Adsorption of fulvic acid on goethite
The adsorption of fulvic acid by goethite was determined experimentally as a function of concentration, pH, and ionic strength. The data were described with the CD-MUSIC model of Hiemstra and Van Riemsdijk (1996), which allows the distribution of charge of the bound fulvate molecule over a surface r...
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| Published in | Geochimica et cosmochimica acta Vol. 64; no. 1; pp. 51 - 60 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Ltd
2000
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The adsorption of fulvic acid by goethite was determined experimentally as a function of concentration, pH, and ionic strength. The data were described with the CD-MUSIC model of
Hiemstra and Van Riemsdijk (1996), which allows the distribution of charge of the bound fulvate molecule over a surface region. Simultaneously, the concentration, pH, and salt dependency of the binding of fulvic acid can be described. Using the same parameters, the basic charging behavior of the goethite in the absence of fulvic acid could be described well. The surface species used in the model indicate that inner sphere coordination of carboxylic groups of the fulvate molecule is important at low pH, whereas at high pH the outer sphere coordination with reactive groups of the fulvate molecule with high proton affinity is important. |
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| AbstractList | The adsorption of fulvic acid by goethite was determined experimentally as a function of concentration, pH, and ionic strength. The data were described with the CD-MUSIC model of
Hiemstra and Van Riemsdijk (1996), which allows the distribution of charge of the bound fulvate molecule over a surface region. Simultaneously, the concentration, pH, and salt dependency of the binding of fulvic acid can be described. Using the same parameters, the basic charging behavior of the goethite in the absence of fulvic acid could be described well. The surface species used in the model indicate that inner sphere coordination of carboxylic groups of the fulvate molecule is important at low pH, whereas at high pH the outer sphere coordination with reactive groups of the fulvate molecule with high proton affinity is important. The adsorption of fulvic acid by goethite was determined experimentally as a function of concentration, pH, and ionic strength. The data were described with the CD-MUSIC model of Hiemstra and Van Riemsdijk (1996), which allows the distribution of charge of the bound fulvate molecule over a surface region. Simultaneously, the concentration, pH, and salt dependency of the binding of fulvic acid can be described. Using the same parameters, the basic charging behavior of the goethite in the absence of fulvic acid could be described well. The surface species used in the model indicate that inner sphere coordination of carboxylic groups of the fulvate molecule is important at low pH, whereas at high pH the outer sphere coordination with reactive groups of the fulvate molecule with high proton affinity is important. |
| Author | Lumsdon, David G. Filius, Jeroen D. Hiemstra, Tjisse Meeussen, Johannes C.L. Van Riemsdijk, Willem H. |
| Author_xml | – sequence: 1 givenname: Jeroen D. surname: Filius fullname: Filius, Jeroen D. organization: Department of Environmental Sciences, Sub-department Soil Science and Plant Nutrition, Wageningen Agricultural University, Wageningen, The Netherlands – sequence: 2 givenname: David G. surname: Lumsdon fullname: Lumsdon, David G. organization: Macaulay Land Use Research Institute, Craigiebuckler, Aberdeen, Scotland, UK – sequence: 3 givenname: Johannes C.L. surname: Meeussen fullname: Meeussen, Johannes C.L. organization: Macaulay Land Use Research Institute, Craigiebuckler, Aberdeen, Scotland, UK – sequence: 4 givenname: Tjisse surname: Hiemstra fullname: Hiemstra, Tjisse organization: Department of Environmental Sciences, Sub-department Soil Science and Plant Nutrition, Wageningen Agricultural University, Wageningen, The Netherlands – sequence: 5 givenname: Willem H. surname: Van Riemsdijk fullname: Van Riemsdijk, Willem H. email: Willem.VanRiemsdijk@bodsch.benp.wau.nl organization: Department of Environmental Sciences, Sub-department Soil Science and Plant Nutrition, Wageningen Agricultural University, Wageningen, The Netherlands |
| BackLink | https://www.osti.gov/biblio/20014505$$D View this record in Osti.gov |
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| Snippet | The adsorption of fulvic acid by goethite was determined experimentally as a function of concentration, pH, and ionic strength. The data were described with... |
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| SubjectTerms | ADSORPTION AQUATIC ECOSYSTEMS ECOLOGICAL CONCENTRATION ENVIRONMENTAL SCIENCES FULVIC ACIDS GOETHITE IONIC CONDUCTIVITY PH VALUE Sectie Bodemkwaliteit SORPTIVE PROPERTIES Sub-department of Soil Quality WIMEK |
| Title | Adsorption of fulvic acid on goethite |
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