Perspective on High-Rate Alkaline Water Splitting

Alkaline water splitting (AWS) represents a sustainable technology for hydrogen gas generation. In comparison to proton exchange membrane water splitting, AWS is an economical approach because non-platinum-group metal-based materials can be used as catalysts and it avoids the usage of expensive prot...

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Published inACS materials letters Vol. 3; no. 2; pp. 224 - 234
Main Authors Kou, Tianyi, Wang, Shanwen, Li, Yat
Format Journal Article
LanguageEnglish
Published American Chemical Society 01.02.2021
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Abstract Alkaline water splitting (AWS) represents a sustainable technology for hydrogen gas generation. In comparison to proton exchange membrane water splitting, AWS is an economical approach because non-platinum-group metal-based materials can be used as catalysts and it avoids the usage of expensive proton exchange membranes. Despite the rapid development of cost-effective and intrinsically active catalysts that showed record-breaking performances at low current density (tens of mA cm–2), the cell efficiency of AWS at large current density (>400 mA cm–2) is still limited. In this Perspective, we aim to share our thoughts on the design of hydrogen evolution and oxygen evolution catalysts for high-rate AWS, the possible problems in catalyst’s performance evaluation, and the stability issues of catalysts.
AbstractList Alkaline water splitting (AWS) represents a sustainable technology for hydrogen gas generation. In comparison to proton exchange membrane water splitting, AWS is an economical approach because non-platinum-group metal-based materials can be used as catalysts and it avoids the usage of expensive proton exchange membranes. Despite the rapid development of cost-effective and intrinsically active catalysts that showed record-breaking performances at low current density (tens of mA cm–2), the cell efficiency of AWS at large current density (>400 mA cm–2) is still limited. In this Perspective, we aim to share our thoughts on the design of hydrogen evolution and oxygen evolution catalysts for high-rate AWS, the possible problems in catalyst’s performance evaluation, and the stability issues of catalysts.
Author Kou, Tianyi
Li, Yat
Wang, Shanwen
AuthorAffiliation Department of Chemistry and Biochemistry
AuthorAffiliation_xml – name: Department of Chemistry and Biochemistry
Author_xml – sequence: 1
  givenname: Tianyi
  orcidid: 0000-0002-1563-7819
  surname: Kou
  fullname: Kou, Tianyi
– sequence: 2
  givenname: Shanwen
  surname: Wang
  fullname: Wang, Shanwen
– sequence: 3
  givenname: Yat
  orcidid: 0000-0002-8058-2084
  surname: Li
  fullname: Li, Yat
  email: yatli@ucsc.edu
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Snippet Alkaline water splitting (AWS) represents a sustainable technology for hydrogen gas generation. In comparison to proton exchange membrane water splitting, AWS...
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Title Perspective on High-Rate Alkaline Water Splitting
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