Specifics of Chemical Composition Origin of Surface Water in the Arctic Zone of Western Siberia
— One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon fluxes and how these fluxes can influence the geochemistry of the surface and ground water. In addition to disturbing the carbon balance, per...
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Published in | Geochemistry international Vol. 60; no. 11; pp. 1153 - 1166 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
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Pleiades Publishing
01.11.2022
Springer Springer Nature B.V |
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Abstract | —
One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon fluxes and how these fluxes can influence the geochemistry of the surface and ground water. In addition to disturbing the carbon balance, permafrost thawing provokes the release of a significant amount of other chemical elements entering natural waters. The paper presents original data obtained by studying surface water in 2020 in the Yamalo–Nenets Autonomous District, which is situated in the Arctic zone of the Russian Federation. Permafrost is widespread in the study area, as also are facilities of the oil and gas industry. This predetermines the importance of research on the chemical composition of natural water, its formation, and ecological–geochemical status, which are critical aspects for assessing the anthropogenic load and predicting the influence of climate changes on the biogeochemical cycles of chemical elements. In the course of our fieldwork, 47 surface water samples were taken in the basins of the Taz, Pur, Ob, and Nadym rivers: 23 samples from rivers and streams and 24 samples from lakes and thaw depressions. The sampling sites were chosen to as comprehensively as possible cover the lake–stream–river system in the catchment areas of major rivers of the Yamalo–Nenets Autonomous District. The chemical composition of the water samples was analyzed at a certified laboratory using methods conventionally applied in solving such problems. The data were processed using statistical methods, including the principal component analysis (PCA). Data analysis demonstrates that surface water in the study area is ultrafresh, with neutral or weakly alkaline pH values. Hydrocarbonate, calcium, and magnesium ions dominate in the ionic composition of the water, and ammonium contents are high in the waters of the lakes and thaw depressions. In addition, the ammonium concentration strongly positively correlates with the content of dissolved organic carbon (DOC) and the values of chemical oxygen demand (COD) and permanganate index (PI). It was found out that the streams (springs and rivers) differ from the lakes and the water of the thaw depressions in higher concentrations of main ions that are brought to the water mainly by natural factors (these are
, Ca
2+
, Mg
2+
, and Na
+
) and higher total dissolved solids (TDS) and pH values. In contrast, the water of the thaw depressions is characterized by the highest concentrations of DOC and the values of other parameters related to organic matter (N–
, COD, and PI). It was shown that the main factors that control the chemical composition of the water are its interaction with organic matter from organic (peat) soil horizons and the mineral components of the underlying rocks and soils. The former factor most significantly impacts the water of the thaw depressions, and the latter one affects mainly the chemical composition of the rivers and streams. The relatively high contents of the chloride and sodium ions in the water of the largest lakes are probably caused by the anthropogenic load. |
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AbstractList | —
One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon fluxes and how these fluxes can influence the geochemistry of the surface and ground water. In addition to disturbing the carbon balance, permafrost thawing provokes the release of a significant amount of other chemical elements entering natural waters. The paper presents original data obtained by studying surface water in 2020 in the Yamalo–Nenets Autonomous District, which is situated in the Arctic zone of the Russian Federation. Permafrost is widespread in the study area, as also are facilities of the oil and gas industry. This predetermines the importance of research on the chemical composition of natural water, its formation, and ecological–geochemical status, which are critical aspects for assessing the anthropogenic load and predicting the influence of climate changes on the biogeochemical cycles of chemical elements. In the course of our fieldwork, 47 surface water samples were taken in the basins of the Taz, Pur, Ob, and Nadym rivers: 23 samples from rivers and streams and 24 samples from lakes and thaw depressions. The sampling sites were chosen to as comprehensively as possible cover the lake–stream–river system in the catchment areas of major rivers of the Yamalo–Nenets