Reduced Graphene Oxide Conformally Wrapped Silver Nanowire Networks for Flexible Transparent Heating and Electromagnetic Interference Shielding
Metal nanowire networks (MNNs) are promising as transparent electrode materials for a diverse range of optoelectronic devices and also work as active materials for electrical heating and electromagnetic interference (EMI) shielding applications. However, the relatively low performance and poor durab...
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| Published in | ACS nano Vol. 14; no. 7; pp. 8754 - 8765 |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
28.07.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Metal nanowire networks (MNNs) are promising as transparent electrode materials for a diverse range of optoelectronic devices and also work as active materials for electrical heating and electromagnetic interference (EMI) shielding applications. However, the relatively low performance and poor durability of MNNs are limiting the practical application of the resulting devices. Here, we report a controllable approach to enhance the conductivity and the stability of MNNs with their transmittance remaining unchanged, in which reduced graphene oxide conformally wrapped silver nanowire networks (AgNW@rGO networks) are synthesized by selective electrodeposition of GO nanosheets on AgNWs followed by a pulsed laser irradiation treatment. Experimental characterizations and finite-difference time-domain simulations indicate that pulsed laser irradiation at a specific wavelength not only reduces the GO but also welds the AgNWs together through a surface plasmon resonance process. As a result, the AgNW@rGO networks exhibit low sheet resistance of 3.3 Ω/□, average transmittance of 91.1%, and good flexibility. Wrapping with rGO improves the maximum electrical heating temperature of the AgNW network transparent heaters due to the effective suppression of the oxidation and the migration of surface silver atoms. In addition, excellent EMI shielding effectiveness of up to 35.5 dB in the 8.2–12.4 GHz frequency range is obtained as a consequence of the combined effects of dual reflection, conduction loss, and multiple dielectric polarization relaxation processes. |
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| AbstractList | Metal nanowire networks (MNNs) are promising as transparent electrode materials for a diverse range of optoelectronic devices and also work as active materials for electrical heating and electromagnetic interference (EMI) shielding applications. However, the relatively low performance and poor durability of MNNs are limiting the practical application of the resulting devices. Here, we report a controllable approach to enhance the conductivity and the stability of MNNs with their transmittance remaining unchanged, in which reduced graphene oxide conformally wrapped silver nanowire networks (AgNW@rGO networks) are synthesized by selective electrodeposition of GO nanosheets on AgNWs followed by a pulsed laser irradiation treatment. Experimental characterizations and finite-difference time-domain simulations indicate that pulsed laser irradiation at a specific wavelength not only reduces the GO but also welds the AgNWs together through a surface plasmon resonance process. As a result, the AgNW@rGO networks exhibit low sheet resistance of 3.3 Ω/□, average transmittance of 91.1%, and good flexibility. Wrapping with rGO improves the maximum electrical heating temperature of the AgNW network transparent heaters due to the effective suppression of the oxidation and the migration of surface silver atoms. In addition, excellent EMI shielding effectiveness of up to 35.5 dB in the 8.2-12.4 GHz frequency range is obtained as a consequence of the combined effects of dual reflection, conduction loss, and multiple dielectric polarization relaxation processes.Metal nanowire networks (MNNs) are promising as transparent electrode materials for a diverse range of optoelectronic devices and also work as active materials for electrical heating and electromagnetic interference (EMI) shielding applications. However, the relatively low performance and poor durability of MNNs are limiting the practical application of the resulting devices. Here, we report a controllable approach to enhance the conductivity and the stability of MNNs with their transmittance remaining unchanged, in which reduced graphene oxide conformally wrapped silver nanowire networks (AgNW@rGO networks) are synthesized by selective electrodeposition of GO nanosheets on AgNWs followed by a pulsed laser irradiation treatment. Experimental characterizations and finite-difference time-domain simulations indicate that pulsed laser irradiation at a specific wavelength not only reduces the GO but also welds the AgNWs together through a surface plasmon resonance process. As a result, the AgNW@rGO networks exhibit low sheet resistance of 3.3 Ω/□, average transmittance of 91.1%, and good flexibility. Wrapping with rGO improves the