Layered Co(OH)2 Deposited Polymeric Carbon Nitrides for Photocatalytic Water Oxidation
Here we report a facile impregnation synthesis of layered Co(OH)2 deposited with g-C3N4 while the pH value is adjusted by using ammonia solution for photocatalytic water oxidation with UV–vis and visible light illumination. This surface modification not only accelerates the interface transfer rate...
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| Published in | ACS catalysis Vol. 5; no. 2; pp. 941 - 947 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
06.02.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Here we report a facile impregnation synthesis of layered Co(OH)2 deposited with g-C3N4 while the pH value is adjusted by using ammonia solution for photocatalytic water oxidation with UV–vis and visible light illumination. This surface modification not only accelerates the interface transfer rate of charge carriers but also reduces the excessive energy barrier for O–O formation, thus leading to enhanced reaction kinetics for photocatalytic water oxidation. The optimum oxygen evolution rates (OERs) of the Co(OH)2/g-C3N4 sample reached 27.4 and 7.1 μmol h–1 under UV–vis (λ >300 nm) and visible light (λ >420 nm) irradiation, which are 5.5 and 7 times faster than those for pristine g-C3N4, respectively. These results underline the possibility for the development of effective, robust, and earth-abundant WOCs for the promotion of water-splitting photocatalysis by sustainable g-C3N4 polymer photocatalysts. |
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| AbstractList | Here we report a facile impregnation synthesis of layered Co(OH)2 deposited with g-C3N4 while the pH value is adjusted by using ammonia solution for photocatalytic water oxidation with UV–vis and visible light illumination. This surface modification not only accelerates the interface transfer rate of charge carriers but also reduces the excessive energy barrier for O–O formation, thus leading to enhanced reaction kinetics for photocatalytic water oxidation. The optimum oxygen evolution rates (OERs) of the Co(OH)2/g-C3N4 sample reached 27.4 and 7.1 μmol h–1 under UV–vis (λ >300 nm) and visible light (λ >420 nm) irradiation, which are 5.5 and 7 times faster than those for pristine g-C3N4, respectively. These results underline the possibility for the development of effective, robust, and earth-abundant WOCs for the promotion of water-splitting photocatalysis by sustainable g-C3N4 polymer photocatalysts. |
| Author | Zhang, Guigang Zang, Shaohong Wang, Xinchen |
| AuthorAffiliation | State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry Fuzhou University |
| AuthorAffiliation_xml | – name: State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry – name: Fuzhou University |
| Author_xml | – sequence: 1 givenname: Guigang surname: Zhang fullname: Zhang, Guigang – sequence: 2 givenname: Shaohong surname: Zang fullname: Zang, Shaohong – sequence: 3 givenname: Xinchen surname: Wang fullname: Wang, Xinchen email: xcwang@fzu.edu.cn |
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| Issue | 2 |
| Keywords | water oxidation photocatalysis cobalt hydroxide heterojunction graphitic carbon nitride |
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| Snippet | Here we report a facile impregnation synthesis of layered Co(OH)2 deposited with g-C3N4 while the pH value is adjusted by using ammonia solution for... |
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| Title | Layered Co(OH)2 Deposited Polymeric Carbon Nitrides for Photocatalytic Water Oxidation |
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