Geochemical characteristics and influencing factors of dissolved rare-earth elements in rivers of coal grain composite area in eastern China

Rare-earth elements are widely used in the study of source tracing and geochemical characteristics, which can reflect the degree of influence of human activities on water environment. In order to reveal the additive effects of various human activities on the geochemical characteristics of rare-earth...

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Published in	Environmental earth sciences Vol. 83; no. 2; p. 78
Main Authors	Hu, Mingyu, Jiang, Chunlu, Xia, Xiang, Li, Yanan
Format	Journal Article
Language	English
Published	Berlin/Heidelberg Springer Berlin Heidelberg 01.01.2024 Springer Nature B.V
Subjects	Additives adsorption Agricultural production atomic absorption spectrometry Biogeosciences China Coal Crystallization Distribution Earth Earth and Environmental Science Earth Sciences Elements Environmental behavior Environmental Science and Engineering Fractionation Gadolinium Geochemistry Geology humans Hydrology/Water Resources Inductively coupled plasma mass spectrometry Mass spectrometry Mass spectroscopy Original Article Plagioclase Rare earth elements Rivers Spatial distribution Surface water Terrestrial Pollution Urbanization Water analysis Water sampling China Coal grain composite area Geochemical characteristics Rare-earth elements Influencing factors
Online Access	Get full text
ISSN	1866-6280 1866-6299
DOI	10.1007/s12665-023-11365-5

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Abstract	Rare-earth elements are widely used in the study of source tracing and geochemical characteristics, which can reflect the degree of influence of human activities on water environment. In order to reveal the additive effects of various human activities on the geochemical characteristics of rare-earth elements in the surface water environment, the content of rare-earth elements in the river in the coal grain composite area of eastern China was determined by inductively coupled plasma mass spectrometry (ICP-MS). The results showed that all water samples were alkaline, ΣREE content ranged 0.18–0.88 μg·L −1 , with an average value of 0.28 μg·L −1 . All the water samples showed significant enrichment of light rare-earth elements due to a combination of natural processes and external inputs. The spatial distribution and fractionation characteristics of rare-earth elements show that rare-earth elements (especially Ce) are prone to adsorption/complexation reactions with colloidal particles, resulting in their removal from rivers, Eu anomaly is related to plagioclase crystallization and human activities (coal development, agricultural production, urbanization process), and Gd anomaly is only related to human activities. The research results can provide scientific reference for revealing the distribution of rare-earth elements and geochemical environmental behavior in rivers environment under the superimposed influence of various human activities.
AbstractList	Rare-earth elements are widely used in the study of source tracing and geochemical characteristics, which can reflect the degree of influence of human activities on water environment. In order to reveal the additive effects of various human activities on the geochemical characteristics of rare-earth elements in the surface water environment, the content of rare-earth elements in the river in the coal grain composite area of eastern China was determined by inductively coupled plasma mass spectrometry (ICP-MS). The results showed that all water samples were alkaline, ΣREE content ranged 0.18–0.88 μg·L−1, with an average value of 0.28 μg·L−1. All the water samples showed significant enrichment of light rare-earth elements due to a combination of natural processes and external inputs. The spatial distribution and fractionation characteristics of rare-earth elements show that rare-earth elements (especially Ce) are prone to adsorption/complexation reactions with colloidal particles, resulting in their removal from rivers, Eu anomaly is related to plagioclase crystallization and human activities (coal development, agricultural production, urbanization process), and Gd anomaly is only related to human activities. The research results can provide scientific reference for revealing the distribution of rare-earth elements and geochemical environmental behavior in rivers environment under the superimposed influence of various human activities. Rare-earth elements are widely used in the study of source tracing and geochemical characteristics, which can reflect the degree of influence of human activities on water environment. In order to reveal the additive effects of various human activities on the geochemical characteristics of rare-earth elements in the surface water environment, the content of rare-earth elements in the river in the coal grain composite area of eastern China was determined by inductively coupled plasma mass spectrometry (ICP-MS). The results showed that all water samples were alkaline, ΣREE content ranged 0.18–0.88 μg·L⁻¹, with an average value of 0.28 μg·L⁻¹. All the water samples showed significant enrichment of light rare-earth elements due to a combination of natural processes and external inputs. The spatial distribution and fractionation characteristics of rare-earth elements show that rare-earth elements (especially Ce) are prone to adsorption/complexation reactions with colloidal particles, resulting in their removal from rivers, Eu anomaly is related to plagioclase crystallization and human activities (coal development, agricultural production, urbanization process), and Gd anomaly is only related to human activities. The research results can provide scientific reference for revealing the distribution of rare-earth elements and geochemical environmental behavior in rivers environment under the superimposed influence of various human activities. Rare-earth elements are widely used in the study of source tracing and geochemical characteristics, which can reflect the degree of influence of human activities on water environment. In order to reveal the additive effects of various human activities on the geochemical characteristics of rare-earth elements in the surface water environment, the content of rare-earth elements in the river in the coal grain composite area of eastern China was determined by inductively coupled plasma mass spectrometry (ICP-MS). The results showed that all water samples were alkaline, ΣREE content ranged 0.18–0.88 μg·L −1 , with an average value of 0.28 μg·L −1 . All the water samples showed significant enrichment of light rare-earth elements due to a combination of natural processes and external inputs. The spatial distribution and fractionation characteristics of rare-earth elements show that rare-earth elements (especially Ce) are prone to adsorption/complexation reactions with colloidal particles, resulting in their removal from rivers, Eu anomaly is related to plagioclase crystallization and human activities (coal development, agricultural production, urbanization process), and Gd anomaly is only related to human activities. The research results can provide scientific reference for revealing the distribution of rare-earth elements and geochemical environmental behavior in rivers environment under the superimposed influence of various human activities.
ArticleNumber	78
Author	Hu, Mingyu Jiang, Chunlu Xia, Xiang Li, Yanan
Author_xml	– sequence: 1 givenname: Mingyu surname: Hu fullname: Hu, Mingyu organization: School of Resources and Environmental Engineering, Anhui University – sequence: 2 givenname: Chunlu surname: Jiang fullname: Jiang, Chunlu email: cumtclj@cumt.edu.cn organization: School of Resources and Environmental Engineering, Anhui University, School of Resources and Geoscience, China University of Mining and Technology – sequence: 3 givenname: Xiang surname: Xia fullname: Xia, Xiang organization: School of Resources and Environmental Engineering, Anhui University – sequence: 4 givenname: Yanan surname: Li fullname: Li, Yanan organization: School of Resources and Environmental Engineering, Anhui University
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Snippet	Rare-earth elements are widely used in the study of source tracing and geochemical characteristics, which can reflect the degree of influence of human...
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SubjectTerms	Additives adsorption Agricultural production atomic absorption spectrometry Biogeosciences China Coal Crystallization Distribution Earth Earth and Environmental Science Earth Sciences Elements Environmental behavior Environmental Science and Engineering Fractionation Gadolinium Geochemistry Geology humans Hydrology/Water Resources Inductively coupled plasma mass spectrometry Mass spectrometry Mass spectroscopy Original Article Plagioclase Rare earth elements Rivers Spatial distribution Surface water Terrestrial Pollution Urbanization Water analysis Water sampling
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Title	Geochemical characteristics and influencing factors of dissolved rare-earth elements in rivers of coal grain composite area in eastern China
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