maximum electrical heating temperature of the AgNW network transparent heaters due to the effective suppression of the oxidation and the migration of surface silver atoms. In addition, excellent EMI shielding effectiveness of up to 35.5 dB in the 8.2-12.4 GHz frequency range is obtained as a consequence of the combined effects of dual reflection, conduction loss, and multiple dielectric polarization relaxation processes. Metal nanowire networks (MNNs) are promising as transparent electrode materials for a diverse range of optoelectronic devices and also work as active materials for electrical heating and electromagnetic interference (EMI) shielding applications. However, the relatively low performance and poor durability of MNNs are limiting the practical application of the resulting devices. Here, we report a controllable approach to enhance the conductivity and the stability of MNNs with their transmittance remaining unchanged, in which reduced graphene oxide conformally wrapped silver nanowire networks (AgNW@rGO networks) are synthesized by selective electrodeposition of GO nanosheets on AgNWs followed by a pulsed laser irradiation treatment. Experimental characterizations and finite-difference time-domain simulations indicate that pulsed laser irradiation at a specific wavelength not only reduces the GO but also welds the AgNWs together through a surface plasmon resonance process. As a result, the AgNW@rGO networks exhibit low sheet resistance of 3.3 Ω/□, average transmittance of 91.1%, and good flexibility. Wrapping with rGO improves the maximum electrical heating temperature of the AgNW network transparent heaters due to the effective suppression of the oxidation and the migration of surface silver atoms. In addition, excellent EMI shielding effectiveness of up to 35.5 dB in the 8.2–12.4 GHz frequency range is obtained as a consequence of the combined effects of dual reflection, conduction loss, and multiple dielectric polarization relaxation processes. |
| Author | Chen, Sai Li, Wanli Liu, Yichun Zhao, Xiaoning Chang, Huicong Li, Peng Ma, Jiangang Yang, Yang Li, Bingsheng Xiao, Lin Xu, Haiyang Ju, Zhongshi |
| AuthorAffiliation | Qian Xuesen Laboratory of Space Technology Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education Center for Functional Sensor & Actuator and World Premier International Center for Materials Nanoarchitectonics |
| AuthorAffiliation_xml | – name: Center for Functional Sensor & Actuator and World Premier International Center for Materials Nanoarchitectonics – name: Qian Xuesen Laboratory of Space Technology – name: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education |
| Author_xml | – sequence: 1 givenname: Yang surname: Yang fullname: Yang, Yang organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 2 givenname: Sai surname: Chen fullname: Chen, Sai organization: Qian Xuesen Laboratory of Space Technology – sequence: 3 givenname: Wanli surname: Li fullname: Li, Wanli organization: Center for Functional Sensor & Actuator and World Premier International Center for Materials Nanoarchitectonics – sequence: 4 givenname: Peng orcidid: 0000-0002-0933-2592 surname: Li fullname: Li, Peng email: lip032@nenu.edu.cn organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 5 givenname: Jiangang surname: Ma fullname: Ma, Jiangang email: majg@nenu.edu.cn organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 6 givenname: Bingsheng surname: Li fullname: Li, Bingsheng organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 7 givenname: Xiaoning orcidid: 0000-0002-0082-2288 surname: Zhao fullname: Zhao, Xiaoning organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 8 givenname: Zhongshi surname: Ju fullname: Ju, Zhongshi organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 9 givenname: Huicong surname: Chang fullname: Chang, Huicong organization: Qian Xuesen Laboratory of Space Technology – sequence: 10 givenname: Lin surname: Xiao fullname: Xiao, Lin organization: Qian Xuesen Laboratory of Space Technology – sequence: 11 givenname: Haiyang surname: Xu fullname: Xu, Haiyang organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education – sequence: 12 givenname: Yichun surname: Liu fullname: Liu, Yichun organization: Key Laboratory of UV-Emitting Materials and Technology, Ministry of Education |
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| Keywords | reduced graphene oxide flexible transparent electrodes electromagnetic interference shielding silver nanowire networks transparent heaters |
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| Snippet | Metal nanowire networks (MNNs) are promising as transparent electrode materials for a diverse range of optoelectronic devices and also work as active materials... |
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| Title | Reduced Graphene Oxide Conformally Wrapped Silver Nanowire Networks for Flexible Transparent Heating and Electromagnetic Interference Shielding |
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