Molecular Catalysis Enables Fast Polyiodide Conversion for Exceptionally Long-Life Zinc–Iodine Batteries

Zinc–iodine (Zn–I2) batteries hold great promise for high-performance, low-cost electrochemical energy storage, but their practical application faces thorny challenges associated with polyiodide shuttling and insufficient cycling stability. Herein, we propose molecular catalysis for long-life Zn–I2...

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Published inACS energy letters Vol. 9; no. 6; pp. 2858 - 2866
Main Authors Chen, Zihui, Wang, Feifei, Ma, Runlin, Jiao, Wanying, Li, Deyuan, Du, Ao, Yan, Zhijie, Yin, Tianyu, Yin, Xunjie, Li, Qiang, Zhang, Xu, Yang, Nianjun, Zhou, Zhen, Yang, Quan-Hong, Yang, Chunpeng
Format Journal Article
LanguageEnglish
Published American Chemical Society 14.06.2024
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Abstract Zinc–iodine (Zn–I2) batteries hold great promise for high-performance, low-cost electrochemical energy storage, but their practical application faces thorny challenges associated with polyiodide shuttling and insufficient cycling stability. Herein, we propose molecular catalysis for long-life Zn–I2 batteries, employing Hemin as an efficient and stable molecular catalyst. The Hemin molecules containing pentacoordinated iron sites significantly adsorb polyiodides, improve the conversion kinetics of iodine species, reduce triiodide concentration, and suppress polyiodide shuttling. Benefiting from molecular catalysis, the Zn–I2 batteries demonstrate an exceptional cycling life, exceeding 62000 cycles with only 0.00052% decay per cycle while maintaining discharge voltage plateaus. The pivotal function of molecular catalysis in both the adsorption and conversion of polyiodide species shows its significant impact on improving the cycling lifespan of Zn–I2 batteries toward long-life energy storage.
AbstractList Zinc–iodine (Zn–I2) batteries hold great promise for high-performance, low-cost electrochemical energy storage, but their practical application faces thorny challenges associated with polyiodide shuttling and insufficient cycling stability. Herein, we propose molecular catalysis for long-life Zn–I2 batteries, employing Hemin as an efficient and stable molecular catalyst. The Hemin molecules containing pentacoordinated iron sites significantly adsorb polyiodides, improve the conversion kinetics of iodine species, reduce triiodide concentration, and suppress polyiodide shuttling. Benefiting from molecular catalysis, the Zn–I2 batteries demonstrate an exceptional cycling life, exceeding 62000 cycles with only 0.00052% decay per cycle while maintaining discharge voltage plateaus. The pivotal function of molecular catalysis in both the adsorption and conversion of polyiodide species shows its significant impact on improving the cycling lifespan of Zn–I2 batteries toward long-life energy storage.
Author Yin, Tianyu
Zhou, Zhen
Yang, Chunpeng
Zhang, Xu
Chen, Zihui
Li, Deyuan
Li, Qiang
Yan, Zhijie
Yang, Nianjun
Yin, Xunjie
Yang, Quan-Hong
Wang, Feifei
Jiao, Wanying
Du, Ao
Ma, Runlin
AuthorAffiliation Department of Chemistry
Haihe Laboratory of Sustainable Chemical Transformations
Nanoyang Group, Tianjin Key Laboratory of Advanced Carbon and Electrochemical Energy Storage, School of Chemical Engineering and Technology, and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin)
National Industry-Education Integration Platform of Energy Storage
Interdisciplinary Research Center for Sustainable Energy Science and Engineering, School of Chemical Engineering
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Snippet Zinc–iodine (Zn–I2) batteries hold great promise for high-performance, low-cost electrochemical energy storage, but their practical application faces thorny...
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Title Molecular Catalysis Enables Fast Polyiodide Conversion for Exceptionally Long-Life Zinc–Iodine Batteries
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