Fabrication and Photovoltaic Conversion Performances of Imidazolyl and Fumaric Acid Composite Langmuir–Blodgett Membranes
Novel organic small molecule structures have received increasing attention in the preparation of multifunctional thin film materials and have become the subject of research in many cutting-edge directions. In this work, imidazolyl and transbutylene glycolic acid molecules and dye molecules were desi...
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| Published in | Langmuir Vol. 40; no. 35; pp. 18642 - 18651 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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United States
American Chemical Society
03.09.2024
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| Abstract | Novel organic small molecule structures have received increasing attention in the preparation of multifunctional thin film materials and have become the subject of research in many cutting-edge directions. In this work, imidazolyl and transbutylene glycolic acid molecules and dye molecules were designed and prepared as composite films by supramolecular self-assembly in the LB technique, and their morphological features and spectral properties were analyzed. The results showed that the prepared LB films presented different aggregation states. In addition, their photoelectrochemical properties, on ITO sheets were tested, all of which showed good optoelectronic properties, and their binding energies, structure optimization, and electrostatic potentials were theoretically calculated by DFT simulations, which proved that the prepared films have good optoelectronic properties, and have the potential to become optoelectronic multifunctional ultrathin film devices. |
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| AbstractList | Novel organic small molecule structures have received increasing attention in the preparation of multifunctional thin film materials and have become the subject of research in many cutting-edge directions. In this work, imidazolyl and transbutylene glycolic acid molecules and dye molecules were designed and prepared as composite films by supramolecular self-assembly in the LB technique, and their morphological features and spectral properties were analyzed. The results showed that the prepared LB films presented different aggregation states. In addition, their photoelectrochemical properties, on ITO sheets were tested, all of which showed good optoelectronic properties, and their binding energies, structure optimization, and electrostatic potentials were theoretically calculated by DFT simulations, which proved that the prepared films have good optoelectronic properties, and have the potential to become optoelectronic multifunctional ultrathin film devices. Novel organic small molecule structures have received increasing attention in the preparation of multifunctional thin film materials and have become the subject of research in many cutting-edge directions. In this work, imidazolyl and transbutylene glycolic acid molecules and dye molecules were designed and prepared as composite films by supramolecular self-assembly in the LB technique, and their morphological features and spectral properties were analyzed. The results showed that the prepared LB films presented different aggregation states. In addition, their photoelectrochemical properties, on ITO sheets were tested, all of which showed good optoelectronic properties, and their binding energies, structure optimization, and electrostatic potentials were theoretically calculated by DFT simulations, which proved that the prepared films have good optoelectronic properties, and have the potential to become optoelectronic multifunctional ultrathin film devices.Novel organic small molecule structures have received increasing attention in the preparation of multifunctional thin film materials and have become the subject of research in many cutting-edge directions. In this work, imidazolyl and transbutylene glycolic acid molecules and dye molecules were designed and prepared as composite films by supramolecular self-assembly in the LB technique, and their morphological features and spectral properties were analyzed. The results showed that the prepared LB films presented different aggregation states. In addition, their photoelectrochemical properties, on ITO sheets were tested, all of which showed good optoelectronic properties, and their binding energies, structure optimization, and electrostatic potentials were theoretically calculated by DFT simulations, which proved that the prepared films have good optoelectronic properties, and have the potential to become optoelectronic multifunctional ultrathin film devices. |
| Author | Yang, Huiqing Qiao, Guiying Han, Yong Bian, Pengfei Zhang, Lexin Liu, Zhiwei Jiao, Tifeng |
| AuthorAffiliation | School of Electrical Engineering State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse |
| AuthorAffiliation_xml | – name: State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse – name: School of Electrical Engineering |
| Author_xml | – sequence: 1 givenname: Pengfei surname: Bian fullname: Bian, Pengfei organization: State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse – sequence: 2 givenname: Huiqing surname: Yang fullname: Yang, Huiqing organization: School of Electrical Engineering – sequence: 3 givenname: Lexin surname: Zhang fullname: Zhang, Lexin organization: State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse – sequence: 4 givenname: Zhiwei surname: Liu fullname: Liu, Zhiwei organization: State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse – sequence: 5 givenname: Guiying surname: Qiao fullname: Qiao, Guiying organization: State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse – sequence: 6 givenname: Yong orcidid: 0000-0003-2915-2174 surname: Han fullname: Han, Yong email: hanyong@ysu.edu.cn organization: School of Electrical Engineering – sequence: 7 givenname: Tifeng orcidid: 0000-0003-1238-0277 surname: Jiao fullname: Jiao, Tifeng email: tfjiao@ysu.edu.cn organization: State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Applied Chemistry, Hebei Key Laboratory of Nano-biotechnology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse |
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| Title | Fabrication and Photovoltaic Conversion Performances of Imidazolyl and Fumaric Acid Composite Langmuir–Blodgett Membranes |
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