Autonomous District. The chemical composition of the water samples was analyzed at a certified laboratory using methods conventionally applied in solving such problems. The data were processed using statistical methods, including the principal component analysis (PCA). Data analysis demonstrates that surface water in the study area is ultrafresh, with neutral or weakly alkaline pH values. Hydrocarbonate, calcium, and magnesium ions dominate in the ionic composition of the water, and ammonium contents are high in the waters of the lakes and thaw depressions. In addition, the ammonium concentration strongly positively correlates with the content of dissolved organic carbon (DOC) and the values of chemical oxygen demand (COD) and permanganate index (PI). It was found out that the streams (springs and rivers) differ from the lakes and the water of the thaw depressions in higher concentrations of main ions that are brought to the water mainly by natural factors (these are
, Ca
2+
, Mg
2+
, and Na
+
) and higher total dissolved solids (TDS) and pH values. In contrast, the water of the thaw depressions is characterized by the highest concentrations of DOC and the values of other parameters related to organic matter (N–
, COD, and PI). It was shown that the main factors that control the chemical composition of the water are its interaction with organic matter from organic (peat) soil horizons and the mineral components of the underlying rocks and soils. The former factor most significantly impacts the water of the thaw depressions, and the latter one affects mainly the chemical composition of the rivers and streams. The relatively high contents of the chloride and sodium ions in the water of the largest lakes are probably caused by the anthropogenic load. Abstract— One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon fluxes and how these fluxes can influence the geochemistry of the surface and ground water. In addition to disturbing the carbon balance, permafrost thawing provokes the release of a significant amount of other chemical elements entering natural waters. The paper presents original data obtained by studying surface water in 2020 in the Yamalo–Nenets Autonomous District, which is situated in the Arctic zone of the Russian Federation. Permafrost is widespread in the study area, as also are facilities of the oil and gas industry. This predetermines the importance of research on the chemical composition of natural water, its formation, and ecological–geochemical status, which are critical aspects for assessing the anthropogenic load and predicting the influence of climate changes on the biogeochemical cycles of chemical elements. In the course of our fieldwork, 47 surface water samples were taken in the basins of the Taz, Pur, Ob, and Nadym rivers: 23 samples from rivers and streams and 24 samples from lakes and thaw depressions. The sampling sites were chosen to as comprehensively as possible cover the lake–stream–river system in the catchment areas of major rivers of the Yamalo–Nenets Autonomous District. The chemical composition of the water samples was analyzed at a certified laboratory using methods conventionally applied in solving such problems. The data were processed using statistical methods, including the principal component analysis (PCA). Data analysis demonstrates that surface water in the study area is ultrafresh, with neutral or weakly alkaline pH values. Hydrocarbonate, calcium, and magnesium ions dominate in the ionic composition of the water, and ammonium contents are high in the waters of the lakes and thaw depressions. In addition, the ammonium concentration strongly positively correlates with the content of dissolved organic carbon (DOC) and the values of chemical oxygen demand (COD) and permanganate index (PI). It was found out that the streams (springs and rivers) differ from the lakes and the water of the thaw depressions in higher concentrations of main ions that are brought to the water mainly by natural factors (these are $${\text{HC}}{{{\text{O}}}_{{\text{3}}}^{ - }$$ , Ca 2+ , Mg 2+ , and Na + ) and higher total dissolved solids (TDS) and pH values. In contrast, the water of the thaw depressions is characterized by the highest concentrations of DOC and the values of other parameters related to organic matter (N– $${\text{N}}{{{\text{H}}}_{4}}^{ + }$$ , COD, and PI). It was shown that the main factors that control the chemical composition of the water are its interaction with organic matter from organic (peat) soil horizons and the mineral components of the underlying rocks and soils. The former factor most significantly impacts the water of the thaw depressions, and the latter one affects mainly the chemical composition of the rivers and streams. The relatively high contents of the chloride and sodium ions in the water of the largest lakes are probably caused by the anthropogenic load. - One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon fluxes and how these fluxes can influence the geochemistry of the