A Sulfide/Polysulfide-Based Ionic Liquid Electrolyte for Quantum Dot-Sensitized Solar Cells
Further development of quantum dot-sensitized solar cells (QDSCs) will require long-term stability in addition to the continuous increase of photovoltaic (PV) conversion efficiency achieved in the last years. We report a robust S2–/S n 2– electrolyte that has been specifically designed for compatibi...
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| Published in | Journal of the American Chemical Society Vol. 133; no. 50; pp. 20156 - 20159 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
21.12.2011
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| Abstract | Further development of quantum dot-sensitized solar cells (QDSCs) will require long-term stability in addition to the continuous increase of photovoltaic (PV) conversion efficiency achieved in the last years. We report a robust S2–/S n 2– electrolyte that has been specifically designed for compatibility with CdSe quantum dots in sensitized solar cells. The new pyrrolidinium ionic liquid reaches 1.86% efficiency and a short-circuit current close to 14 mA·cm–2 under air-mass 1.5 global illumination and improves the device lifetime with good photoanode stability over 240 h. PV characterization showed that the solar cell limitations relate to poor catalysis of regeneration at the counter electrode and high recombination. Further improvement of these factors in the robust electrolyte configuration may thus have a significant impact for advancing the state-of-the-art in QDSCs. |
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| AbstractList | Further development of quantum dot-sensitized solar cells (QDSCs) will require long-term stability in addition to the continuous increase of photovoltaic (PV) conversion efficiency achieved in the last years. We report a robust S(2-)/S(n)(2-) electrolyte that has been specifically designed for compatibility with CdSe quantum dots in sensitized solar cells. The new pyrrolidinium ionic liquid reaches 1.86% efficiency and a short-circuit current close to 14 mA·cm(-2) under air-mass 1.5 global illumination and improves the device lifetime with good photoanode stability over 240 h. PV characterization showed that the solar cell limitations relate to poor catalysis of regeneration at the counter electrode and high recombination. Further improvement of these factors in the robust electrolyte configuration may thus have a significant impact for advancing the state-of-the-art in QDSCs. Further development of quantum dot-sensitized solar cells (QDSCs) will require long-term stability in addition to the continuous increase of photovoltaic (PV) conversion efficiency achieved in the last years. We report a robust S2–/S n 2– electrolyte that has been specifically designed for compatibility with CdSe quantum dots in sensitized solar cells. The new pyrrolidinium ionic liquid reaches 1.86% efficiency and a short-circuit current close to 14 mA·cm–2 under air-mass 1.5 global illumination and improves the device lifetime with good photoanode stability over 240 h. PV characterization showed that the solar cell limitations relate to poor catalysis of regeneration at the counter electrode and high recombination. Further improvement of these factors in the robust electrolyte configuration may thus have a significant impact for advancing the state-of-the-art in QDSCs. |
| Author | Giménez, Sixto Jovanovski, Vasko Bisquert, Juan González-Pedro, Victoria Mora-Seró, Iván Grande, Hans Tena-Zaera, Ramon Azaceta, Eneko Cabañero, Germán |
| AuthorAffiliation | Universitat Jaume I CIDETEC-IK4 National Institute of Chemistry |
| AuthorAffiliation_xml | – name: CIDETEC-IK4 – name: National Institute of Chemistry – name: Universitat Jaume I |
| Author_xml | – sequence: 1 givenname: Vasko surname: Jovanovski fullname: Jovanovski, Vasko – sequence: 2 givenname: Victoria surname: González-Pedro fullname: González-Pedro, Victoria – sequence: 3 givenname: Sixto surname: Giménez fullname: Giménez, Sixto – sequence: 4 givenname: Eneko surname: Azaceta fullname: Azaceta, Eneko – sequence: 5 givenname: Germán surname: Cabañero fullname: Cabañero, Germán – sequence: 6 givenname: Hans surname: Grande fullname: Grande, Hans – sequence: 7 givenname: Ramon surname: Tena-Zaera fullname: Tena-Zaera, Ramon email: rtena@cidetec.es, sero@fca.uji.es – sequence: 8 givenname: Iván surname: Mora-Seró fullname: Mora-Seró, Iván email: rtena@cidetec.es, sero@fca.uji.es – sequence: 9 givenname: Juan surname: Bisquert fullname: Bisquert, Juan |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22107441$$D View this record in MEDLINE/PubMed |
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| Title | A Sulfide/Polysulfide-Based Ionic Liquid Electrolyte for Quantum Dot-Sensitized Solar Cells |
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