Electrospray Deposition of {200} Oriented Regular-Assembly BaTiO3 Nanocrystal Films under an Electric Field
Highly oriented, regularly assembled nanocrystalline films have recently emerged as attractive new functional materials. In this study, we deposited a BaTiO3 (BT) nanocube dispersion on a Si substrate by electrospraying, resulting in a dense, regularly assembled BT nanocrystalline film. X-ray diffra...
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Published in | Langmuir Vol. 35; no. 16; pp. 5496 - 5500 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
Published |
American Chemical Society
23.04.2019
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Abstract | Highly oriented, regularly assembled nanocrystalline films have recently emerged as attractive new functional materials. In this study, we deposited a BaTiO3 (BT) nanocube dispersion on a Si substrate by electrospraying, resulting in a dense, regularly assembled BT nanocrystalline film. X-ray diffraction analysis revealed that applying a voltage between the electrospray nozzle and the Si substrate during electrospraying caused the BT nanocubes to form a regular array in the 200 plane aligned perpendicularly to the substrate. The volume fraction of BT nanocubes in the 200 plane in the assembly was estimated by the orientation distribution function analysis to be about 50%. The formation of this regularly assembled layer was determined to be linked to the interaction between the vaporized solvent and the substrate, enabled by the enhanced wettability under the electric field. Electrospray deposition has potential applications in the manufacture of nanocrystalline assembled films for nanofunctional devices. |
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AbstractList | Highly oriented, regularly assembled nanocrystalline films have recently emerged as attractive new functional materials. In this study, we deposited a BaTiO3 (BT) nanocube dispersion on a Si substrate by electrospraying, resulting in a dense, regularly assembled BT nanocrystalline film. X-ray diffraction analysis revealed that applying a voltage between the electrospray nozzle and the Si substrate during electrospraying caused the BT nanocubes to form a regular array in the 200 plane aligned perpendicularly to the substrate. The volume fraction of BT nanocubes in the 200 plane in the assembly was estimated by the orientation distribution function analysis to be about 50%. The formation of this regularly assembled layer was determined to be linked to the interaction between the vaporized solvent and the substrate, enabled by the enhanced wettability under the electric field. Electrospray deposition has potential applications in the manufacture of nanocrystalline assembled films for nanofunctional devices. |
Author | Suehiro, Satoshi Takahashi, Seiji Kimura, Teiichi Mimura, Ken-ichi Tanaka, Makoto Kato, Kazumi |
AuthorAffiliation | Materials Research and Development Laboratory National Institute of Advanced Industrial Science and Technology (AIST) Inorganic Functional Material Research Institute |
AuthorAffiliation_xml | – name: Materials Research and Development Laboratory – name: National Institute of Advanced Industrial Science and Technology (AIST) – name: Inorganic Functional Material Research Institute |
Author_xml | – sequence: 1 givenname: Satoshi orcidid: 0000-0002-9648-0461 surname: Suehiro fullname: Suehiro, Satoshi email: s_suehiro@jfcc.or.jp organization: Materials Research and Development Laboratory – sequence: 2 givenname: Teiichi surname: Kimura fullname: Kimura, Teiichi organization: Materials Research and Development Laboratory – sequence: 3 givenname: Makoto surname: Tanaka fullname: Tanaka, Makoto organization: Materials Research and Development Laboratory – sequence: 4 givenname: Seiji surname: Takahashi fullname: Takahashi, Seiji organization: Materials Research and Development Laboratory – sequence: 5 givenname: Ken-ichi surname: Mimura fullname: Mimura, Ken-ichi organization: National Institute of Advanced Industrial Science and Technology (AIST) – sequence: 6 givenname: Kazumi surname: Kato fullname: Kato, Kazumi organization: National Institute of Advanced Industrial Science and Technology (AIST) |
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Title | Electrospray Deposition of {200} Oriented Regular-Assembly BaTiO3 Nanocrystal Films under an Electric Field |
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