surface and ground water. In addition to disturbing the carbon balance, permafrost thawing provokes the release of a significant amount of other chemical elements entering natural waters. The paper presents original data obtained by studying surface water in 2020 in the Yamalo-Nenets Autonomous District, which is situated in the Arctic zone of the Russian Federation. Permafrost is widespread in the study area, as also are facilities of the oil and gas industry. This predetermines the importance of research on the chemical composition of natural water, its formation, and ecological-geochemical status, which are critical aspects for assessing the anthropogenic load and predicting the influence of climate changes on the biogeochemical cycles of chemical elements. In the course of our fieldwork, 47 surface water samples were taken in the basins of the Taz, Pur, Ob, and Nadym rivers: 23 samples from rivers and streams and 24 samples from lakes and thaw depressions. The sampling sites were chosen to as comprehensively as possible cover the lake-stream-river system in the catchment areas of major rivers of the Yamalo-Nenets Autonomous District. The chemical composition of the water samples was analyzed at a certified laboratory using methods conventionally applied in solving such problems. The data were processed using statistical methods, including the principal component analysis (PCA). Data analysis demonstrates that surface water in the study area is ultrafresh, with neutral or weakly alkaline pH values. Hydrocarbonate, calcium, and magnesium ions dominate in the ionic composition of the water, and ammonium contents are high in the waters of the lakes and thaw depressions. In addition, the ammonium concentration strongly positively correlates with the content of dissolved organic carbon (DOC) and the values of chemical oxygen demand (COD) and permanganate index (PI). It was found out that the streams (springs and rivers) differ from the lakes and the water of the thaw depressions in higher concentrations of main ions that are brought to the water mainly by natural factors (these are [Formula omitted], Ca.sup.2+, Mg.sup.2+, and Na.sup.+) and higher total dissolved solids (TDS) and pH values. In contrast, the water of the thaw depressions is characterized by the highest concentrations of DOC and the values of other parameters related to organic matter (N- [Formula omitted], COD, and PI). It was shown that the main factors that control the chemical composition of the water are its interaction with organic matter from organic (peat) soil horizons and the mineral components of the underlying rocks and soils. The former factor most significantly impacts the water of the thaw depressions, and the latter one affects mainly the chemical composition of the rivers and streams. The relatively high contents of the chloride and sodium ions in the water of the largest lakes are probably caused by the anthropogenic load. Abstract—One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon fluxes and how these fluxes can influence the geochemistry of the surface and ground water. In addition to disturbing the carbon balance, permafrost thawing provokes the release of a significant amount of other chemical elements entering natural waters. The paper presents original data obtained by studying surface water in 2020 in the Yamalo–Nenets Autonomous District, which is situated in the Arctic zone of the Russian Federation. Permafrost is widespread in the study area, as also are facilities of the oil and gas industry. This predetermines the importance of research on the chemical composition of natural water, its formation, and ecological–geochemical status, which are critical aspects for assessing the anthropogenic load and predicting the influence of climate changes on the biogeochemical cycles of chemical elements. In the course of our fieldwork, 47 surface water samples were taken in the basins of the Taz, Pur, Ob, and Nadym rivers: 23 samples from rivers and streams and 24 samples from lakes and thaw depressions. The sampling sites were chosen to as comprehensively as possible cover the lake–stream–river system in the catchment areas of major rivers of the Yamalo–Nenets Autonomous District. The chemical composition of the water samples was analyzed at a certified laboratory using methods conventionally applied in solving such problems. The data were processed using statistical methods, including the principal component analysis (PCA). Data analysis demonstrates that surface water in the study area is ultrafresh, with neutral or weakly alkaline pH values. Hydrocarbonate, calcium, and magnesium ions dominate in the ionic composition of the water, and ammonium contents are high in the waters of the lakes and thaw depressions. In addition, the ammonium concentration strongly positively correlates with the content of dissolved organic carbon (DOC) and the values of chemical oxygen demand (COD) and permanganate index (PI). It was found out that the streams (springs and