Orientation of Thiophenol Adsorbed on Silver Determined by Nonlinear Vibrational Spectroscopy of the Carbon Skeleton

The orientation of thiophenol adsorbed on silver is determined by comparing ab initio calculated and experimental sum-frequency generation (SFG) spectra measured between 9 and 20 μm using a tandem KTP/CdSe optical parametric oscillator. The molecule S−C bond is tilted ∼37° from the surface normal wi...

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Published inThe journal of physical chemistry. B Vol. 108; no. 41; pp. 16135 - 16138
Main Authors Mani, A. A, Schultz, Z. D, Caudano, Y, Champagne, B, Humbert, C, Dreesen, L, Gewirth, A. A, White, J. O, Thiry, P. A, Peremans, A
Format Journal Article Web Resource
LanguageEnglish
Published American Chemical Society 14.10.2004
Subjects
Chemical Physics
Condensed Matter
Materials Science
Optics
Physical, chemical, mathematical & earth Sciences
Physics
Physique
Physique, chimie, mathématiques & sciences de la terre
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Abstract The orientation of thiophenol adsorbed on silver is determined by comparing ab initio calculated and experimental sum-frequency generation (SFG) spectra measured between 9 and 20 μm using a tandem KTP/CdSe optical parametric oscillator. The molecule S−C bond is tilted ∼37° from the surface normal with the aromatic ring plane perpendicular to the surface.
AbstractList The orientation of thiophenol adsorbed on silver is determined by comparing ab initio calculated and experimental sum-frequency generation (SFG) spectra measured between 9 and 20 μm using a tandem KTP/CdSe optical parametric oscillator. The molecule S−C bond is tilted ∼37° from the surface normal with the aromatic ring plane perpendicular to the surface.
The orientation of thiophenol adsorbed on silver is determined by comparing ab initio calculated and experimental sum-frequency generation (SFG) spectra measured between 9 and 20 µm using a tandem KTP/CdSe optical parametric oscillator. The molecule S-C bond is tilted ~37° from the surface normal with the aromatic ring plane perpendicular to the surface.
Author Gewirth, A. A
Caudano, Y
White, J. O
Thiry, P. A
Schultz, Z. D
Mani, A. A
Humbert, C
Dreesen, L
Peremans, A
Champagne, B
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Snippet The orientation of thiophenol adsorbed on silver is determined by comparing ab initio calculated and experimental sum-frequency generation (SFG) spectra...
The orientation of thiophenol adsorbed on silver is determined by comparing ab initio calculated and experimental sum-frequency generation (SFG) spectra...
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SubjectTerms Chemical Physics
Condensed Matter
Materials Science
Optics
Physical, chemical, mathematical & earth Sciences
Physics
Physique
Physique, chimie, mathématiques & sciences de la terre
Title Orientation of Thiophenol Adsorbed on Silver Determined by Nonlinear Vibrational Spectroscopy of the Carbon Skeleton
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