Photocatalytic Degradation of Methylene Blue by Titanium Dioxide: Experimental and Modeling Study
The application of semiconductors in water treatment via photocatalysis of various pollutants has attracted much attention from researchers. In this work, photocatalytic degradation of methylene blue by P25 titanium dioxide was studied experimentally and then via modeling. The effects of lamp choice...
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| Published in | Industrial & engineering chemistry research Vol. 53; no. 38; pp. 14641 - 14649 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
24.09.2014
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The application of semiconductors in water treatment via photocatalysis of various pollutants has attracted much attention from researchers. In this work, photocatalytic degradation of methylene blue by P25 titanium dioxide was studied experimentally and then via modeling. The effects of lamp choice, concentration of catalyst, and methylene blue were analyzed. Desorption of methylene blue at the start of light radiation was observed, and analyzed in detail for the first time. Both desorption and degradation processes were modeled, and experimental data was fitted to a pseudo-first-order model with sufficient accuracy. The effects of catalyst and initial dye concentration on reaction rate constants were discussed. |
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| AbstractList | The application of semiconductors in water treatment via photocatalysis of various pollutants has attracted much attention from researchers. In this work, photocatalytic degradation of methylene blue by P25 titanium dioxide was studied experimentally and then via modeling. The effects of lamp choice, concentration of catalyst, and methylene blue were analyzed. Desorption of methylene blue at the start of light radiation was observed, and analyzed in detail for the first time. Both desorption and degradation processes were modeled, and experimental data was fitted to a pseudo-first-order model with sufficient accuracy. The effects of catalyst and initial dye concentration on reaction rate constants were discussed. |
| Author | Zhao, X. S Rangaiah, G. P Xu, Chen |
| AuthorAffiliation | School of Chemical Engineering The University of Queensland National University of Singapore Department of Chemical & Biomolecular Engineering |
| AuthorAffiliation_xml | – name: School of Chemical Engineering – name: Department of Chemical & Biomolecular Engineering – name: National University of Singapore – name: The University of Queensland |
| Author_xml | – sequence: 1 givenname: Chen surname: Xu fullname: Xu, Chen organization: National University of Singapore – sequence: 2 givenname: G. P surname: Rangaiah fullname: Rangaiah, G. P email: chegpr@nus.edu.sg organization: National University of Singapore – sequence: 3 givenname: X. S surname: Zhao fullname: Zhao, X. S organization: The University of Queensland |
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| SubjectTerms | catalysts desorption engineering methylene blue photocatalysis pollutants semiconductors titanium dioxide water treatment |
| Title | Photocatalytic Degradation of Methylene Blue by Titanium Dioxide: Experimental and Modeling Study |
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