Triplet–Triplet Annihilation in 9,10-Diphenylanthracene Derivatives: The Role of Intersystem Crossing and Exciton Diffusion

Triplet–triplet annihilation (TTA) is an attractive way to boost the efficiency of conventional fluorescent organic light-emitting diodes (OLEDs). TTA-active anthracene derivatives are often considered as state-of-the-art emitters due to the proper energy level alignment. In this work, TTA propertie...

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Published inJournal of physical chemistry. C Vol. 121; no. 15; pp. 8515 - 8524
Main Authors Serevičius, Tomas, Komskis, Regimantas, Adomėnas, Povilas, Adomėnienė, Ona, Kreiza, Gediminas, Jankauskas, Vygintas, Kazlauskas, Karolis, Miasojedovas, Aru̅nas, Jankus, Vygintas, Monkman, Andy, Juršėnas, Saulius
Format Journal Article
LanguageEnglish
Published American Chemical Society 20.04.2017
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Abstract Triplet–triplet annihilation (TTA) is an attractive way to boost the efficiency of conventional fluorescent organic light-emitting diodes (OLEDs). TTA-active anthracene derivatives are often considered as state-of-the-art emitters due to the proper energy level alignment. In this work, TTA properties of a series of highly fluorescent nonsymmetrical anthracene compounds bearing 9-(4-arylphenyl) moiety and 10-(4-hexylphenyl) fragments were assessed. Two different methods to enhance the TTA efficiency are demonstrated. First, the intensity of TTA-based delayed fluorescence directly depended on the intersystem crossing (ISC) rate. This ISC rate can be significantly enhanced in more conjugated compounds due to the resonant alignment of S1 and T2 energy levels. While enhanced ISC rate slightly quenches the intensity of prompt fluorescence, the rise of the triplet population boosts the intensity of resultant delayed fluorescence. Second, the triplet annihilation rate can be significantly enhanced by optimization of triplet exciton diffusion regime in the films of anthracene derivatives. We show that the proper layer preparation technology has a crucial influence on uniformity and energetic disorder of the film. This enhances the nondispersive triplet diffusion and increases the resulting delayed fluorescence intensity.
AbstractList Triplet–triplet annihilation (TTA) is an attractive way to boost the efficiency of conventional fluorescent organic light-emitting diodes (OLEDs). TTA-active anthracene derivatives are often considered as state-of-the-art emitters due to the proper energy level alignment. In this work, TTA properties of a series of highly fluorescent nonsymmetrical anthracene compounds bearing 9-(4-arylphenyl) moiety and 10-(4-hexylphenyl) fragments were assessed. Two different methods to enhance the TTA efficiency are demonstrated. First, the intensity of TTA-based delayed fluorescence directly depended on the intersystem crossing (ISC) rate. This ISC rate can be significantly enhanced in more conjugated compounds due to the resonant alignment of S1 and T2 energy levels. While enhanced ISC rate slightly quenches the intensity of prompt fluorescence, the rise of the triplet population boosts the intensity of resultant delayed fluorescence. Second, the triplet annihilation rate can be significantly enhanced by optimization of triplet exciton diffusion regime in the films of anthracene derivatives. We show that the proper layer preparation technology has a crucial influence on uniformity and energetic disorder of the film. This enhances the nondispersive triplet diffusion and increases the resulting delayed fluorescence intensity.
Author Miasojedovas, Aru̅nas
Monkman, Andy
Adomėnas, Povilas
Kazlauskas, Karolis
Komskis, Regimantas
Jankauskas, Vygintas
Kreiza, Gediminas
Adomėnienė, Ona
Serevičius, Tomas
Juršėnas, Saulius
Jankus, Vygintas
AuthorAffiliation Durham University
Institute of Applied Research
Department of Solid State Electronics
Department of Physics
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Title Triplet–Triplet Annihilation in 9,10-Diphenylanthracene Derivatives: The Role of Intersystem Crossing and Exciton Diffusion
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