Surface Modification of Sulfur Electrodes by Chemically Anchored Cross-Linked Polymer Coating for Lithium–Sulfur Batteries
Lithium–sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated (CAPC) sulfur electrode was prepared, through chemical bonding by coordinated Cu ions and cross-linking, to improve cyclability for Li/S bat...
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| Published in | ACS applied materials & interfaces Vol. 7; no. 3; pp. 1401 - 1405 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
28.01.2015
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1944-8244 1944-8252 1944-8252 |
| DOI | 10.1021/am508528p |
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| Abstract | Lithium–sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated (CAPC) sulfur electrode was prepared, through chemical bonding by coordinated Cu ions and cross-linking, to improve cyclability for Li/S batteries. This electrode retained specific capacities greater than 665 mAh g–1 at high current density of 3.35 A g–1 (2C rate) after 100 cycles with an excellent Coulombic efficiency of 100%. |
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| AbstractList | Lithium–sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated (CAPC) sulfur electrode was prepared, through chemical bonding by coordinated Cu ions and cross-linking, to improve cyclability for Li/S batteries. This electrode retained specific capacities greater than 665 mAh g–1 at high current density of 3.35 A g–1 (2C rate) after 100 cycles with an excellent Coulombic efficiency of 100%. Lithium–sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated (CAPC) sulfur electrode was prepared, through chemical bonding by coordinated Cu ions and cross-linking, to improve cyclability for Li/S batteries. This electrode retained specific capacities greater than 665 mAh g–¹ at high current density of 3.35 A g–¹ (2C rate) after 100 cycles with an excellent Coulombic efficiency of 100%. Lithium-sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated (CAPC) sulfur electrode was prepared, through chemical bonding by coordinated Cu ions and cross-linking, to improve cyclability for Li/S batteries. This electrode retained specific capacities greater than 665 mAh g(-1) at high current density of 3.35 A g(-1) (2C rate) after 100 cycles with an excellent Coulombic efficiency of 100%.Lithium-sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated (CAPC) sulfur electrode was prepared, through chemical bonding by coordinated Cu ions and cross-linking, to improve cyclability for Li/S batteries. This electrode retained specific capacities greater than 665 mAh g(-1) at high current density of 3.35 A g(-1) (2C rate) after 100 cycles with an excellent Coulombic efficiency of 100%. |
| Author | Kim, Tae-Hyun Mun, Junyoung Chu, Hodong Lilly Thankamony, Roshni Lim, Sanghyun Yim, Taeeun Kim, Young-Jun |
| AuthorAffiliation | Incheon National University Department of Energy and Chemical Engineering Korea Electronics Technology Institute Organic Material Synthesis Lab. Department of Chemistry Advanced Batteries Research Center |
| AuthorAffiliation_xml | – name: Advanced Batteries Research Center – name: Incheon National University – name: Organic Material Synthesis Lab. Department of Chemistry – name: Department of Energy and Chemical Engineering – name: Korea Electronics Technology Institute |
| Author_xml | – sequence: 1 givenname: Sanghyun surname: Lim fullname: Lim, Sanghyun organization: Incheon National University – sequence: 2 givenname: Roshni surname: Lilly Thankamony fullname: Lilly Thankamony, Roshni organization: Incheon National University – sequence: 3 givenname: Taeeun surname: Yim fullname: Yim, Taeeun organization: Korea Electronics Technology Institute – sequence: 4 givenname: Hodong surname: Chu fullname: Chu, Hodong organization: Incheon National University – sequence: 5 givenname: Young-Jun surname: Kim fullname: Kim, Young-Jun organization: Korea Electronics Technology Institute – sequence: 6 givenname: Junyoung surname: Mun fullname: Mun, Junyoung email: jymun@incheon.ac.kr organization: Incheon National University – sequence: 7 givenname: Tae-Hyun surname: Kim fullname: Kim, Tae-Hyun email: tkim@incheon.ac.kr organization: Incheon National University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25569854$$D View this record in MEDLINE/PubMed |
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| Snippet | Lithium–sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated... Lithium-sulfur batteries suffer from severe self-discharge due to polysulfide dissolution into electrolytes. In this work, a chemically anchored polymer-coated... |
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| SubjectTerms | batteries chemical bonding coatings copper crosslinking electrodes ions polymers sulfur |
| Title | Surface Modification of Sulfur Electrodes by Chemically Anchored Cross-Linked Polymer Coating for Lithium–Sulfur Batteries |
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