Fast-Recoverable, Self-Healable, and Adhesive Nanocomposite Hydrogel Consisting of Hybrid Nanoparticles for Ultrasensitive Strain and Pressure Sensing
To meet various practical requirements and enhance human experience, hydrogels possessing multifunctionality are of great significance for flexible wearable sensors. Herein, a novel strategy has been developed to fabricate nanocomposite hydrogels with a combination of excellent stretchability, rapid...
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| Published in | Chemistry of materials Vol. 33; no. 15; pp. 6146 - 6157 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
10.08.2021
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| Online Access | Get full text |
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| Abstract | To meet various practical requirements and enhance human experience, hydrogels possessing multifunctionality are of great significance for flexible wearable sensors. Herein, a novel strategy has been developed to fabricate nanocomposite hydrogels with a combination of excellent stretchability, rapid recoverability, self-healing, and outstanding adhesiveness. The PAAc/SiO2-g-PAAm nanocomposite hydrogels were facilely prepared through the polymerization of acrylic acid (AAc) using SiO2-g-polyacrylamide core–shell hybrid nanoparticles (SiO2-g-PAAm) as the dynamic cross-linking center. The densely dynamic hydrogen bonds between PAAc matrices and grafted PAAm chains could reversibly be destructed and reconstructed to dissipate a large amount of energy. Due to this unique feature, the formulated hydrogels showed a wide spectrum of desirable properties, including skin-mimetic modulus, excellent stretchability (1600%), exceptional self-healing properties (96.5% at ambient temperature), and fast recoverability. The sensors fabricated with the prepared hydrogels exhibited a high detection sensitivity in the strain range from 50% to 500% with a gauge factor value of 5.86, rapid response time, and good antifatigue performance. Depending on the outstanding adhesiveness, this sensor could attach to different substrates to release the real-time motion monitoring. In the practical wearable sensing test, various human motions, including tiny-scaled swallowing, laughing, and speaking, as well as large-scaled wrist, elbow, and knee movements during basketball shooting, could be sensed. These demonstrations heralded the potential application of our sensor in accurate and long-term human motion monitoring. |
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| AbstractList | To meet various practical requirements and enhance human experience, hydrogels possessing multifunctionality are of great significance for flexible wearable sensors. Herein, a novel strategy has been developed to fabricate nanocomposite hydrogels with a combination of excellent stretchability, rapid recoverability, self-healing, and outstanding adhesiveness. The PAAc/SiO2-g-PAAm nanocomposite hydrogels were facilely prepared through the polymerization of acrylic acid (AAc) using SiO2-g-polyacrylamide core–shell hybrid nanoparticles (SiO2-g-PAAm) as the dynamic cross-linking center. The densely dynamic hydrogen bonds between PAAc matrices and grafted PAAm chains could reversibly be destructed and reconstructed to dissipate a large amount of energy. Due to this unique feature, the formulated hydrogels showed a wide spectrum of desirable properties, including skin-mimetic modulus, excellent stretchability (1600%), exceptional self-healing properties (96.5% at ambient temperature), and fast recoverability. The sensors fabricated with the prepared hydrogels exhibited a high detection sensitivity in the strain range from 50% to 500% with a gauge factor value of 5.86, rapid response time, and good antifatigue performance. Depending on the outstanding adhesiveness, this sensor could attach to different substrates to release the real-time motion monitoring. In the practical wearable sensing test, various human motions, including tiny-scaled swallowing, laughing, and speaking, as well as large-scaled wrist, elbow, and knee movements during basketball shooting, could be sensed. These demonstrations heralded the potential application of our sensor in accurate and long-term human motion monitoring. |
| Author | Zhang, Haopeng Wang, Yufei Zheng, Yong Yu, Xiaohui Fan, Xiaoshan Liu, Tianxi |
| AuthorAffiliation | Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology Jiangnan University |
| AuthorAffiliation_xml | – name: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology – name: Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering – name: Jiangnan University |
| Author_xml | – sequence: 1 givenname: Xiaohui surname: Yu fullname: Yu, Xiaohui organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology – sequence: 2 givenname: Yong surname: Zheng fullname: Zheng, Yong organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology – sequence: 3 givenname: Haopeng surname: Zhang fullname: Zhang, Haopeng organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology – sequence: 4 givenname: Yufei surname: Wang fullname: Wang, Yufei organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology – sequence: 5 givenname: Xiaoshan orcidid: 0000-0002-0617-7400 surname: Fan fullname: Fan, Xiaoshan email: xsfan@dhu.edu.cn organization: State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Innovation Center for Textile Science and Technology – sequence: 6 givenname: Tianxi orcidid: 0000-0002-5592-7386 surname: Liu fullname: Liu, Tianxi email: txliu@fudan.edu.cn organization: Jiangnan University |
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| Title | Fast-Recoverable, Self-Healable, and Adhesive Nanocomposite Hydrogel Consisting of Hybrid Nanoparticles for Ultrasensitive Strain and Pressure Sensing |
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