Glass-Encapsulated Light Harvesters: More Efficient Dye-Sensitized Solar Cells by Deposition of Self-Aligned, Conformal, and Self-Limited Silica Layers
A major loss mechanism in dye-sensitized solar cells (DSCs) is recombination at the TiO2/electrolyte interface. Here we report a method to reduce greatly this loss mechanism. We deposit insulating and transparent silica (SiO2) onto the open areas of a nanoparticulate TiO2 surface while avoiding any...
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| Published in | Journal of the American Chemical Society Vol. 134; no. 23; pp. 9537 - 9540 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
13.06.2012
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| Online Access | Get full text |
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| Abstract | A major loss mechanism in dye-sensitized solar cells (DSCs) is recombination at the TiO2/electrolyte interface. Here we report a method to reduce greatly this loss mechanism. We deposit insulating and transparent silica (SiO2) onto the open areas of a nanoparticulate TiO2 surface while avoiding any deposition of SiO2 over or under the organic dye molecules. The SiO2 coating covers the highly convoluted surface of the TiO2 conformally and with a uniform thickness throughout the thousands of layers of nanoparticles. DSCs incorporating these selective and self-aligned SiO2 layers achieved a 36% increase in relative efficiency versus control uncoated cells. |
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| AbstractList | A major loss mechanism in dye-sensitized solar cells (DSCs) is recombination at the TiO2/electrolyte interface. Here we report a method to reduce greatly this loss mechanism. We deposit insulating and transparent silica (SiO2) onto the open areas of a nanoparticulate TiO2 surface while avoiding any deposition of SiO2 over or under the organic dye molecules. The SiO2 coating covers the highly convoluted surface of the TiO2 conformally and with a uniform thickness throughout the thousands of layers of nanoparticles. DSCs incorporating these selective and self-aligned SiO2 layers achieved a 36% increase in relative efficiency versus control uncoated cells. A major loss mechanism in dye-sensitized solar cells (DSCs) is recombination at the TiO(2)/electrolyte interface. Here we report a method to reduce greatly this loss mechanism. We deposit insulating and transparent silica (SiO(2)) onto the open areas of a nanoparticulate TiO(2) surface while avoiding any deposition of SiO(2) over or under the organic dye molecules. The SiO(2) coating covers the highly convoluted surface of the TiO(2) conformally and with a uniform thickness throughout the thousands of layers of nanoparticles. DSCs incorporating these selective and self-aligned SiO(2) layers achieved a 36% increase in relative efficiency versus control uncoated cells. |
| Author | Son, Ho-Jin Gordon, Roy G Aaltonen, Titta Hupp, Joseph T Prasittichai, Chaiya Wang, Xinwei Jeong, Nak Cheon |
| AuthorAffiliation | Northwestern University Harvard University Argonne National Laboratory |
| AuthorAffiliation_xml | – name: Argonne National Laboratory – name: Harvard University – name: Northwestern University |
| Author_xml | – sequence: 1 givenname: Ho-Jin surname: Son fullname: Son, Ho-Jin – sequence: 2 givenname: Xinwei surname: Wang fullname: Wang, Xinwei – sequence: 3 givenname: Chaiya surname: Prasittichai fullname: Prasittichai, Chaiya – sequence: 4 givenname: Nak Cheon surname: Jeong fullname: Jeong, Nak Cheon – sequence: 5 givenname: Titta surname: Aaltonen fullname: Aaltonen, Titta – sequence: 6 givenname: Roy G surname: Gordon fullname: Gordon, Roy G email: gordon@chemistry.harvard.edu, j-hupp@northwestern.edu – sequence: 7 givenname: Joseph T surname: Hupp fullname: Hupp, Joseph T email: gordon@chemistry.harvard.edu, j-hupp@northwestern.edu |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22650384$$D View this record in MEDLINE/PubMed |
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