Self-Hybridized Polaritonic Emission from Layered Perovskites

Light–matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered hybrid organic/inorganic perovskites (2D HOIPs) support strongly bound excitons at room temperature with some of the highest oscillator streng...

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Published inNano letters Vol. 21; no. 14; pp. 6245 - 6252
Main Authors Anantharaman, Surendra B, Stevens, Christopher E, Lynch, Jason, Song, Baokun, Hou, Jin, Zhang, Huiqin, Jo, Kiyoung, Kumar, Pawan, Blancon, Jean-Christophe, Mohite, Aditya D, Hendrickson, Joshua R, Jariwala, Deep
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 28.07.2021
Subjects
Chemistry
Materials Science
Physics
Science & Technology - Other Topics
Hybrid states
Polaritons
Boser action
Rabi splitting
Ruddlesden−Popper perovskites
Online AccessGet full text
ISSN1530-6984
1530-6992
1530-6992
DOI10.1021/acs.nanolett.1c02058

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Abstract Light–matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered hybrid organic/inorganic perovskites (2D HOIPs) support strongly bound excitons at room temperature with some of the highest oscillator strengths and electric loss tangents among the known excitonic materials. Here, we report strong light–matter coupling in Ruddlesden–Popper phase 2D HOIP crystals without the necessity of an external cavity. We report the concurrent occurrence of multiple orders of hybrid light–matter states via both reflectance and luminescence spectroscopy in thick (>100 nm) crystals and near-unity absorption in thin (<20 nm) crystals. We observe resonances with quality factors of >250 in hybridized exciton-polaritons and identify a linear correlation between exciton-polariton mode splitting and extinction coefficient of the various 2D HOIPs. Our work opens the door to studying polariton dynamics in self-hybridized and open cavity systems with broad applications in optoelectronics and photochemistry.
AbstractList Light–matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered hybrid organic/inorganic perovskites (2D HOIPs) support strongly bound excitons at room temperature with some of the highest oscillator strengths and electric loss tangents among the known excitonic materials. Here, we report strong light–matter coupling in Ruddlesden–Popper phase 2D HOIP crystals without the necessity of an external cavity. We report the concurrent occurrence of multiple orders of hybrid light–matter states via both reflectance and luminescence spectroscopy in thick (>100 nm) crystals and near-unity absorption in thin (<20 nm) crystals. We observe resonances with quality factors of >250 in hybridized exciton-polaritons and identify a linear correlation between exciton-polariton mode splitting and extinction coefficient of the various 2D HOIPs. Our work opens the door to studying polariton dynamics in self-hybridized and open cavity systems with broad applications in optoelectronics and photochemistry.
Light-matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered hybrid organic/inorganic perovskites (2D HOIPs) support strongly bound excitons at room temperature with some of the highest oscillator strengths and electric loss tangents among the known excitonic materials. Here, we report strong light-matter coupling in Ruddlesden-Popper phase 2D HOIP crystals without the necessity of an external cavity. We report the concurrent occurrence of multiple orders of hybrid light-matter states via both reflectance and luminescence spectroscopy in thick (>100 nm) crystals and near-unity absorption in thin (<20 nm) crystals. We observe resonances with quality factors of >250 in hybridized exciton-polaritons and identify a linear correlation between exciton-polariton mode splitting and extinction coefficient of the various 2D HOIPs. Our work opens the door to studying polariton dynamics in self-hybridized and open cavity systems with broad applications in optoelectronics and photochemistry.Light-matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered hybrid organic/inorganic perovskites (2D HOIPs) support strongly bound excitons at room temperature with some of the highest oscillator strengths and electric loss tangents among the known excitonic materials. Here, we report strong light-matter coupling in Ruddlesden-Popper phase 2D HOIP crystals without the necessity of an external cavity. We report the concurrent occurrence of multiple orders of hybrid light-matter states via both reflectance and luminescence spectroscopy in thick (>100 nm) crystals and near-unity absorption in thin (<20 nm) crystals. We observe resonances with quality factors of >250 in hybridized exciton-polaritons and identify a linear correlation between exciton-polariton mode splitting and extinction coefficient of the various 2D HOIPs. Our work opens the door to studying polariton dynamics in self-hybridized and open cavity systems with broad applications in optoelectronics and photochemistry.
Not provided.
Author Lynch, Jason
Song, Baokun
Blancon, Jean-Christophe
Hou, Jin
Mohite, Aditya D
Kumar, Pawan
Jo, Kiyoung
Hendrickson, Joshua R
Stevens, Christopher E
Jariwala, Deep
Anantharaman, Surendra B
Zhang, Huiqin
AuthorAffiliation Department of Materials Science and Nanoengineering
Department of Chemical and Biomolecular Engineering
Department of Electrical and Systems Engineering
Rice University
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Keywords Hybrid states
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Boser action
Rabi splitting
Ruddlesden−Popper perovskites
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Snippet Light–matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered...
Light-matter coupling in excitonic materials has been the subject of intense recent investigations due to emergence of new materials. Two-dimensional layered...
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SubjectTerms Chemistry
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Science & Technology - Other Topics
Title Self-Hybridized Polaritonic Emission from Layered Perovskites
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