Recycled carbonates in the mantle sources of natural kamafugites; a zinc isotope perspective

Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced experimentally in the presence of CO2. Nevertheless, there is not yet direct evidence for a CO2-rich mantle source and the possible presence of recyc...

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Published inThe American mineralogist Vol. 108; no. 5; pp. 987 - 998
Main Authors Ma Lei, Ma Lei, Liu Shengao, Liu Shengao, Zhao Zhidan, Zhao Zhidan, Yu Xuehui, Yu Xuehui
Format Journal Article
LanguageEnglish
Published Washington Mineralogical Society of America 01.05.2023
Walter de Gruyter GmbH
Subjects
Aluminum oxide
Asia
Carbon dioxide
Carbonates
Cenozoic
chain silicates
China
clinopyroxene
Correlation
diopside
Far East
framework silicates
geochemical cycle
Geochemistry
igneous and metamorphic rocks
igneous rocks
Isotopes
kamafugite
Kamafugites
leucite
magmas
magmatic differentiation
mantle
Melting
Melts
metals
Modelling
nepheline
nepheline group
Orogeny
oxides
Peridotite
perovskite
Petrology
plate tectonics
pyroxene group
Qinling Mountains
recycled carbonates
rich source
Silica
Silicates
Silicon dioxide
stable isotopes
subduction
Tracers
Volcanic rocks
West Qinling
Zinc
Zinc isotopes
Zn isotopes
Zn-66
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Abstract Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced experimentally in the presence of CO2. Nevertheless, there is not yet direct evidence for a CO2-rich mantle source and the possible presence of recycled carbonates in the source of natural kamafugites. Marine carbonates have a heavier zinc isotopic composition (δ66Zn) than that of the mantle by up to 1.0 per mille, making zinc isotopes a sensitive tracer for recycled carbonates in the sources of mantle-derived magmas. Here we take Cenozoic kamafugites from the West Qinling orogen in China as an example to address the origin of this rare volcanic rock. The West Qinling kamafugites are strongly silica-undersaturated (SiO2 = 37.0 to 43.0 wt%) and have significantly higher δ66Zn (0.30 per mille to 0.47 per mille) than that of the normal mantle (0.18±0.05 per mille). No correlation δ66Zn and MgO or SiO2 contents is observed, indicating that δ66Zn was not a result of magmatic differentiation. Modeling of melting indicates that even at extremely low degree (∼0.5%), partial melting of a normal peridotitic source is still unlikely to produce silicate δ66Zn values exceeding 0.30 per mille. Thus, the elevated δ66Zn of the West Qinling kamafugites demonstrates the presence of recycled carbonates in their mantle sources. Binary-mixing modeling suggests that the source contains ∼5 to 15% recycled carbonates, which is supported by the positive correlation between 2D66Zn and CaO/Al2O3. Overall, the West Qinling kamafugites represent the products of low-degree partial melting of a recycled carbonate-bearing peridotite source, which provides evidence for an important role of recycled carbonates in the origin of natural kamafugite suites.
AbstractList Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced experimentally in the presence of CO . Nevertheless, there is not yet direct evidence for a CO -rich mantle source and the possible presence of recycled carbonates in the source of natural kamafugites. Marine carbonates have a heavier zinc isotopic composition (δ Zn) than that of the mantle by up to 1.0‰, making zinc isotopes a sensitive tracer for recycled carbonates in the sources of mantle-derived magmas. Here we take Cenozoic kamafugites from the West Qinling orogen in China as an example to address the origin of this rare volcanic rock. The West Qinling kamafugites are strongly silica-undersaturated (SiO = 37.0 to 43.0 wt%) and have significantly higher δ Zn (0.30‰ to 0.47‰) than that of the normal mantle (0.18 ± 0.05‰). No correlation between δ Zn and MgO or SiO contents is observed, indicating that the high δ Zn was not a result of magmatic differentiation. Modeling of melting indicates that even at extremely low degree (~0.5%), partial melting of a normal peridotitic source is still unlikely to produce silicate melts with δ Zn values exceeding 0.30‰. Thus, the elevated δ Zn of the West Qinling kamafugites demonstrates the presence of recycled carbonates in their mantle sources. Binary-mixing modeling suggests that the source contains ~5 to 15% recycled carbonates, which is supported by the positive correlation between δ Zn and CaO/Al . Overall, the West Qinling kamafugites represent the products of low-degree partial melting of a recycled carbonate-bearing peridotite source, which provides evidence for an important role of recycled carbonates in the origin of natural kamafugite suites.
Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced experimentally in the presence of CO2. Nevertheless, there is not yet direct evidence for a CO2-rich mantle source and the possible presence of recycled carbonates in the source of natural kamafugites. Marine carbonates have a heavier zinc isotopic composition (δ66Zn) than that of the mantle by up to 1.0 per mille, making zinc isotopes a sensitive tracer for recycled carbonates in the sources of mantle-derived magmas. Here we take Cenozoic kamafugites from the West Qinling orogen in China as an example to address the origin of this rare volcanic rock. The West Qinling kamafugites are strongly silica-undersaturated (SiO2 = 37.0 to 43.0 wt%) and have significantly higher δ66Zn (0.30 per mille to 0.47 per mille) than that of the normal mantle (0.18±0.05 per mille). No correlation δ66Zn and MgO or SiO2 contents is observed, indicating that δ66Zn was not a result of magmatic differentiation. Modeling of melting indicates that even at extremely low degree (∼0.5%), partial melting of a normal peridotitic source is still unlikely to produce silicate δ66Zn values exceeding 0.30 per mille. Thus, the elevated δ66Zn of the West Qinling kamafugites demonstrates the presence of recycled carbonates in their mantle sources. Binary-mixing modeling suggests that the source contains ∼5 to 15% recycled carbonates, which is supported by the positive correlation between 2D66Zn and CaO/Al2O3. Overall, the West Qinling kamafugites represent the products of low-degree partial melting of a recycled carbonate-bearing peridotite source, which provides evidence for an important role of recycled carbonates in the origin of natural kamafugite suites.
Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced experimentally in the presence of CO2. Nevertheless, there is not yet direct evidence for a CO2-rich mantle source and the possible presence of recycled carbonates in the source of natural kamafugites. Marine carbonates have a heavier zinc isotopic composition (δ66Zn) than that of the mantle by up to 1.0‰, making zinc isotopes a sensitive tracer for recycled carbonates in the sources of mantle-derived magmas. Here we take Cenozoic kamafugites from the West Qinling orogen in China as an example to address the origin of this rare volcanic rock. The West Qinling kamafugites are strongly silica-undersaturated (SiO2 = 37.0 to 43.0 wt%) and have significantly higher δ66Zn (0.30‰ to 0.47‰) than that of the normal mantle (0.18 ± 0.05‰). No correlation between δ66Zn and MgO or SiO2 contents is observed, indicating that the high δ66Zn was not a result of magmatic differentiation. Modeling of melting indicates that even at extremely low degree (~0.5%), partial melting of a normal peridotitic source is still unlikely to produce silicate melts with δ66Zn values exceeding 0.30‰. Thus, the elevated δ66Zn of the West Qinling kamafugites demonstrates the presence of recycled carbonates in their mantle sources. Binary-mixing modeling suggests that the source contains ~5 to 15% recycled carbonates, which is supported by the positive correlation between δ66Zn and CaO/Al2O3. Overall, the West Qinling kamafugites represent the products of low-degree partial melting of a recycled carbonate-bearing peridotite source, which provides evidence for an important role of recycled carbonates in the origin of natural kamafugite suites.
Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced experimentally in the presence of CO2. Nevertheless, there is not yet direct evidence for a CO2-rich mantle source and the possible presence of recycled carbonates in the source of natural kamafugites. Marine carbonates have a heavier zinc isotopic composition (δ66Zn) than that of the mantle by up to 1.0‰, making zinc isotopes a sensitive tracer for recycled carbonates in the sources of mantle-derived magmas. Here we take Cenozoic kamafugites from the West Qinling orogen in China as an example to address the origin of this rare volcanic rock. The West Qinling kamafugites are strongly silica-undersaturated (SiO2 = 37.0 to 43.0 wt%) and have significantly higher δ66Zn (0.30‰ to 0.47‰) than that of the normal mantle (0.18 ± 0.05‰). No correlation between δ66Zn and MgO or SiO2 contents is observed, indicating that the high δ66Zn was not a result of magmatic differentiation. Modeling of melting indicates that even at extremely low degree (~0.5%), partial melting of a normal peridotitic source is still unlikely to produce silicate melts with δ 66Zn values exceeding 0.30‰. Thus, the elevated δ66Zn of the West Qinling kamafugites demonstrates the presence of recycled carbonates in their mantle sources. Binary-mixing modeling suggests that the source contains ~5 to 15% recycled carbonates, which is supported by the positive correlation between δ66Zn and CaO/Al2O3. Overall, the West Qinling kamafugites represent the products of low-degree partial melting of a recycled carbonate-bearing peridotite source, which provides evidence for an important role of recycled carbonates in the origin of natural kamafugite suites.
Author Ma Lei, Ma Lei
Liu Shengao, Liu Shengao
Zhao Zhidan, Zhao Zhidan
Yu Xuehui, Yu Xuehui
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Snippet Kamafugites are strongly silica-undersaturated melts that are difficult to produce by partial melting of volatile-free peridotites but can be produced...
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SubjectTerms Aluminum oxide
Asia
Carbon dioxide
Carbonates
Cenozoic
chain silicates
China
clinopyroxene
Correlation
diopside
Far East
framework silicates
geochemical cycle
Geochemistry
igneous and metamorphic rocks
igneous rocks
Isotopes
kamafugite
Kamafugites
leucite
magmas
magmatic differentiation
mantle
Melting
Melts
metals
Modelling
nepheline
nepheline group
Orogeny
oxides
Peridotite
perovskite
Petrology
plate tectonics
pyroxene group
Qinling Mountains
recycled carbonates
rich source
Silica
Silicates
Silicon dioxide
stable isotopes
subduction
Tracers
Volcanic rocks
West Qinling
Zinc
Zinc isotopes
Zn isotopes
Zn-66
Title Recycled carbonates in the mantle sources of natural kamafugites; a zinc isotope perspective
URI https://pubs.geoscienceworld.org/ammin/article/108/5/987/622882/Recycled-carbonates-in-the-mantle-sources-of
https://www.degruyter.com/doi/10.2138/am-2022-8382
https://www.proquest.com/docview/2811137231
Volume 108
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