Hydrothermal remobilization of subseafloor sulfide mineralization along mid-ocean ridges contributes to the global oceanic zinc isotopic mass balance
Hydrothermal activity on mid-ocean ridges is an important mechanism for the delivery of Zn from the mantle to the surface environment. Zinc isotopic fractionation during hydrothermal activity is mainly controlled by the precipitation of Zn-bearing sulfide minerals, in which isotopically light Zn is...
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| Published in | Geochimica et cosmochimica acta Vol. 335; pp. 56 - 67 |
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| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
15.10.2022
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| Abstract | Hydrothermal activity on mid-ocean ridges is an important mechanism for the delivery of Zn from the mantle to the surface environment. Zinc isotopic fractionation during hydrothermal activity is mainly controlled by the precipitation of Zn-bearing sulfide minerals, in which isotopically light Zn is preferentially retained in solid phases rather than in solution during mineral precipitation. Thus, seafloor hydrothermal activity is expected to supply isotopically heavy Zn to the ocean. Here, we studied sulfide-rich samples from the Duanqiao-1 hydrothermal field, located on the Southwest Indian Ridge. We report that, at the hand-specimen scale, late-stage conduit sulfide material has lower δ66Zn values (−0.05 ± 0.15 ‰; n = 19) than early-stage material (+0.13 ± 0.15 ‰; n = 10). These lower values correlate with enrichments in Pb, As, Cd, and Ag, and elevated δ34S values. We attribute the low δ66Zn values to the remobilization of earlier sub-seafloor Zn-rich mineralization. Based on endmember mass balance calculations, and an assumption of a fractionation factor (αZnS-Sol.) of about 0.9997 between sphalerite and its parent solution, the remobilized Zn was found consist of about 1/3 to 2/3 of the total Zn in the fluid that formed the conduit samples. Our study suggests that late-stage subsurface hydrothermal remobilization may release isotopically-light Zn to the ocean, and that this process may be common along mid-ocean ridges, thus increasing the size of the previously identified isotopically light Zn sink in the ocean. |
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| AbstractList | Hydrothermal activity on mid-ocean ridges is an important mechanism for the delivery of Zn from the mantle to the surface environment. Zinc isotopic fractionation during hydrothermal activity is mainly controlled by the precipitation of Zn-bearing sulfide minerals, in which isotopically light Zn is preferentially retained in solid phases rather than in solution during mineral precipitation. Thus, seafloor hydrothermal activity is expected to supply isotopically heavy Zn to the ocean. Here, we studied sulfide-rich samples from the Duanqiao-1 hydrothermal field, located on the Southwest Indian Ridge. We report that, at the hand-specimen scale, late-stage conduit sulfide material has lower δ66Zn values (−0.05 ± 0.15 ‰; n = 19) than early-stage material (+0.13 ± 0.15 ‰; n = 10). These lower values correlate with enrichments in Pb, As, Cd, and Ag, and elevated δ34S values. We attribute the low δ66Zn values to the remobilization of earlier sub-seafloor Zn-rich mineralization. Based on endmember mass balance calculations, and an assumption of a fractionation factor (αZnS-Sol.) of about 0.9997 between sphalerite and its parent solution, the remobilized Zn was found consist of about 1/3 to 2/3 of the total Zn in the fluid that formed the conduit samples. Our study suggests that late-stage subsurface hydrothermal remobilization may release isotopically-light Zn to the ocean, and that this process may be common along mid-ocean ridges, thus increasing the size of the previously identified isotopically light Zn sink in the ocean. |
| Author | Liang, Jin Li, Xiaohu Li, Wei Ding, Teng Zhu, Chuanwei Zhang, Huichao Liao, Shili Dias, Ágata Alveirinho Tao, Chunhui Wen, Hanjie Yang, Weifang Liu, Jia Jamieson, John W. |
| Author_xml | – sequence: 1 givenname: Shili surname: Liao fullname: Liao, Shili organization: Key Laboratory of Submarine Geosciences, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou 310012, Zhejiang, China – sequence: 2 givenname: Chunhui surname: Tao fullname: Tao, Chunhui email: taochunhuimail@163.com organization: Key Laboratory of Submarine Geosciences, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou 310012, Zhejiang, China – sequence: 3 givenname: Hanjie surname: Wen fullname: Wen, Hanjie email: wenhanjie@vip.gyig.ac.cn organization: School of Earth Sciences and Resources, Chang’An University, Xi’an 710054, China – sequence: 4 givenname: Weifang surname: Yang fullname: Yang, Weifang organization: Key Laboratory of Submarine Geosciences, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou 310012, Zhejiang, China – sequence: 5 givenname: Jia surname: Liu fullname: Liu, Jia organization: Key Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China – sequence: 6 givenname: John W. surname: Jamieson fullname: Jamieson, John W. organization: Department of Earth Sciences, Memorial University of Newfoundland, St. John’s, NL A1B 3X5, Canada – sequence: 7 givenname: Ágata Alveirinho surname: Dias fullname: Dias, Ágata Alveirinho organization: Institute of Science and Environment, University of Saint Joseph, Macao SAR, China – sequence: 8 givenname: Chuanwei surname: Zhu fullname: Zhu, Chuanwei organization: State Key Laboratory of Ore Deposit Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China – sequence: 9 givenname: Jin surname: Liang fullname: Liang, Jin organization: Key Laboratory of Submarine Geosciences, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou 310012, Zhejiang, China – sequence: 10 givenname: Wei surname: Li fullname: Li, Wei organization: Key Laboratory of Submarine Geosciences, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou 310012, Zhejiang, China – sequence: 11 givenname: Teng surname: Ding fullname: Ding, Teng organization: Institute of Marine Geology, College of Oceanography, Hohai University, Nanjing 210098, China – sequence: 12 givenname: Xiaohu surname: Li fullname: Li, Xiaohu organization: Key Laboratory of Submarine Geosciences, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou 310012, Zhejiang, China – sequence: 13 givenname: Huichao surname: Zhang fullname: Zhang, Huichao organization: Institute of Marine Geology, College of Oceanography, Hohai University, Nanjing 210098, China |
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| Keywords | Subsurface remobilization Hydrothermal activity Mid ocean ridge Zinc isotopic mass balance |
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| Title | Hydrothermal remobilization of subseafloor sulfide mineralization along mid-ocean ridges contributes to the global oceanic zinc isotopic mass balance |
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