Surface Electrochemistry of Carbon Electrodes and Faradaic Reactions in Capacitive Deionization

Recent advances in electrochemical desalination techniques have paved way for utilization of saline water. In particular, capacitive deionization (CDI) enables removal of salts with high energy efficiency and economic feasibility, while its applicability has been challenged by degradation of carbon...

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Published inEnvironmental science & technology Vol. 56; no. 17; pp. 12602 - 12612
Main Authors Kang, Jin Soo, Kim, Seoni, Kang, Jiho, Joo, Hwajoo, Jang, Junghwan, Jo, Kyusik, Park, Subin, Kim, Hyoung-il, Yoo, Sung Jong, Yoon, Jeyong, Sung, Yung-Eun, Hatton, T. Alan
Format Journal Article
LanguageEnglish
Published Easton American Chemical Society 06.09.2022
Subjects
Carbon
Chemical reactions
Deionization
Desalination
Electrochemical desalination
Electrochemistry
Electrodes
Energy efficiency
Saline water
Salts
Treatment and Resource Recovery
desalination
Faradaic reaction
electrochemistry
capacitive deionization
carbon
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Abstract Recent advances in electrochemical desalination techniques have paved way for utilization of saline water. In particular, capacitive deionization (CDI) enables removal of salts with high energy efficiency and economic feasibility, while its applicability has been challenged by degradation of carbon electrodes in long-term operations. Herein, we report a thorough investigation on the surface electrochemistry of carbon electrodes and Faradaic reactions that are responsible for stability issues of CDI systems. By using bare and membrane CDI (MCDI) as model systems, we identified various electrochemical reactions of carbon electrodes with water or oxygen, with thermodynamics and kinetics governed by the electrode potential and pH. As a result, a complete overview of the Faradaic reactions taking place in CDI was constructed by tracing the physicochemical changes occurring in CDI and MCDI systems.
AbstractList Recent advances in electrochemical desalination techniques have paved way for utilization of saline water. In particular, capacitive deionization (CDI) enables removal of salts with high energy efficiency and economic feasibility, while its applicability has been challenged by degradation of carbon electrodes in long-term operations. Herein, we report a thorough investigation on the surface electrochemistry of carbon electrodes and Faradaic reactions that are responsible for stability issues of CDI systems. By using bare and membrane CDI (MCDI) as model systems, we identified various electrochemical reactions of carbon electrodes with water or oxygen, with thermodynamics and kinetics governed by the electrode potential and pH. As a result, a complete overview of the Faradaic reactions taking place in CDI was constructed by tracing the physicochemical changes occurring in CDI and MCDI systems.
Author Kim, Hyoung-il
Kim, Seoni
Joo, Hwajoo
Yoon, Jeyong
Yoo, Sung Jong
Hatton, T. Alan
Kang, Jiho
Jo, Kyusik
Kang, Jin Soo
Jang, Junghwan
Sung, Yung-Eun
Park, Subin
AuthorAffiliation Department of Civil and Environmental Engineering
Center for Hydrogen·Fuel Cell Research
Korea Institute of Science and Technology (KIST)
Department of Chemical Engineering
School of Chemical and Biological Engineering and Institute of Chemical Processes (ICP)
Yonsei University
Center for Nanoparticle Research
Department of Energy Systems Engineering
Department of Energy Resources Engineering and Research Institute of Energy and Resources
Institute for Basic Science (IBS)
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Faradaic reaction
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Snippet Recent advances in electrochemical desalination techniques have paved way for utilization of saline water. In particular, capacitive deionization (CDI) enables...
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SubjectTerms Carbon
Chemical reactions
Deionization
Desalination
Electrochemical desalination
Electrochemistry
Electrodes
Energy efficiency
Saline water
Salts
Treatment and Resource Recovery
Title Surface Electrochemistry of Carbon Electrodes and Faradaic Reactions in Capacitive Deionization
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