A Highly Ordered Nanoporous, Two-Dimensional Covalent Organic Framework with Modifiable Pores, and Its Application in Water Purification and Ion Sieving
The preparation of membranes with high selectivity based on specific chemical properties such as size and charge would impact the efficiency of the world’s energy supply, the production of clean water, and many other separation technologies. We report a flexible synthetic protocol for preparing high...
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| Published in | Journal of the American Chemical Society Vol. 140; no. 51; pp. 18200 - 18207 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
WASHINGTON
American Chemical Society
26.12.2018
Amer Chemical Soc |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The preparation of membranes with high selectivity based on specific chemical properties such as size and charge would impact the efficiency of the world’s energy supply, the production of clean water, and many other separation technologies. We report a flexible synthetic protocol for preparing highly ordered two-dimensional nanoporous polymeric materials (termed covalent organic frameworks or COFs) that allow for placing virtually any function group within the nanopores. We demonstrate that membranes, fabricated with this new family of materials with carboxylated pore walls, are very water permeable, as well as highly charged and size selective. |
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| AbstractList | The preparation of membranes with high selectivity based on specific chemical properties such as size and charge would impact the efficiency of the world’s energy supply, the production of clean water, and many other separation technologies. We report a flexible synthetic protocol for preparing highly ordered two-dimensional nanoporous polymeric materials (termed covalent organic frameworks or COFs) that allow for placing virtually any function group within the nanopores. We demonstrate that membranes, fabricated with this new family of materials with carboxylated pore walls, are very water permeable, as well as highly charged and size selective. |
| Author | Newell, Brian Parkinson, Bruce A Yin, Jiashi Hoberg, John O Kuehl, Valerie A Li-Oakey, Katie Dongmei Duong, Phuoc H. H Mastorovich, Bruce |
| AuthorAffiliation | Department of Chemistry Central Instrument Facility Department of Chemical Engineering |
| AuthorAffiliation_xml | – name: Department of Chemical Engineering – name: Central Instrument Facility – name: – name: Department of Chemistry |
| Author_xml | – sequence: 1 givenname: Valerie A surname: Kuehl fullname: Kuehl, Valerie A – sequence: 2 givenname: Jiashi surname: Yin fullname: Yin, Jiashi – sequence: 3 givenname: Phuoc H. H surname: Duong fullname: Duong, Phuoc H. H – sequence: 4 givenname: Bruce surname: Mastorovich fullname: Mastorovich, Bruce – sequence: 5 givenname: Brian surname: Newell fullname: Newell, Brian organization: Central Instrument Facility – sequence: 6 givenname: Katie Dongmei orcidid: 0000-0002-0529-9203 surname: Li-Oakey fullname: Li-Oakey, Katie Dongmei email: dli1@uwyo.edu – sequence: 7 givenname: Bruce A orcidid: 0000-0002-8950-1922 surname: Parkinson fullname: Parkinson, Bruce A email: bparkin1@uwyo.edu – sequence: 8 givenname: John O orcidid: 0000-0003-3833-8122 surname: Hoberg fullname: Hoberg, John O email: hoberg@uwyo.edu |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30512941$$D View this record in MEDLINE/PubMed |
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| Snippet | The preparation of membranes with high selectivity based on specific chemical properties such as size and charge would impact the efficiency of the world’s... The preparation of membranes with high selectivity based on specific chemical properties such as size and charge would impact the efficiency of the world's... |
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| Title | A Highly Ordered Nanoporous, Two-Dimensional Covalent Organic Framework with Modifiable Pores, and Its Application in Water Purification and Ion Sieving |
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