Atomic Fe Dispersed Hierarchical Mesoporous Fe–N–C Nanostructures for an Efficient Oxygen Reduction Reaction
Due to the scarcity and high cost of precious metals, the hydrogen economy would ultimately rely on non-platinum-group-metal (non-PGM) catalysts. The non-PGM-catalyzed oxygen reduction reaction, which is the bottleneck for the application of hydrogen fuel cells, is challenging because of the limited...
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| Published in | ACS catalysis Vol. 11; no. 1; pp. 74 - 81 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
01.01.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Due to the scarcity and high cost of precious metals, the hydrogen economy would ultimately rely on non-platinum-group-metal (non-PGM) catalysts. The non-PGM-catalyzed oxygen reduction reaction, which is the bottleneck for the application of hydrogen fuel cells, is challenging because of the limited activity and durability of non-PGM catalysts. A stabilized single-atom catalyst may be a possible solution to this issue. In this work, we employ a coordination-assisted polymerization assembly strategy to synthesize an atomic Fe and N co-doped ordered mesoporous carbon nanosphere (denoted as meso-Fe–N–C). The meso-Fe–N–C possesses a hierarchical structure with a high surface area of 494.7 m2 g–1 as well as a high dispersion of Fe (2.9 wt %) and abundant N (4.4 wt %). With these beneficial structural properties, the meso-Fe–N–C exhibits excellent activity and durability toward the oxygen reduction reaction, outperforming the state-of-the-art Pt/C electrocatalysts. |
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| AbstractList | Due to the scarcity and high cost of precious metals, the hydrogen economy would ultimately rely on non-platinum-group-metal (non-PGM) catalysts. The non-PGM-catalyzed oxygen reduction reaction, which is the bottleneck for the application of hydrogen fuel cells, is challenging because of the limited activity and durability of non-PGM catalysts. A stabilized single-atom catalyst may be a possible solution to this issue. In this work, we employ a coordination-assisted polymerization assembly strategy to synthesize an atomic Fe and N co-doped ordered mesoporous carbon nanosphere (denoted as meso-Fe–N–C). The meso-Fe–N–C possesses a hierarchical structure with a high surface area of 494.7 m2 g–1 as well as a high dispersion of Fe (2.9 wt %) and abundant N (4.4 wt %). With these beneficial structural properties, the meso-Fe–N–C exhibits excellent activity and durability toward the oxygen reduction reaction, outperforming the state-of-the-art Pt/C electrocatalysts. |
| Author | Zhou, Yu Zhang, Jiahao Kang, Yijin Yu, Yanan Ma, Dongsheng Stach, Eric A Xiong, Lei Foucher, Alexandre C Yue, Qin |
| AuthorAffiliation | Department of Materials Science and Engineering Institute of Fundamental and Frontier Science |
| AuthorAffiliation_xml | – name: Institute of Fundamental and Frontier Science – name: Department of Materials Science and Engineering |
| Author_xml | – sequence: 1 givenname: Yu surname: Zhou fullname: Zhou, Yu organization: Institute of Fundamental and Frontier Science – sequence: 2 givenname: Yanan surname: Yu fullname: Yu, Yanan organization: Institute of Fundamental and Frontier Science – sequence: 3 givenname: Dongsheng surname: Ma fullname: Ma, Dongsheng organization: Institute of Fundamental and Frontier Science – sequence: 4 givenname: Alexandre C orcidid: 0000-0001-5042-4002 surname: Foucher fullname: Foucher, Alexandre C organization: Department of Materials Science and Engineering – sequence: 5 givenname: Lei surname: Xiong fullname: Xiong, Lei organization: Institute of Fundamental and Frontier Science – sequence: 6 givenname: Jiahao surname: Zhang fullname: Zhang, Jiahao organization: Institute of Fundamental and Frontier Science – sequence: 7 givenname: Eric A orcidid: 0000-0002-3366-2153 surname: Stach fullname: Stach, Eric A organization: Department of Materials Science and Engineering – sequence: 8 givenname: Qin surname: Yue fullname: Yue, Qin email: qinyue@uestc.edu.cn organization: Institute of Fundamental and Frontier Science – sequence: 9 givenname: Yijin orcidid: 0000-0002-3627-5845 surname: Kang fullname: Kang, Yijin email: kangyijin@uestc.edu.cn organization: Institute of Fundamental and Frontier Science |
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| Keywords | Fe−N−C single-atom catalyst oxygen reduction reaction electrocatalysis mesoporous |
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| Title | Atomic Fe Dispersed Hierarchical Mesoporous Fe–N–C Nanostructures for an Efficient Oxygen Reduction Reaction |
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