rivers) differ from the lakes and the water of the thaw depressions in higher concentrations of main ions that are brought to the water mainly by natural factors (these are , Ca2+, Mg2+, and Na+) and higher total dissolved solids (TDS) and pH values. In contrast, the water of the thaw depressions is characterized by the highest concentrations of DOC and the values of other parameters related to organic matter (N–, COD, and PI). It was shown that the main factors that control the chemical composition of the water are its interaction with organic matter from organic (peat) soil horizons and the mineral components of the underlying rocks and soils. The former factor most significantly impacts the water of the thaw depressions, and the latter one affects mainly the chemical composition of the rivers and streams. The relatively high contents of the chloride and sodium ions in the water of the largest lakes are probably caused by the anthropogenic load. |
Audience | Academic |
Author | Sokolov, D. A. Kolubaeva, Yu. V. Ivanova, I. S. Soldatova, E. A. |
Author_xml | – sequence: 1 givenname: E. A. surname: Soldatova fullname: Soldatova, E. A. email: 2a61@mail.ru organization: Tomsk Branch, Trofimuk Institute of Petroleum Geology and Geophysics, Siberian Branch, Russian Academy of Sciences, University of Tyumen – sequence: 2 givenname: I. S. surname: Ivanova fullname: Ivanova, I. S. email: ivanovais_1986@mail.ru organization: Tomsk Branch, Trofimuk Institute of Petroleum Geology and Geophysics, Siberian Branch, Russian Academy of Sciences – sequence: 3 givenname: Yu. V. surname: Kolubaeva fullname: Kolubaeva, Yu. V. email: kolubaeva@inbox.ru organization: Tomsk Branch, Trofimuk Institute of Petroleum Geology and Geophysics, Siberian Branch, Russian Academy of Sciences – sequence: 4 givenname: D. A. surname: Sokolov fullname: Sokolov, D. A. email: Sokolovdenis@mail.ru organization: Tomsk Branch, Trofimuk Institute of Petroleum Geology and Geophysics, Siberian Branch, Russian Academy of Sciences, Institute of Soil Science and Agrochemistry, Siberian Branch, Russian Academy of Sciences |
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Cites_doi | 10.1134/S0016702920060087 10.1007/978-3-030-50930-9_24 10.1038/s41598-019-55662-1 10.1002/lol2.10063 10.3390/w12061817 10.1134/S0016702916120090 10.1016/j.gca.2019.11.005 10.1016/j.chnaes.2015.04.004 10.5194/bg-12-3009-2015 10.3390/w9120985 10.1073/pnas.1307031110 10.1134/S1875372811040056 10.1134/S1028334X16010141 10.1177/001316446002000116 10.1016/j.proenv.2012.01.099 10.1016/j.apgeochem.2014.12.004 10.1007/s12237-011-9386-6 10.1016/j.chemosphere.2020.128953 10.5194/bg-12-6301-2015 10.3390/w13213107 10.3390/w12061830 |
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Copyright | The Author(s) 2022. ISSN 0016-7029, Geochemistry International, 2022, Vol. 60, No. 11, pp. 1153–1166. © The Author(s), 2022. This article is an open access publication, corrected publication 2022. Russian Text © The Author(s), 2022, published in Geokhimiya, 2022, Vol. 67, No. 11, pp. 1142–1156. COPYRIGHT 2022 Springer The Author(s) 2022. ISSN 0016-7029, Geochemistry International, 2022, Vol. 60, No. 11, pp. 1153–1166. © The Author(s), 2022. This article is an open access publication, corrected publication 2022. Russian Text © The Author(s), 2022, published in Geokhimiya, 2022, Vol. 67, No. 11, pp. 1142–1156. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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Keywords | rivers natural water biogenic elements thaw depressions organic matter lakes Arctic zone Yamalo–Nenets Autonomous District |
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One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon... Abstract— One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic... - One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic carbon... Abstract—One of the most urgent problems on which current studies of Arctic and subarctic territories are focused is how permafrost thawing can affect organic... |
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SubjectTerms | Ammonium Ammonium compounds Analysis Anthropogenic factors Aquatic resources Arctic research Arctic zone Biogeochemical cycle Biogeochemical cycles Calcium Calcium ions Carbon Catchment area Catchment areas Chemical composition Chemical elements Chemical oxygen demand Climate change Creeks & streams Data analysis Dissolved organic carbon Dissolved solids Earth and Environmental Science Earth Sciences Elements Fieldwork Fluxes Geochemistry Groundwater Human influences Ions Lakes Magnesium Melting Natural waters Oil and gas industry Organic matter Organic soils Peat Permafrost pH effects Polar environments Principal components analysis Rivers Sodium Soil horizons Statistical methods Streams Surface water Thawing Water sampling Water springs Water, Underground |
Title | Specifics of Chemical Composition Origin of Surface Water in the Arctic Zone of Western Siberia |
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