A Self-Detecting and Self-Cleaning Biomimetic Porous Metal-Based Hydrogel for Oil/Water Separation

Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a po...

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Published inACS applied materials & interfaces Vol. 14; no. 22; pp. 26057 - 26067
Main Authors Li, Zhaoxin, Sang, Shengtian, Jiang, Shuyue, Chen, Liang, Zhang, Haifeng
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 08.06.2022
Subjects
Applications of Polymer, Composite, and Coating Materials
biomimetics
carbon nanotubes
crosslinking
foams
hydrogels
hydrophilicity
oils
pollution
polyvinyl alcohol
skeleton
tannins
wood
self-detection
hydrogel coating
self-cleaning
oil/water separation
super-wetting surface
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Abstract Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a porous metal-based hydrogel is proposed, inspired by the porous structure of wood. Porous copper foam with nano-Cu­(OH)2 is used as the skeleton, and its surface is coated with a polyvinyl alcohol, tannic acid, and multiwalled carbon nanotube cross-linked hydrogel coating. The hydrogel has superhydrophilicity and excellent oil/water separation efficiency (>99%) and can adapt to various environments. This approach can also realize hydrogel pollution degree self-detection according to the change in the electrical signal generated during the oil/water separation process, and the hydrogel can also be recovered by soaking to realize self-cleaning. This study will provide new insights into the application of oil/water separation materials in practical industrial manufacturing.
AbstractList Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a porous metal-based hydrogel is proposed, inspired by the porous structure of wood. Porous copper foam with nano-Cu(OH) is used as the skeleton, and its surface is coated with a polyvinyl alcohol, tannic acid, and multiwalled carbon nanotube cross-linked hydrogel coating. The hydrogel has superhydrophilicity and excellent oil/water separation efficiency (>99%) and can adapt to various environments. This approach can also realize hydrogel pollution degree self-detection according to the change in the electrical signal generated during the oil/water separation process, and the hydrogel can also be recovered by soaking to realize self-cleaning. This study will provide new insights into the application of oil/water separation materials in practical industrial manufacturing.
Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a porous metal-based hydrogel is proposed, inspired by the porous structure of wood. Porous copper foam with nano-Cu(OH)₂ is used as the skeleton, and its surface is coated with a polyvinyl alcohol, tannic acid, and multiwalled carbon nanotube cross-linked hydrogel coating. The hydrogel has superhydrophilicity and excellent oil/water separation efficiency (>99%) and can adapt to various environments. This approach can also realize hydrogel pollution degree self-detection according to the change in the electrical signal generated during the oil/water separation process, and the hydrogel can also be recovered by soaking to realize self-cleaning. This study will provide new insights into the application of oil/water separation materials in practical industrial manufacturing.
Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a porous metal-based hydrogel is proposed, inspired by the porous structure of wood. Porous copper foam with nano-Cu(OH)2 is used as the skeleton, and its surface is coated with a polyvinyl alcohol, tannic acid, and multiwalled carbon nanotube cross-linked hydrogel coating. The hydrogel has superhydrophilicity and excellent oil/water separation efficiency (>99%) and can adapt to various environments. This approach can also realize hydrogel pollution degree self-detection according to the change in the electrical signal generated during the oil/water separation process, and the hydrogel can also be recovered by soaking to realize self-cleaning. This study will provide new insights into the application of oil/water separation materials in practical industrial manufacturing.Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a porous metal-based hydrogel is proposed, inspired by the porous structure of wood. Porous copper foam with nano-Cu(OH)2 is used as the skeleton, and its surface is coated with a polyvinyl alcohol, tannic acid, and multiwalled carbon nanotube cross-linked hydrogel coating. The hydrogel has superhydrophilicity and excellent oil/water separation efficiency (>99%) and can adapt to various environments. This approach can also realize hydrogel pollution degree self-detection according to the change in the electrical signal generated during the oil/water separation process, and the hydrogel can also be recovered by soaking to realize self-cleaning. This study will provide new insights into the application of oil/water separation materials in practical industrial manufacturing.
Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to monitor the pollution degree and self-cleaning during the separation process limits their application in industrial production. In this study, a porous metal-based hydrogel is proposed, inspired by the porous structure of wood. Porous copper foam with nano-Cu­(OH)2 is used as the skeleton, and its surface is coated with a polyvinyl alcohol, tannic acid, and multiwalled carbon nanotube cross-linked hydrogel coating. The hydrogel has superhydrophilicity and excellent oil/water separation efficiency (>99%) and can adapt to various environments. This approach can also realize hydrogel pollution degree self-detection according to the change in the electrical signal generated during the oil/water separation process, and the hydrogel can also be recovered by soaking to realize self-cleaning. This study will provide new insights into the application of oil/water separation materials in practical industrial manufacturing.
Author Li, Zhaoxin
Jiang, Shuyue
Zhang, Haifeng
Chen, Liang
Sang, Shengtian
AuthorAffiliation MEMS Center
Ministry of Education
Key Laboratory of Micro-Systems and Micro-Structures Manufacturing
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hydrogel coating
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oil/water separation
super-wetting surface
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Snippet Porous materials with super-wetting surfaces (superhydrophilic/underwater superoleophobic) are ideal for oil/water separation. However, the inability to...
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SubjectTerms Applications of Polymer, Composite, and Coating Materials
biomimetics
carbon nanotubes
crosslinking
foams
hydrogels
hydrophilicity
oils
pollution
polyvinyl alcohol
skeleton
tannins
wood
Title A Self-Detecting and Self-Cleaning Biomimetic Porous Metal-Based Hydrogel for Oil/Water Separation
URI http://dx.doi.org/10.1021/acsami.2c05327
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