Programming Hierarchical Self-Assembly of Patchy Particles into Colloidal Crystals via Colloidal Molecules
Colloidal self-assembly is a promising bottom-up route to a wide variety of three-dimensional structures, from clusters to crystals. Programming hierarchical self-assembly of colloidal building blocks, which can give rise to structures ordered at multiple levels to rival biological complexity, poses...
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| Published in | ACS nano Vol. 12; no. 3; pp. 2355 - 2364 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
27.03.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Colloidal self-assembly is a promising bottom-up route to a wide variety of three-dimensional structures, from clusters to crystals. Programming hierarchical self-assembly of colloidal building blocks, which can give rise to structures ordered at multiple levels to rival biological complexity, poses a multiscale design problem. Here we explore a generic design principle that exploits a hierarchy of interaction strengths and employ this design principle in computer simulations to demonstrate the hierarchical self-assembly of triblock patchy colloidal particles into two distinct colloidal crystals. We obtain cubic diamond and body-centered cubic crystals via distinct clusters of uniform size and shape, namely, tetrahedra and octahedra, respectively. Such a conceptual design framework has the potential to reliably encode hierarchical self-assembly of colloidal particles into a high level of sophistication. Moreover, the design framework underpins a bottom-up route to cubic diamond colloidal crystals, which have remained elusive despite being much sought after for their attractive photonic applications. |
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| AbstractList | Colloidal self-assembly is a promising bottom-up route to a wide variety of three-dimensional structures, from clusters to crystals. Programming hierarchical self-assembly of colloidal building blocks, which can give rise to structures ordered at multiple levels to rival biological complexity, poses a multiscale design problem. Here we explore a generic design principle that exploits a hierarchy of interaction strengths and employ this design principle in computer simulations to demonstrate the hierarchical self-assembly of triblock patchy colloidal particles into two distinct colloidal crystals. We obtain cubic diamond and body-centered cubic crystals via distinct clusters of uniform size and shape, namely, tetrahedra and octahedra, respectively. Such a conceptual design framework has the potential to reliably encode hierarchical self-assembly of colloidal particles into a high level of sophistication. Moreover, the design framework underpins a bottom-up route to cubic diamond colloidal crystals, which have remained elusive despite being much sought after for their attractive photonic applications. |
| Author | Avins, Christopher Chakrabarti, Dwaipayan Morphew, Daniel Shaw, James |
| AuthorAffiliation | University of Birmingham School of Chemistry |
| AuthorAffiliation_xml | – name: University of Birmingham – name: School of Chemistry |
| Author_xml | – sequence: 1 givenname: Daniel surname: Morphew fullname: Morphew, Daniel – sequence: 2 givenname: James surname: Shaw fullname: Shaw, James – sequence: 3 givenname: Christopher surname: Avins fullname: Avins, Christopher – sequence: 4 givenname: Dwaipayan orcidid: 0000-0002-2939-2808 surname: Chakrabarti fullname: Chakrabarti, Dwaipayan email: d.chakrabarti@bham.ac.uk |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29457457$$D View this record in MEDLINE/PubMed |
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