Engineering Spiny PtFePd@PtFe/Pt Core@Multishell Nanowires with Enhanced Performance for Alcohol Electrooxidation
Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D na...
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| Published in | ACS applied materials & interfaces Vol. 11; no. 34; pp. 30880 - 30886 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
28.08.2019
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| Abstract | Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D nanomaterials is still a worthy subject. By creatively introducing a trimetallic nanoalloy, core@multishell structure, and 1D nanowire (NW) morphology, we have constructed a kind of novel spiny PtFePd@PtFe/Pt core@multishell 1D NW catalysts with PtFePd as the core and PtFe/Pt as the multishell on the basis of improving catalytic property. The composition-optimized Pt5FePd2 1D NWs display remarkable catalytic properties for ethanol oxidation reaction and methanol oxidation reaction, in which mass activities are 4.965 and 4.038 A mg–1, 4.6 and 5.0 and 4.0 and 9.2-fold higher than Pt/C and Pd/C catalysts. Furthermore, the obtained Pt5FePd2 NWs can also retain favorable stability after durability tests. The unique core@multishell structure, spiny 1D NWs with many steps and kinks, and interior electronic and synergistic effect all contribute to the advanced catalytic performance. The present work has rationally designed the novel 1D PtFePd@PtFe/Pt core@multishell NW catalysts and offered a meaningful guideline for the designing of high-performance electrocatalysts. |
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| AbstractList | Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D nanomaterials is still a worthy subject. By creatively introducing a trimetallic nanoalloy, core@multishell structure, and 1D nanowire (NW) morphology, we have constructed a kind of novel spiny PtFePd@PtFe/Pt core@multishell 1D NW catalysts with PtFePd as the core and PtFe/Pt as the multishell on the basis of improving catalytic property. The composition-optimized Pt5FePd2 1D NWs display remarkable catalytic properties for ethanol oxidation reaction and methanol oxidation reaction, in which mass activities are 4.965 and 4.038 A mg–1, 4.6 and 5.0 and 4.0 and 9.2-fold higher than Pt/C and Pd/C catalysts. Furthermore, the obtained Pt5FePd2 NWs can also retain favorable stability after durability tests. The unique core@multishell structure, spiny 1D NWs with many steps and kinks, and interior electronic and synergistic effect all contribute to the advanced catalytic performance. The present work has rationally designed the novel 1D PtFePd@PtFe/Pt core@multishell NW catalysts and offered a meaningful guideline for the designing of high-performance electrocatalysts. Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D nanomaterials is still a worthy subject. By creatively introducing a trimetallic nanoalloy, core@multishell structure, and 1D nanowire (NW) morphology, we have constructed a kind of novel spiny PtFePd@PtFe/Pt core@multishell 1D NW catalysts with PtFePd as the core and PtFe/Pt as the multishell on the basis of improving catalytic property. The composition-optimized Pt₅FePd₂ 1D NWs display remarkable catalytic properties for ethanol oxidation reaction and methanol oxidation reaction, in which mass activities are 4.965 and 4.038 A mg–¹, 4.6 and 5.0 and 4.0 and 9.2-fold higher than Pt/C and Pd/C catalysts. Furthermore, the obtained Pt₅FePd₂ NWs can also retain favorable stability after durability tests. The unique core@multishell structure, spiny 1D NWs with many steps and kinks, and interior electronic and synergistic effect all contribute to the advanced catalytic performance. The present work has rationally designed the novel 1D PtFePd@PtFe/Pt core@multishell NW catalysts and offered a meaningful guideline for the designing of high-performance electrocatalysts. Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D nanomaterials is still a worthy subject. By creatively introducing a trimetallic nanoalloy, core@multishell structure, and 1D nanowire (NW) morphology, we have constructed a kind of novel spiny PtFePd@PtFe/Pt core@multishell 1D NW catalysts with PtFePd as the core and PtFe/Pt as the multishell on the basis of improving catalytic property. The composition-optimized Pt5FePd2 1D NWs display remarkable catalytic properties for ethanol oxidation reaction and methanol oxidation reaction, in which mass activities are 4.965 and 4.038 A mg-1, 4.6 and 5.0 and 4.0 and 9.2-fold higher than Pt/C and Pd/C catalysts. Furthermore, the obtained Pt5FePd2 NWs can also retain favorable stability after durability tests. The unique core@multishell structure, spiny 1D NWs with many steps and kinks, and interior electronic and synergistic effect all contribute to the advanced catalytic performance. The present work has rationally designed the novel 1D PtFePd@PtFe/Pt core@multishell NW catalysts and offered a meaningful guideline for the designing of high-performance electrocatalysts.Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D nanomaterials is still a worthy subject. By creatively introducing a trimetallic nanoalloy, core@multishell structure, and 1D nanowire (NW) morphology, we have constructed a kind of novel spiny PtFePd@PtFe/Pt core@multishell 1D NW catalysts with PtFePd as the core and PtFe/Pt as the multishell on the basis of improving catalytic property. The composition-optimized Pt5FePd2 1D NWs display remarkable catalytic properties for ethanol oxidation reaction and methanol oxidation reaction, in which mass activities are 4.965 and 4.038 A mg-1, 4.6 and 5.0 and 4.0 and 9.2-fold higher than Pt/C and Pd/C catalysts. Furthermore, the obtained Pt5FePd2 NWs can also retain favorable stability after durability tests. The unique core@multishell structure, spiny 1D NWs with many steps and kinks, and interior electronic and synergistic effect all contribute to the advanced catalytic performance. The present work has rationally designed the novel 1D PtFePd@PtFe/Pt core@multishell NW catalysts and offered a meaningful guideline for the designing of high-performance electrocatalysts. Engineering robust electrocatalysts is always a key point in direct alcohol fuel cells. Catalysts with a one-dimension (1D) structure are well studied and considered as promising candidates among various catalysts in the past decades; however, the precise regulation on the surface structure of 1D nanomaterials is still a worthy subject. By creatively introducing a trimetallic nanoalloy, core@multishell structure, and 1D nanowire (NW) morphology, we have constructed a kind of novel spiny PtFePd@PtFe/Pt core@multishell 1D NW catalysts with PtFePd as the core and PtFe/Pt as the multishell on the basis of improving catalytic property. The composition-optimized Pt FePd 1D NWs display remarkable catalytic properties for ethanol oxidation reaction and methanol oxidation reaction, in which mass activities are 4.965 and 4.038 A mg , 4.6 and 5.0 and 4.0 and 9.2-fold higher than Pt/C and Pd/C catalysts. Furthermore, the obtained Pt FePd NWs can also retain favorable stability after durability tests. The unique core@multishell structure, spiny 1D NWs with many steps and kinks, and interior electronic and synergistic effect all contribute to the advanced catalytic performance. The present work has rationally designed the novel 1D PtFePd@PtFe/Pt core@multishell NW catalysts and offered a meaningful guideline for the designing of high-performance electrocatalysts. |
| Author | Zhang, Yangping Shiraishi, Yukihide Du, Yukou Gao, Fei Wang, Caiqin |
| AuthorAffiliation | Tokyo University of Science Yamaguchi Nanjing Forestry University College of Science College of Chemistry, Chemical Engineering and Materials Science |
| AuthorAffiliation_xml | – name: Tokyo University of Science Yamaguchi – name: College of Chemistry, Chemical Engineering and Materials Science – name: College of Science – name: Nanjing Forestry University |
| Author_xml | – sequence: 1 givenname: Yangping surname: Zhang fullname: Zhang, Yangping organization: College of Chemistry, Chemical Engineering and Materials Science – sequence: 2 givenname: Fei surname: Gao fullname: Gao, Fei organization: College of Chemistry, Chemical Engineering and Materials Science – sequence: 3 givenname: Caiqin surname: Wang fullname: Wang, Caiqin email: wangcaiqin@njfu.edu.cn organization: Nanjing Forestry University – sequence: 4 givenname: Yukihide surname: Shiraishi fullname: Shiraishi, Yukihide organization: Tokyo University of Science Yamaguchi – sequence: 5 givenname: Yukou orcidid: 0000-0002-9161-1821 surname: Du fullname: Du, Yukou email: duyk@suda.edu.cn organization: College of Chemistry, Chemical Engineering and Materials Science |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31368299$$D View this record in MEDLINE/PubMed |
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| Keywords | direct alcohol fuel cells 1D nanowires core@multishell ethanol oxidation reaction methanol oxidation reaction |
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| SubjectTerms | catalysts catalytic activity durability engineering ethanol fuel cells guidelines methanol nanowires oxidation palladium platinum synergism |
| Title | Engineering Spiny PtFePd@PtFe/Pt Core@Multishell Nanowires with Enhanced Performance for Alcohol Electrooxidation |
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