Silver Nitrate Impregnated Pellet-Type Adsorbents for Propylene/Propane Separation

Adsorptive separation of propylene from propane using adsorption has attracted much attention due to its energy efficiency compared to distillation. We prepared propylene-selective adsorbents suitable for pressure swing adsorption (PSA) separation by impregnating AgNO3 on high-surface-area pellets s...

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Published inIndustrial & engineering chemistry research Vol. 45; no. 26; pp. 9129 - 9135
Main Authors Ko, Chang Hyun, Han, Sang-Sup, Park, Jong-Ho, Cho, Soon-Haeng, Kim, Jong-Nam
Format Journal Article
LanguageEnglish
Published Washington, DC American Chemical Society 20.12.2006
Subjects
Applied sciences
Chemical engineering
Exact sciences and technology
Pellet
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Abstract Adsorptive separation of propylene from propane using adsorption has attracted much attention due to its energy efficiency compared to distillation. We prepared propylene-selective adsorbents suitable for pressure swing adsorption (PSA) separation by impregnating AgNO3 on high-surface-area pellets such as silica, clay, and aluminosilica as substrates. Considering adsorption capacity, selectivity, desorption rate, and pellet crush strength before and after impregnation, AgNO3/aluminosilica was the most suitable adsorbent among the three adsorbents. A large portion of the AgNO3 was located inside micropores in the aluminosilica after impregnation. The propylene adsorption capacity of AgNO3/aluminosilica was 2.3 mmol/g, and the selectivity of propylene over propane was 3.1 at 298 K and 3 kgf/cm2. However, the adsorption capacity of AgNO3/aluminosilica for propylene decreased by exposing the adsorbent to hydrogen.
AbstractList Adsorptive separation of propylene from propane using adsorption has attracted much attention due to its energy efficiency compared to distillation. We prepared propylene-selective adsorbents suitable for pressure swing adsorption (PSA) separation by impregnating AgNO3 on high-surface-area pellets such as silica, clay, and aluminosilica as substrates. Considering adsorption capacity, selectivity, desorption rate, and pellet crush strength before and after impregnation, AgNO3/aluminosilica was the most suitable adsorbent among the three adsorbents. A large portion of the AgNO3 was located inside micropores in the aluminosilica after impregnation. The propylene adsorption capacity of AgNO3/aluminosilica was 2.3 mmol/g, and the selectivity of propylene over propane was 3.1 at 298 K and 3 kgf/cm2. However, the adsorption capacity of AgNO3/aluminosilica for propylene decreased by exposing the adsorbent to hydrogen.
Author Park, Jong-Ho
Kim, Jong-Nam
Ko, Chang Hyun
Han, Sang-Sup
Cho, Soon-Haeng
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Snippet Adsorptive separation of propylene from propane using adsorption has attracted much attention due to its energy efficiency compared to distillation. We...
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Title Silver Nitrate Impregnated Pellet-Type Adsorbents for Propylene/Propane Separation
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