Phase Engineering of Iron–Cobalt Sulfides for Zn–Air and Na–Ion Batteries

Rechargeable batteries are promising platforms for sustainable development of energy conversion and storage technologies. Highly efficient multifunctional electrodes based on bimetallic sulfides for rechargeable batteries are extremely desirable but still challenging to tailor with controllable phas...

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Published inACS nano Vol. 14; no. 8; pp. 10438 - 10451
Main Authors Lu, Shu, Jiang, Jun, Yang, Hai, Zhang, Ying-Jie, Pei, Dan-Ni, Chen, Jie-Jie, Yu, Yan
Format Journal Article
LanguageEnglish
Published American Chemical Society 25.08.2020
Subjects
iron cobalt sulfides
Zn−air battery
alloying and support effect
energy storage
Na−ion battery
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Abstract Rechargeable batteries are promising platforms for sustainable development of energy conversion and storage technologies. Highly efficient multifunctional electrodes based on bimetallic sulfides for rechargeable batteries are extremely desirable but still challenging to tailor with controllable phase and structure. Here, we report a colloidal strategy to fabricate FeCo-based bimetallic sulfides on reduced graphene oxide (rGO), which are expected to display highly efficient oxygen electrocatalysis and sodium storage performances. Specifically, as-screened FeCo8S8 nanosheets (NSs) on rGO originating from suitable tailoring of the Co9S8 matrix with Fe at the atomic level exhibited a very low potential difference (0.77 V) at 10 mA cm–2 and negligible voltage loss after 200 cycles as an air electrode for Zn–air batteries. For Na–ion batteries, FeCo8S8 NS/rGO demonstrated a superior high-rate capability (188 mAh g–1 at 20 A g–1) with long-term cycling stability. The bifunctional electrocatalytic property and sodium storage performance are attributed to not only the synergistic effect of Fe/Co but also the optimized catalytic activity and ion transport ability by the in situ rGO hybrid. This work demonstrates the potential applications of FeCo-based bimetallic sulfides as efficient electrode materials for both rechargeable Zn–air and Na–ion batteries.
AbstractList Rechargeable batteries are promising platforms for sustainable development of energy conversion and storage technologies. Highly efficient multifunctional electrodes based on bimetallic sulfides for rechargeable batteries are extremely desirable but still challenging to tailor with controllable phase and structure. Here, we report a colloidal strategy to fabricate FeCo-based bimetallic sulfides on reduced graphene oxide (rGO), which are expected to display highly efficient oxygen electrocatalysis and sodium storage performances. Specifically, as-screened FeCo8S8 nanosheets (NSs) on rGO originating from suitable tailoring of the Co9S8 matrix with Fe at the atomic level exhibited a very low potential difference (0.77 V) at 10 mA cm–2 and negligible voltage loss after 200 cycles as an air electrode for Zn–air batteries. For Na–ion batteries, FeCo8S8 NS/rGO demonstrated a superior high-rate capability (188 mAh g–1 at 20 A g–1) with long-term cycling stability. The bifunctional electrocatalytic property and sodium storage performance are attributed to not only the synergistic effect of Fe/Co but also the optimized catalytic activity and ion transport ability by the in situ rGO hybrid. This work demonstrates the potential applications of FeCo-based bimetallic sulfides as efficient electrode materials for both rechargeable Zn–air and Na–ion batteries.
Rechargeable batteries are promising platforms for sustainable development of energy conversion and storage technologies. Highly efficient multifunctional electrodes based on bimetallic sulfides for rechargeable batteries are extremely desirable but still challenging to tailor with controllable phase and structure. Here, we report a colloidal strategy to fabricate FeCo-based bimetallic sulfides on reduced graphene oxide (rGO), which are expected to display highly efficient oxygen electrocatalysis and sodium storage performances. Specifically, as-screened FeCo8S8 nanosheets (NSs) on rGO originating from suitable tailoring of the Co9S8 matrix with Fe at the atomic level exhibited a very low potential difference (0.77 V) at 10 mA cm-2 and negligible voltage loss after 200 cycles as an air electrode for Zn-air batteries. For Na-ion batteries, FeCo8S8 NS/rGO demonstrated a superior high-rate capability (188 mAh g-1 at 20 A g-1) with long-term cycling stability. The bifunctional electrocatalytic property and sodium storage performance are attributed to not only the synergistic effect of Fe/Co but also the optimized catalytic activity and ion transport ability by the in situ rGO hybrid. This work demonstrates the potential applications of FeCo-based bimetallic sulfides as efficient electrode materials for both rechargeable Zn-air and Na-ion batteries.Rechargeable batteries are promising platforms for sustainable development of energy conversion and storage technologies. Highly efficient multifunctional electrodes based on bimetallic sulfides for rechargeable batteries are extremely desirable but still challenging to tailor with controllable phase and structure. Here, we report a colloidal strategy to fabricate FeCo-based bimetallic sulfides on reduced graphene oxide (rGO), which are expected to display highly efficient oxygen electrocatalysis and sodium storage performances. Specifically, as-screened FeCo8S8 nanosheets (NSs) on rGO originating from suitable tailoring of the Co9S8 matrix with Fe at the atomic level exhibited a very low potential difference (0.77 V) at 10 mA cm-2 and negligible voltage loss after 200 cycles as an air electrode for Zn-air batteries. For Na-ion batteries, FeCo8S8 NS/rGO demonstrated a superior high-rate capability (188 mAh g-1 at 20 A g-1) with long-term cycling stability. The bifunctional electrocatalytic property and sodium storage performance are attributed to not only the synergistic effect of Fe/Co but also the optimized catalytic activity and ion transport ability by the in situ rGO hybrid. This work demonstrates the potential applications of FeCo-based bimetallic sulfides as efficient electrode materials for both rechargeable Zn-air and Na-ion batteries.
Author Yang, Hai
Zhang, Ying-Jie
Chen, Jie-Jie
Yu, Yan
Jiang, Jun
Pei, Dan-Ni
Lu, Shu
AuthorAffiliation University of Science and Technology of China
Dalian National Laboratory for Clean Energy (DNL)
CAS Key Laboratory of Urban Pollutant Conversion, Department of Applied Chemistry
Chinese Academy of Sciences (CAS)
National Synchrotron Radiation Laboratory
School of Metallurgy and Environment
Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering
University of Science & Technology of China
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Keywords iron cobalt sulfides
Zn−air battery
alloying and support effect
energy storage
Na−ion battery
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Snippet Rechargeable batteries are promising platforms for sustainable development of energy conversion and storage technologies. Highly efficient multifunctional...
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Title Phase Engineering of Iron–Cobalt Sulfides for Zn–Air and Na–Ion Batteries
URI http://dx.doi.org/10.1021/acsnano.0c04309
https://www.proquest.com/docview/2427303356
Volume 14
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