Origin and spatial distribution of heavy metals and carcinogenic risk assessment in mining areas at You'xi County southeast China
An extensive study on the spatial distribution and source apportionment of heavy metals in soils and so by risk assessment at You'xi County, a major Pb–Zn mining area southeast China, was conducted in this contribution. A total of 93 soil samples were examined with the concentration of heavy me...
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| Published in | Geoderma Vol. 310; pp. 99 - 106 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
15.01.2018
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| Abstract | An extensive study on the spatial distribution and source apportionment of heavy metals in soils and so by risk assessment at You'xi County, a major Pb–Zn mining area southeast China, was conducted in this contribution. A total of 93 soil samples were examined with the concentration of heavy metals (As, Cd, Cr, Cu, Hg, Pb, and Zn), pH, and soil organic matter (SOM) contents by using geostatistical approaches combined with geographic information system (GIS) analysis. The mean values of heavy metals were determined to be 7.9±5.8, 12.8±14.1, 80.4±42.0, 34.4±45.0, 0.12±0.13 368.5±873.6, and 369.6±505.5mgkg−1 (mean±SD) for As, Cd, Cr, Cu, Hg, Pb, and Zn, respectively. Contents of all heavy metals present in the study area were considerably higher than their background values of provincial and national standards except for As. A principle component analysis revealed the main origin of heavy metals: soil parent materials for Cu, Pb, and Zn; atmospheric deposition during mining processes for Cr, and Hg; and human farming activities for Cd. Carcinogenic risk was assessed with an average value of 69.3×10−6mgkg−1, suggesting an average of 69 individuals per million people being predisposed to cancer. Meanwhile, the identification of heavy metal sources in agricultural soils might be beneficial to local soil protection and soil quality improvement.
•Spatial distribution of heavy metals in the study area has been investigated.•GIS mapping and correlation interpretation have been analyzed.•Carcinogenic risk assessment has been revealed in the study area. |
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| AbstractList | An extensive study on the spatial distribution and source apportionment of heavy metals in soils and so by risk assessment at You'xi County, a major Pb–Zn mining area southeast China, was conducted in this contribution. A total of 93 soil samples were examined with the concentration of heavy metals (As, Cd, Cr, Cu, Hg, Pb, and Zn), pH, and soil organic matter (SOM) contents by using geostatistical approaches combined with geographic information system (GIS) analysis. The mean values of heavy metals were determined to be 7.9±5.8, 12.8±14.1, 80.4±42.0, 34.4±45.0, 0.12±0.13 368.5±873.6, and 369.6±505.5mgkg−1 (mean±SD) for As, Cd, Cr, Cu, Hg, Pb, and Zn, respectively. Contents of all heavy metals present in the study area were considerably higher than their background values of provincial and national standards except for As. A principle component analysis revealed the main origin of heavy metals: soil parent materials for Cu, Pb, and Zn; atmospheric deposition during mining processes for Cr, and Hg; and human farming activities for Cd. Carcinogenic risk was assessed with an average value of 69.3×10−6mgkg−1, suggesting an average of 69 individuals per million people being predisposed to cancer. Meanwhile, the identification of heavy metal sources in agricultural soils might be beneficial to local soil protection and soil quality improvement.
•Spatial distribution of heavy metals in the study area has been investigated.•GIS mapping and correlation interpretation have been analyzed.•Carcinogenic risk assessment has been revealed in the study area. An extensive study on the spatial distribution and source apportionment of heavy metals in soils and so by risk assessment at You'xi County, a major Pb–Zn mining area southeast China, was conducted in this contribution. A total of 93 soil samples were examined with the concentration of heavy metals (As, Cd, Cr, Cu, Hg, Pb, and Zn), pH, and soil organic matter (SOM) contents by using geostatistical approaches combined with geographic information system (GIS) analysis. The mean values of heavy metals were determined to be 7.9±5.8, 12.8±14.1, 80.4±42.0, 34.4±45.0, 0.12±0.13 368.5±873.6, and 369.6±505.5mgkg⁻¹ (mean±SD) for As, Cd, Cr, Cu, Hg, Pb, and Zn, respectively. Contents of all heavy metals present in the study area were considerably higher than their background values of provincial and national standards except for As. A principle component analysis revealed the main origin of heavy metals: soil parent materials for Cu, Pb, and Zn; atmospheric deposition during mining processes for Cr, and Hg; and human farming activities for Cd. Carcinogenic risk was assessed with an average value of 69.3×10⁻⁶mgkg⁻¹, suggesting an average of 69 individuals per million people being predisposed to cancer. Meanwhile, the identification of heavy metal sources in agricultural soils might be beneficial to local soil protection and soil quality improvement. |
| Author | Qiu, Hai-Yuan Chen, Ben Jiao, Wen-Bin Kang, Bin Lü, Jian Huang, Xiao-Xia |
| Author_xml | – sequence: 1 givenname: Jian surname: Lü fullname: Lü, Jian email: jian_lu_fafu@163.com organization: Fujian Provincial Key Laboratory of Soil Environmental Health and Regulation, College of Resources and Environment, Fujian Agriculture and Forestry University, Fuzhou 350002, China – sequence: 2 givenname: Wen-Bin surname: Jiao fullname: Jiao, Wen-Bin organization: Fujian Provincial Key Laboratory of Soil Environmental Health and Regulation, College of Resources and Environment, Fujian Agriculture and Forestry University, Fuzhou 350002, China – sequence: 3 givenname: Hai-Yuan surname: Qiu fullname: Qiu, Hai-Yuan organization: Fujian Monitoring Center of Geological Environment, Fuzhou 350001, China – sequence: 4 givenname: Ben surname: Chen fullname: Chen, Ben organization: College of Oceanography and Environmental Science, Xiamen University, Xiamen 361005, China – sequence: 5 givenname: Xiao-Xia surname: Huang fullname: Huang, Xiao-Xia organization: School of Resource Environment and Earth Science, Yunnan University, Kunming 650091, China – sequence: 6 givenname: Bin surname: Kang fullname: Kang, Bin organization: Fisheries College, Jimei University, Xiamen 361021, China |
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| SubjectTerms | agricultural soils arsenic atmospheric deposition cadmium Carcinogenic risk China chromium copper geographic information systems geostatistics Heavy metal pollution heavy metals humans lead mercury mining neoplasms Pb–Zn mine risk assessment soil organic matter soil parent materials Soil quality soil sampling zinc |
| Title | Origin and spatial distribution of heavy metals and carcinogenic risk assessment in mining areas at You'xi County southeast China |
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