Conjugated Self-Assembled Monolayer as Stable Hole-Selective Contact for Inverted Perovskite Solar Cells
The alkyl linker-based self-assembled monolayer (SAM) has emerged as an efficient hole-selective contact (HSC) for inverted perovskite solar cells (PSCs). Despite being effective in hole-extraction and interfacial passivation, its hole-transporting capability is limited by the insulating alkyl linke...
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| Published in | ACS materials letters Vol. 4; no. 10; pp. 1976 - 1983 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
03.10.2022
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| Online Access | Get full text |
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| Abstract | The alkyl linker-based self-assembled monolayer (SAM) has emerged as an efficient hole-selective contact (HSC) for inverted perovskite solar cells (PSCs). Despite being effective in hole-extraction and interfacial passivation, its hole-transporting capability is limited by the insulating alkyl linker, along with poor stability due to the isolated and nonconjugated electron-rich moiety. Here, we report a series of conjugated SAMs that exhibit excellent photo- and electrical stabilities. The conjugated molecular structure not only enhances charge transport but also stabilizes the electron-rich arylamines through electron/charge delocalization. Moreover, it enables convenient modulation of frontier orbital energy levels for interfacial band alignment. By scrutinization of the conjugation-linker and hole-transporting head, an optimal conjugated SAM (MPA-Ph-CA) in combination with the standard triple cation perovskite Cs0.05(FA0.92MA0.08)0.95Pb(I0.92Br0.08)3 achieved an efficient inverted PSC with a power conversion efficiency (PCE) of 22.53% (certified 22.12%). Moreover, the MPA-Ph-CA based devices showed excellent stability, retaining over 95% of their initial PCEs under one sun constant irradiation for 800 h. The synchronously enhanced efficiency and stability suggest that conjugated SAM-based HSCs are promising for further advancing inverted PSCs. |
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| AbstractList | The alkyl linker-based self-assembled monolayer (SAM) has emerged as an efficient hole-selective contact (HSC) for inverted perovskite solar cells (PSCs). Despite being effective in hole-extraction and interfacial passivation, its hole-transporting capability is limited by the insulating alkyl linker, along with poor stability due to the isolated and nonconjugated electron-rich moiety. Here, we report a series of conjugated SAMs that exhibit excellent photo- and electrical stabilities. The conjugated molecular structure not only enhances charge transport but also stabilizes the electron-rich arylamines through electron/charge delocalization. Moreover, it enables convenient modulation of frontier orbital energy levels for interfacial band alignment. By scrutinization of the conjugation-linker and hole-transporting head, an optimal conjugated SAM (MPA-Ph-CA) in combination with the standard triple cation perovskite Cs0.05(FA0.92MA0.08)0.95Pb(I0.92Br0.08)3 achieved an efficient inverted PSC with a power conversion efficiency (PCE) of 22.53% (certified 22.12%). Moreover, the MPA-Ph-CA based devices showed excellent stability, retaining over 95% of their initial PCEs under one sun constant irradiation for 800 h. The synchronously enhanced efficiency and stability suggest that conjugated SAM-based HSCs are promising for further advancing inverted PSCs. |
| Author | Wu, Yongzhen Zhang, Shuo Wang, Yanbo Mu, Chenkai Han, Liyuan Wu, Ruihan Zhu, Wei-Hong |
| AuthorAffiliation | Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering State Key Laboratory of Metal Matrix Composites |
| AuthorAffiliation_xml | – name: Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering – name: State Key Laboratory of Metal Matrix Composites |
| Author_xml | – sequence: 1 givenname: Shuo surname: Zhang fullname: Zhang, Shuo organization: Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering – sequence: 2 givenname: Ruihan surname: Wu fullname: Wu, Ruihan organization: Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering – sequence: 3 givenname: Chenkai surname: Mu fullname: Mu, Chenkai organization: Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering – sequence: 4 givenname: Yanbo surname: Wang fullname: Wang, Yanbo organization: State Key Laboratory of Metal Matrix Composites – sequence: 5 givenname: Liyuan orcidid: 0000-0001-9766-9015 surname: Han fullname: Han, Liyuan organization: State Key Laboratory of Metal Matrix Composites – sequence: 6 givenname: Yongzhen orcidid: 0000-0003-3000-403X surname: Wu fullname: Wu, Yongzhen email: wu.yongzhen@ecust.edu.cn organization: Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering – sequence: 7 givenname: Wei-Hong orcidid: 0000-0001-9103-166X surname: Zhu fullname: Zhu, Wei-Hong email: whzhu@ecust.edu.cn organization: Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Shanghai Key Laboratory of Functional Materials Chemistry, Frontiers Science Center for Materiobiology and Dynamic Chemistry, Institute of Fine Chemicals, School of Chemistry and Molecular Engineering |
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| Title | Conjugated Self-Assembled Monolayer as Stable Hole-Selective Contact for Inverted Perovskite Solar Cells |
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