults and crystallographic phase changes(wurtzite/zin...
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Published in | Nano letters Vol. 13; no. 1; pp. 9 - 13 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
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American Chemical Society
09.01.2013
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Abstract | We have observed that thin InP nanowires generated by vapor–liquid–solid growth display spontaneous periodic diameter oscillations when large group III supersaturations are used. Diameter variations are associated with a large number of stacking faults and crystallographic phase changes(wurtzite/zinc-blende); also the axial distance between oscillations depends on the indium precursor flow used during the run. We attribute the morphology changes to a substantial deformation of the triple phase line (vapor–liquid–solid) at the catalyst nanoparticle edge originated from multistep nucleation during growth. The deformation alters the mechanical force balance acting on the nanoparticle during growth in such a way that the particle displaces from the nanowire top and wets the nanowire sidewall. Subsequently, as catalytic growth occurs at the sidewall, the associated increase in diameter will eventually push the NP back to its original wire-top position until the onset of a new instability at the triple phase line. |
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AbstractList | We have observed that thin InP nanowires generated by vapor-liquid-solid growth display spontaneous periodic diameter oscillations when large group III supersaturations are used. Diameter variations are associated with a large number of stacking faults and crystallographic phase changes(wurtzite/zinc-blende); also the axial distance between oscillations depends on the indium precursor flow used during the run. We attribute the morphology changes to a substantial deformation of the triple phase line (vapor-liquid-solid) at the catalyst nanoparticle edge originated from multistep nucleation during growth. The deformation alters the mechanical force balance acting on the nanoparticle during growth in such a way that the particle displaces from the nanowire top and wets the nanowire sidewall. Subsequently, as catalytic growth occurs at the sidewall, the associated increase in diameter will eventually push the NP back to its original wire-top position until the onset of a new instability at the triple phase line. |
Author | Tizei, L. H. G Oliveira, D. S Ugarte, D Cotta, M. A |
AuthorAffiliation | Universidade Estadual de Campinas |
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Keywords | Nanowire vapor−liquid−solid InP wetting kinetic roughness Stacking faults Deformation Nucleation Catalysts Phase transformations Crystal growth from vapors Ruthenium nitride Precursor III-V compound Indium phosphide Zinc Interfaces Nanoparticles Vapor phase Morphology Growth mechanism Instability Nanowires Nanostructured materials Nanomaterial synthesis III-V semiconductors |
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Snippet | We have observed that thin InP nanowires generated by vapor–liquid–solid growth display spontaneous periodic diameter oscillations when large group III... We have observed that thin InP nanowires generated by vapor-liquid-solid growth display spontaneous periodic diameter oscillations when large group III... |
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SubjectTerms | Catalysts Condensed matter: structure, mechanical and thermal properties Cross-disciplinary physics: materials science; rheology Deformation Equations of state, phase equilibria, and phase transitions Exact sciences and technology Indium phosphides Instability Low-dimensional structures (superlattices, quantum well structures, multilayers): structure, and nonelectronic properties Materials science Nanocrystalline materials Nanoscale materials and structures: fabrication and characterization Nanostructure Nanowires Oscillations Phase transformations Physics Quantum wires Specific phase transitions Spontaneous Structural transitions in nanoscale materials Surfaces and interfaces; thin films and whiskers (structure and nonelectronic properties) |
Title | Spontaneous Periodic Diameter Oscillations in InP Nanowires: The Role of Interface Instabilities |
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