Functional Porous Organic Polymers with Conjugated Triaryl Triazine as the Core for Superfast Adsorption Removal of Organic Dyes
Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of...
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| Published in | ACS applied materials & interfaces Vol. 13; no. 5; pp. 6359 - 6366 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
10.02.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of porous organic polymer (POP) adsorbents. These planar monomers with multiple phenolic hydroxyl groups facilitated the formation of aza-linked polymers with hierarchical porous structures, sheet-like morphology, good surface wettability, and high degree of functionality. Such structural characteristics of the CTT-POP adsorbents provided superfast adsorption of various cationic dyes from water. For the adsorption of methylene blue dye, the pseudo-second-order rate constant of CTT-POP-1 is 12.9 g mg–1 min–1, superior to those reported in the existing literature. In addition, CTT-POP-1 can be regenerated at least seven times with no loss in performance, indicating its potential application in water treatment. |
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| AbstractList | Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of porous organic polymer (POP) adsorbents. These planar monomers with multiple phenolic hydroxyl groups facilitated the formation of aza-linked polymers with hierarchical porous structures, sheet-like morphology, good surface wettability, and high degree of functionality. Such structural characteristics of the CTT-POP adsorbents provided superfast adsorption of various cationic dyes from water. For the adsorption of methylene blue dye, the pseudo-second-order rate constant of CTT-POP-1 is 12.9 g mg
min
, superior to those reported in the existing literature. In addition, CTT-POP-1 can be regenerated at least seven times with no loss in performance, indicating its potential application in water treatment. Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of porous organic polymer (POP) adsorbents. These planar monomers with multiple phenolic hydroxyl groups facilitated the formation of aza-linked polymers with hierarchical porous structures, sheet-like morphology, good surface wettability, and high degree of functionality. Such structural characteristics of the CTT-POP adsorbents provided superfast adsorption of various cationic dyes from water. For the adsorption of methylene blue dye, the pseudo-second-order rate constant of CTT-POP-1 is 12.9 g mg–¹ min–¹, superior to those reported in the existing literature. In addition, CTT-POP-1 can be regenerated at least seven times with no loss in performance, indicating its potential application in water treatment. Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of porous organic polymer (POP) adsorbents. These planar monomers with multiple phenolic hydroxyl groups facilitated the formation of aza-linked polymers with hierarchical porous structures, sheet-like morphology, good surface wettability, and high degree of functionality. Such structural characteristics of the CTT-POP adsorbents provided superfast adsorption of various cationic dyes from water. For the adsorption of methylene blue dye, the pseudo-second-order rate constant of CTT-POP-1 is 12.9 g mg–1 min–1, superior to those reported in the existing literature. In addition, CTT-POP-1 can be regenerated at least seven times with no loss in performance, indicating its potential application in water treatment. Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of porous organic polymer (POP) adsorbents. These planar monomers with multiple phenolic hydroxyl groups facilitated the formation of aza-linked polymers with hierarchical porous structures, sheet-like morphology, good surface wettability, and high degree of functionality. Such structural characteristics of the CTT-POP adsorbents provided superfast adsorption of various cationic dyes from water. For the adsorption of methylene blue dye, the pseudo-second-order rate constant of CTT-POP-1 is 12.9 g mg-1 min-1, superior to those reported in the existing literature. In addition, CTT-POP-1 can be regenerated at least seven times with no loss in performance, indicating its potential application in water treatment.Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl triazines (CTT), containing intramolecular hydrogen-bonding patterns, were recognized to be intriguing building blocks for the construction of porous organic polymer (POP) adsorbents. These planar monomers with multiple phenolic hydroxyl groups facilitated the formation of aza-linked polymers with hierarchical porous structures, sheet-like morphology, good surface wettability, and high degree of functionality. Such structural characteristics of the CTT-POP adsorbents provided superfast adsorption of various cationic dyes from water. For the adsorption of methylene blue dye, the pseudo-second-order rate constant of CTT-POP-1 is 12.9 g mg-1 min-1, superior to those reported in the existing literature. In addition, CTT-POP-1 can be regenerated at least seven times with no loss in performance, indicating its potential application in water treatment. |
| Author | Hu, Bing Cao, Xiao-Mei Hong, Xin Ding, San-Yuan Huang, Xiao-Qing Zhang, Yong Lin, Hui |
| AuthorAffiliation | State Key Laboratory of Applied Organic Chemistry, College of Chemistry and Chemical Engineering Key Laboratory of Jiangxi Province for the Persistent Pollutants Control and Resources Recycle Nanchang Hangkong University Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering |
| AuthorAffiliation_xml | – name: Nanchang Hangkong University – name: Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering – name: State Key Laboratory of Applied Organic Chemistry, College of Chemistry and Chemical Engineering – name: Key Laboratory of Jiangxi Province for the Persistent Pollutants Control and Resources Recycle |
| Author_xml | – sequence: 1 givenname: Yong orcidid: 0000-0001-8911-4650 surname: Zhang fullname: Zhang, Yong email: yong_zhanggnnu@126.com organization: Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering – sequence: 2 givenname: Xin surname: Hong fullname: Hong, Xin organization: Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering – sequence: 3 givenname: Xiao-Mei surname: Cao fullname: Cao, Xiao-Mei organization: Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering – sequence: 4 givenname: Xiao-Qing surname: Huang fullname: Huang, Xiao-Qing organization: Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering – sequence: 5 givenname: Bing surname: Hu fullname: Hu, Bing organization: Key Laboratory of Organo-Pharmaceutical Chemistry, College of Chemistry and Chemical Engineering – sequence: 6 givenname: San-Yuan orcidid: 0000-0003-2160-4092 surname: Ding fullname: Ding, San-Yuan organization: State Key Laboratory of Applied Organic Chemistry, College of Chemistry and Chemical Engineering – sequence: 7 givenname: Hui surname: Lin fullname: Lin, Hui email: linhui07lanzhou@163.com organization: Nanchang Hangkong University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33517654$$D View this record in MEDLINE/PubMed |
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| Snippet | Developing efficient adsorbents for the removal of water pollutants is of great significance for environmental protection. In this study, conjugated triaryl... |
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| SubjectTerms | adsorbents adsorption Energy, Environmental, and Catalysis Applications hydrogen bonding methylene blue polymers triazines water treatment wettability |
| Title | Functional Porous Organic Polymers with Conjugated Triaryl Triazine as the Core for Superfast Adsorption Removal of Organic Dyes |
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