Perovskite-Type Oxides as the Catalyst Precursors for Preparing Supported Metallic Nanocatalysts: A Review
Industrial and nanometallic catalysts are composed of an active component of metallic nanoparticles tailored by one or more additives and/or other metals, which should be in interaction and highly dispersed on a support. Therefore, it is a tough challenge to design and prepare such complicated catal...
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| Published in | Industrial & engineering chemistry research Vol. 57; no. 1; pp. 1 - 17 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
10.01.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Industrial and nanometallic catalysts are composed of an active component of metallic nanoparticles tailored by one or more additives and/or other metals, which should be in interaction and highly dispersed on a support. Therefore, it is a tough challenge to design and prepare such complicated catalysts. One promising way involves using perovskite-type oxides (PTOs, or written as ABO3 according to the composition) as the catalyst precursors. That is the subject of this Review, with the aim to provide inspiration for designing and developing supported metallic nanocatalysts. The contents include ABO3, partially substituted ABO3 (A1‑y A′ y BO3, AB1‑x B′ x O3, and A1‑y A′ y B1‑x B′ x O3), and PTOs supported on a support as the catalysts precursors. In PTOs, transition metal ions at A, A′, B, and B′ sites are confined in a PTO crystallite, and those ions are mixed uniformly at the atomic level, which is the basis for using PTOs as the precursors. |
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| AbstractList | Industrial and nanometallic catalysts are composed of an active component of metallic nanoparticles tailored by one or more additives and/or other metals, which should be in interaction and highly dispersed on a support. Therefore, it is a tough challenge to design and prepare such complicated catalysts. One promising way involves using perovskite-type oxides (PTOs, or written as ABO₃ according to the composition) as the catalyst precursors. That is the subject of this Review, with the aim to provide inspiration for designing and developing supported metallic nanocatalysts. The contents include ABO₃, partially substituted ABO₃ (A₁₋yA′yBO₃, AB₁₋ₓB′ₓO₃, and A₁₋yA′yB₁₋ₓB′ₓO₃), and PTOs supported on a support as the catalysts precursors. In PTOs, transition metal ions at A, A′, B, and B′ sites are confined in a PTO crystallite, and those ions are mixed uniformly at the atomic level, which is the basis for using PTOs as the precursors. Industrial and nanometallic catalysts are composed of an active component of metallic nanoparticles tailored by one or more additives and/or other metals, which should be in interaction and highly dispersed on a support. Therefore, it is a tough challenge to design and prepare such complicated catalysts. One promising way involves using perovskite-type oxides (PTOs, or written as ABO3 according to the composition) as the catalyst precursors. That is the subject of this Review, with the aim to provide inspiration for designing and developing supported metallic nanocatalysts. The contents include ABO3, partially substituted ABO3 (A1‑y A′ y BO3, AB1‑x B′ x O3, and A1‑y A′ y B1‑x B′ x O3), and PTOs supported on a support as the catalysts precursors. In PTOs, transition metal ions at A, A′, B, and B′ sites are confined in a PTO crystallite, and those ions are mixed uniformly at the atomic level, which is the basis for using PTOs as the precursors. |
| Author | Liu, Guilong Yang, Qilei Liu, Yuan |
| AuthorAffiliation | Tianjin Key Laboratory of Applied Catalysis Science & Technology, School of Chemical Engineering & Technology Collaborative Innovation Center of Chemical Science & Engineering College of Chemistry and Chemical Engineering |
| AuthorAffiliation_xml | – name: College of Chemistry and Chemical Engineering – name: Collaborative Innovation Center of Chemical Science & Engineering – name: Tianjin Key Laboratory of Applied Catalysis Science & Technology, School of Chemical Engineering & Technology |
| Author_xml | – sequence: 1 givenname: Qilei surname: Yang fullname: Yang, Qilei organization: Collaborative Innovation Center of Chemical Science & Engineering – sequence: 2 givenname: Guilong surname: Liu fullname: Liu, Guilong email: glliu@tju.edu.cn organization: College of Chemistry and Chemical Engineering – sequence: 3 givenname: Yuan orcidid: 0000-0001-9785-8799 surname: Liu fullname: Liu, Yuan email: yuanliu@tju.edu.cn organization: Collaborative Innovation Center of Chemical Science & Engineering |
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| Title | Perovskite-Type Oxides as the Catalyst Precursors for Preparing Supported Metallic Nanocatalysts: A Review |
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